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Comptes Rendus Physique

Measuring short range stray electric fields with a force quantum sensor

Yann Balland, Franck Pereira dos Santos

Published Oct 2, 2025• 0 citations
Publisher

Abstract

We use a quantum sensor based on trapped atom interferometry, and designed for probing short range atom-surface interactions, to characterize parasitic electric fields produced by adsorbed atoms or surface charges on a dielectric mirror. Applying controlled external fields with in-situ electrodes allows measuring electric field gradients with a relative uncertainty of order of 1% via variations of the force induced onto the atoms. More, our sensor can also be configured as a trapped microwave clock, allowing for direct measurements of the electric field amplitude via the Stark shift of the hyperfine transition frequency. Such measurements of the electric field amplitudes and gradients as a function of the atom-surface distance can be used to construct a model for the spatial distribution of the atoms adsorbed onto the surface of the mirror, and to accurately correct local force measurements, such as related to the Casimir–Polder interaction, from the detrimental impact of adsorbed atoms or stray charges.

DOI
10.5802/crphys.264

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We use a quantum sensor based on trapped atom interferometry, and designed for probing short range atom-surface interactions, to characterize parasitic electric fields produced by adsorbed atoms or surface charges on a dielectric mirror. Applying controlled external fields with in-situ electrodes allows measuring electric field gradients with a relative uncertainty of order of 1% via variations of the force induced onto the atoms. More, our sensor can also be configured as a trapped microwave clock, allowing for direct measurements of the electric field amplitude via the Stark shift of the hyperfine transition frequency. Such measurements of the electric field amplitudes and gradients as a function of the atom-surface distance can be used to construct a model for the spatial distribution of the atoms adsorbed onto the surface of the mirror, and to accurately correct local force measurements, such as related to the Casimir–Polder interaction, from the detrimental impact of adsorbed atoms or stray charges.
We report on the realization of a quantum sensor based on trapped atom interferometry in an optical lattice for the measurement of atom-surface interactions, with sub-micrometer-level control of the mean atom-surface separation distance. The force sensor reaches a short-term sensitivity of 3.4×10^{-28} N at 1 s and a long-term stability of 4 qN (4×10^{-30} N). We perform force measurements in the 0-300 μm range, and despite significant stray forces caused by adsorbed atoms on the surface, we obtain evidence of the Casimir-Polder force.
In this paper we demonstrate a technique of utilizing magnetically trapped neutral 87Rb^{87}\mathrm{Rb}87Rb atoms to measure the magnitude and direction of stray electric fields emanating from surface contaminants. We apply an alternating external electric field that adds to (or subtracts from) the stray field in such a way as to resonantly drive the trapped atoms into a mechanical dipole oscillation. The growth rate of the oscillation's amplitude provides information about the magnitude and sign of the stray field gradient. Using this measurement technique, we are able to reconstruct the vector electric field produced by surface contaminants. In addition, we can accurately measure the electric fields generated from adsorbed atoms purposely placed onto the surface and account for their systematic effects, which can plague a precision surface-force measurement. We show that baking the substrate can reduce the electric fields emanating from adsorbate and that the mechanism for reduction is likely surface diffusion, not desorption.
The authors propose a novel experiment based on atoms trapped close to a macroscopic surface, to study the interactions between the atoms and the surface at very small separations (0.6 to 10 mum). In this range the dominant potential is the QED interaction (Casimir-Polder and Van der Waals) between the surface and the atom. Additionally, several theoretical models suggest the possibility of Yukawa type potentials with sub-mm range, arising from new physics related to gravity. The paper proposes a set-up very similar to neutral atom optical lattice clocks, but with the atoms trapped in lattice sites close to the reflecting mirror. A sequence of pulses of the probe laser at different frequencies is then used to create an interferometer with a coherent superposition between atomic states at different distances from the mirror (in different lattice sites). Assuming atom interferometry state of the art measurement of the phase difference and a duration of the superposition of about 0.1s we expect to be able to measure the potential difference between separated states with an uncertainty of about 10-4Hz. A preliminary analysis of systematic effects for different atoms (Sr, Yb, Rb, Cs) indicates no fundamentally limiting effect at the same level of uncertainty, but does influence the choice of atom and isotope. Based on those estimates, we expect that such an experiment would improve the best existing measurements of the atom-wall QED interaction by <2 orders of magnitude, whilst gaining up to 4 orders of magnitude on the best present limits on new interactions in the range between 100 nm and 100mum
