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arXiv:0705.2027 · Physical Review A

Measuring electric fields from surface contaminants with neutral atoms

John Obrecht, Robert J. Wild, Eric Cornell

Published Jun 19, 2007• 80 citations
arXivHTMLPDF

Abstract

In this paper we demonstrate a technique of utilizing magnetically trapped neutral $^{87}\mathrm{Rb}$ atoms to measure the magnitude and direction of stray electric fields emanating from surface contaminants. We apply an alternating external electric field that adds to (or subtracts from) the stray field in such a way as to resonantly drive the trapped atoms into a mechanical dipole oscillation. The growth rate of the oscillation's amplitude provides information about the magnitude and sign of the stray field gradient. Using this measurement technique, we are able to reconstruct the vector electric field produced by surface contaminants. In addition, we can accurately measure the electric fields generated from adsorbed atoms purposely placed onto the surface and account for their systematic effects, which can plague a precision surface-force measurement. We show that baking the substrate can reduce the electric fields emanating from adsorbate and that the mechanism for reduction is likely surface diffusion, not desorption.

DOI
10.1103/physreva.75.062903

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In this paper we demonstrate a technique of utilizing magnetically trapped neutral 87Rb^{87}\mathrm{Rb}87Rb atoms to measure the magnitude and direction of stray electric fields emanating from surface contaminants. We apply an alternating external electric field that adds to (or subtracts from) the stray field in such a way as to resonantly drive the trapped atoms into a mechanical dipole oscillation. The growth rate of the oscillation's amplitude provides information about the magnitude and sign of the stray field gradient. Using this measurement technique, we are able to reconstruct the vector electric field produced by surface contaminants. In addition, we can accurately measure the electric fields generated from adsorbed atoms purposely placed onto the surface and account for their systematic effects, which can plague a precision surface-force measurement. We show that baking the substrate can reduce the electric fields emanating from adsorbate and that the mechanism for reduction is likely surface diffusion, not desorption.
We use a quantum sensor based on trapped atom interferometry, and designed for probing short range atom-surface interactions, to characterize parasitic electric fields produced by adsorbed atoms or surface charges on a dielectric mirror. Applying controlled external fields with in-situ electrodes allows measuring electric field gradients with a relative uncertainty of order of 1% via variations of the force induced onto the atoms. More, our sensor can also be configured as a trapped microwave clock, allowing for direct measurements of the electric field amplitude via the Stark shift of the hyperfine transition frequency. Such measurements of the electric field amplitudes and gradients as a function of the atom-surface distance can be used to construct a model for the spatial distribution of the atoms adsorbed onto the surface of the mirror, and to accurately correct local force measurements, such as related to the Casimir–Polder interaction, from the detrimental impact of adsorbed atoms or stray charges.
Experiments handling Rydberg atoms near surfaces must necessarily deal with the high sensitivity of Rydberg atoms to (stray) electric fields that typically emanate from adsorbates on the surface. We demonstrate a method to modify and reduce the stray electric field by changing the adsorbate distribution. We use one of the Rydberg excitation lasers to locally affect the adsorbed dipole distribution. By adjusting the averaged exposure time we change the strength (with the minimal value less than 0.2V/cm0.2\phantom{\rule{0.28em}{0ex}}\mathrm{V}/\mathrm{cm}0.2V/cm at $78\phantom{\rule{0.28em}{0ex}}\ensuremath{\mu}\mathrm{m}$ from the chip) and even the sign of the perpendicular field component. This technique is a useful tool for experiments handling Rydberg atoms near surfaces, including atom chips.
Trapping a Rydberg atom close to a surface is an important step towards the realisation of many proposals for quantum information processing or hybrid quantum systems. One of the challenges in these experiments is posed by the electric field emanating from contaminations on the surface. Here we report on measurements of an electric field created by 87 Rb atoms adsorbed on a 25 nm thick layer of SiO 2 , covering a 90 nm layer of Au. The electric field is measured using a two-photon transition to the and states. The electric field value that we measure is higher than typical values measured above metal surfaces, but is consistent with a recent measurement above a SiO 2 surface. In addition, we measure the temporal behaviour of the field and observe that we can reduce it in a single experimental cycle, using ultraviolet light or by mildly locally heating the surface with one of the excitation lasers, whereas the buildup of the field takes thousands of cycles. We explain these results by a change in the adatom distribution on the surface. These results indicate that, while the stray electric field can be reduced, achieving field-free conditions above a silica-coated gold chip remains challenging.
A magnetically trapped 87Rb^{87}\mathrm{Rb}87Rb Bose-Einstein condensate is used as a sensitive probe of short-range electrical forces. In particular, the electric polarization of, and the subsequent electric field generated by, 87Rb^{87}\mathrm{Rb}87Rb adsorbates on conducting and insulating surfaces is measured by characterizing perturbations to the magnetic trapping potential using high quality factor condensate excitations. The nature of the alterations to the electrical properties of Rb\mathrm{Rb}Rb adsorbates is studied on titanium (metal) and silicon (semiconductor) surfaces, which exhibit nearly identical properties, and on glass (insulator), which displays a smaller transitory electrical effect. The limits of this technique in detecting electrical fields and ramifications for measurements of short-range forces near surfaces are discussed.
The ability to characterize static and time-dependent electric fields in situ is an important prerequisite for quantum-optics experiments with atoms close to surfaces. Especially in experiments which aim at coupling Rydberg atoms to the near field of superconducting circuits, the identification and subsequent elimination of sources of stray fields are crucial. We present a technique that allows the determination of stray-electric-field distributions $[{F}_{\mathrm{x}}^{\mathrm{str}}(\stackrel{P\vec}{r}),{F}_{\mathrm{y}}^{\mathrm{str}}(\stackrel{P\vec}{r}),{F}_{\mathrm{z}}^{\mathrm{str}}(\stackrel{P\vec}{r})]$ at distances of less than 2 mm from (cryogenic) surfaces using coherent Rydberg-Stark spectroscopy in a pulsed supersonic beam of metastable 1s12s11S01{s}^{1}2{s}^{1}{}^{1}{S}_{0}1s12s11S0​ helium atoms. We demonstrate the capabilities of this technique by characterizing the electric stray field emanating from a structured superconducting surface. Exploiting coherent population transfer with microwave radiation from a coplanar waveguide, the same technique allows the characterization of the microwave-field distribution above the surface.
Rydberg-assisted atomic electrometry with thermal vapors offers a promising approach for detecting external electric fields. However, this technique presents significant challenges for measuring low frequencies due to the effects of metal-alkali atoms adsorbed on the interior surface of the vacuum chamber. In this work, we apply high-contrast Rydberg electromagnetically induced transparency (EIT) spectroscopy to systematically investigate these effects, including the influence of laser power and electric field strength. We demonstrate the ability to measure electric field frequencies ranging from 10 Hz to 1 MHz. Additionally, this study identifies a fundamental limit for data capacity in such measurements. Furthermore, we propose a method for precise Stark shift measurements by locking the coupling laser to Zeeman-split Rydberg EIT peaks. Using the Zeeman shift in a reference cell as a stable frequency reference, we are able to track Stark-induced shifts in a science cell and confirm excellent agreement with theoretical predictions. These results provide valuable insights for future precision measurement techniques and field sensing applications based on Rydberg atom systems.