We describe an experiment based on atoms trapped close to a macroscopic surface, to study the interactions between the atoms and the surface at very small separations $(0.6--10\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{m})$. In this range the dominant potential is the QED interaction (Casimir-Polder and van der Waals) between the surface and the atom. Additionally, several theoretical models suggest the possibility of Yukawa-type potentials with sub-millimeter range, arising from new physics related to gravity. The proposed setup is very similar to neutral atom optical lattice clocks, but with the atoms trapped in lattice sites close to the reflecting mirror. A sequence of pulses of the probe laser at different frequencies is then used to create an interferometer with a coherent superposition between atomic states at different distances from the mirror (in different lattice sites). Assuming atom interferometry state-of-the-art measurement of the phase difference and a duration of the superposition of about 0.1s0.1\phantom{\rule{0.3em}{0ex}}\mathrm{s}0.1s, we expect to be able to measure the potential difference between separated states with an uncertainty of $\ensuremath{\approx}{10}^{\ensuremath{-}4}\phantom{\rule{0.3em}{0ex}}\mathrm{Hz}$. An analysis of systematic effects for different atoms and surfaces indicates no fundamentally limiting effect at the same level of uncertainty, but does influence the choice of atom and surface material. Based on those estimates, we expect that such an experiment would improve the best existing measurements of the atom-wall QED interaction by \ensuremath{\geqslant} 2 orders of magnitude, while gaining up to four orders of magnitude on the best present limits on new interactions in the range between 100nm100\phantom{\rule{0.3em}{0ex}}\mathrm{nm}100nm and $100\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{m}$.
Highly excited (Rydberg) atoms have exaggerated properties making them extremely sensitive to external electromagnetic fields and interacting strongly with their environment. Atomic vapor cells represent an attractive platform for studying Rydberg atoms and fabricating quantum devices. For example, Rydberg atoms in vapor cells have been used as sensitive detectors of electric fields of frequencies ranging from DC up to the THz range but also as single photon sources for quantum technology applications exploiting collective phenomena due to the Rydberg blockade effect [1]. Rydberg atoms also find applications in fundamental physics, in particular for the measurement of dispersive interactions of the Casimir-Polder type (atom-surface interactions) [2]. One major advantage of Rydberg atoms is that they expose limitations in the traditional perturbative approach of Casimir-Polder (CP) theory [3, 4]. Indeed, in the extreme near-field, the dipole approximation breaks down and higher-order terms need to be considered. We report on extensive experimental measurements of the Rydberg-surface interaction using spectroscopy in cesium vapor nanocells of a thickness ranging roughly from 200-700nm, as well as selective reflection spectroscopy on a macroscopic cesium all-sapphire cell. Atoms are first excited to the Cs(6P) level with a 894nm pump laser and subsequently a green laser ≈ 510nm probes Rydberg nD or nS states, where the principal quantum number n ranges between 15-17. Our experiments evidence the dipole-dipole term of the Casimir-Polder interaction providing a measurement of the C3 coefficient for cesium Rydberg states. Furthermore, our experiment clearly evidences an additional interaction that induces shifts and broadens the linewidth of the probed transitions in the vicinity of the dielectric windows of our cells. We believe that this interaction is due to electric fields that are either generated by patch charges (trapped on the surface or induced by the excitation lasers), or by cesium adsorbants. We show that the different polarizability (of opposing sign) between S and D Rydberg states can be exploited to extract quantitative measurements of the strength and distance scaling (z-dependence) of such parasitic electrostatic interactions.Our experiments suggest that the sensitivity of Rydberg atoms to external electric fields could provide a unique tool for probing electrostatic interactions in the vicinity of surfaces. This could allow systematic error corrections in Casimir-Polder experiments with excited or even ground state atoms that aim at putting bounds on the existence of non-Newtonian gravity [5]. We are currently exploring the possibility of coating the internal window interfaces with conducting 2D material such as graphene to reduce the influence of parasitic charges. This could allow us to probe atoms closer to the surface, where quadrupole interactions could be experimentally attainable for the first time [4].References[1] H. Kubler, J. P. Shaffer, T. Baluktsian, R. Loew, T. Pfau, Nat. Photon., 4, 112–116 (2013).[2] V. Sandoghdar et al., Phys. Rev. Lett 68, 3432–3435 (1993).[3] J. A. Crosse et al., Phys. Rev. A 82, 3010901 (2010).[4] B. Dutta et al., Phys. Rev. Res. 6, L022035 (2024).[5] A. Laliotis, B-S. Lu, M. Ducloy, D. Wilkowski, AVS Quantum Sci. 3, 043501 (2021).