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Optics Express

Collective reflectivity from a one-dimensional dense chain of atoms

Sung-Mi Yoo, Juha Javanainen

Published Sep 1, 2025• 0 citations
Publisher

Abstract

We theoretically develop a quantum-mechanical scheme to study propagation of a laser beam through a one-dimensional (1D) dense chain of N effective two-level cold atoms tightly fixed in a free space. Atoms with half a wavelength separation are modeled as a collection of spins with angular momenta ±12, being at equivalent field positions. At an arbitrary driving field, we derive a reflectivity in terms of coherences between N + 1 collective eigenstates of the atoms from the steady-state solutions of the quantum master equation. We unravel that the reflectivity of incident light arises from scattering of electric fields in backward direction from the participating dipoles in the excitation. We identified splitting of reflectivity plotted as a function of detuning of incident light from atomic resonance as the Autler-Townes (AT) effect. Our scheme finds that the width of this reflectivity dip is scaled as a function of a ratio of the driving field frequency to the collective decay rate.

DOI
10.1364/oe.568491

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We theoretically develop a quantum-mechanical scheme to study propagation of a laser beam through a one-dimensional (1D) dense chain of N effective two-level cold atoms tightly fixed in a free space. Atoms with half a wavelength separation are modeled as a collection of spins with angular momenta ±12, being at equivalent field positions. At an arbitrary driving field, we derive a reflectivity in terms of coherences between N + 1 collective eigenstates of the atoms from the steady-state solutions of the quantum master equation. We unravel that the reflectivity of incident light arises from scattering of electric fields in backward direction from the participating dipoles in the excitation. We identified splitting of reflectivity plotted as a function of detuning of incident light from atomic resonance as the Autler-Townes (AT) effect. Our scheme finds that the width of this reflectivity dip is scaled as a function of a ratio of the driving field frequency to the collective decay rate.
Manipulation of light using atoms plays a fundamental and important role in emerging technologies such as integrated photonics, information storage, and quantum sensors. Specifically, there have been intense theoretical efforts involving large samples of cold neutral atoms for coherent control of light. Here we present a theoretical scheme that enables efficient computation of collective optical responses of mono- and bi-layer planar square lattices of dense, cold two-level atoms using classical electrodynamics of coupled dipoles in the limit of low laser intensity. The steady-state transmissivity and reflectivity are obtained at a field point far away from the atomic lattices in the regime with no Bragg reflection. While our earlier method was based on exact solution of the electrodynamics for a small-scale lattice, here we calculate the dipole moments assuming that they are the same at all lattice sites, as for an infinite lattice. Atomic lattices with effectively over one hundred times more sites than in our earlier exact computations can then be simulated numerically with fewer computational resources. We have implemented an automatic selection of the number of sites under the given convergence criteria. We compare the numerical results from both computational schemes. We also find similarities and differences of a stack of two atomic lattices from a two-atom sample. Such aspects may be exploited to engineer a stack for potential applications.
Light–matter interaction in cold atomic ensembles is one of the central topics in modern quantum and atomic optics with important applications in various quantum technologies. The collective response of dense atomic gases under light excitation depends crucially on the spatial distribution of atoms and the geometry of the ensemble. We analyze near-resonant light transmission in two-dimensional dense ultracold atomic ensembles with short-range positional correlations. Based on coupled-dipole simulations, we show that the collective effects, manifested as notable shifts of transmission resonance frequency and considerable modification of optical depths, are influenced strongly by positional correlations. Mean-field theories such as the Lorentz–Lorenz relation are not capable of describing such collective effects. We also investigate the statistical distribution of eigenstates and provide a connection between the transmission spectra and eigenstate distribution by utilizing the population weighted detuning and decay rate of all eigenstates. We further demonstrate the intricate interplay between dipole–dipole interactions and positional correlations by increasing the number densities of atoms.
We experimentally study resonant light scattering by a one-dimensional randomly filled chain of cold two-level atoms. By a local measurement of the light scattered along the chain, we observe constructive interferences in light-induced dipole-dipole interactions between the atoms. They lead to a shift of the collective resonance despite the average interatomic distance being larger than the wavelength of the light. This result demonstrates that strong collective effects can be enhanced by structuring the geometrical arrangement of the ensemble. We also explore the high intensity regime where atoms cannot be described classically. We compare our measurement to a mean-field, nonlinear coupled-dipole model accounting for the saturation of the response of a single atom.
Abstract A cloud of cold N two‐level atoms driven by a resonant laser beam shows cooperative effects both in the scattered radiation field and in the radiation pressure force acting on the cloud center‐of‐mass. The induced dipoles synchronize and the scattered light presents superradiant and/or subradiant features. We present a quantum description of the process in terms of a master equation for the atomic density matrix in the scalar, Born‐Markov approximations, reduced to the single‐excitation limit. From a perturbative approach for weak incident field, we derive from the master equation the effective Hamiltonian, valid in the linear regime. We discuss the validity of the driven timed Dicke ansatz and of a partial wave expansion for different optical thicknesses and we give analytical expressions for the scattered intensity and the radiation pressure force on the center of mass. We also derive an expression for collective suppression of the atomic excitation and the scattered light by these correlated dipoles.
This poster presents a first analysis of the laws of reflection of cold atoms by an evanescent wave atomic mirror. We demonstrate that when the laser beam is tuned to the blue of the atomic transition, i.e, for a positive frequency detuning compared to the frequency resonance Δ = ωL−ωa, there is a reflection without a contact with the surface of the prism (no adsorption). The condition for an internal total reflection is θ>θc = arcsin (1/n) where θ is the incidence angle of the laser wave on the internal face of the prism and n is its refraction index. The evanescent wave is parallel to the surface and propagates over few wavelengths only for θ = θc. The atomic trajectory is such as the incidence angle φi is different from the reflection angle φr (non respect of the first law of reflection in photonic optics). We’ll have to demonstrate the reflection law in atom optics and give numerical examples as an illustration [1]. At its interaction with the evanescent wave, the atom is submitted to a pressure radiation force Fx parallel to the surface of separation which communicates a quantity of motion in the direction of the x axis. It is also submitted to a dipolar force Fy perpendicular to the separation surface responsible of the repulsion of cold atoms in the case where we neglect the Van der Waals forces. We define R as the ratio of two forces Fx and Fy. Their expressions, function of the detuning, are given by the Ehrenfest theorem and the Bloch equations [2]. When the ratio R tends towards zero (spontaneous emission negligible for a detuning important compared to natural linewidth of the excited state), the first law of Descartes reflection is thus satisfied idem φi = φr Thus, it is simple to demonstrate that the atomic trajectories obey to the general reflection law: tg φr = tg φi−2R where R is independent of the spatial component. Its expression is given by the ratio of the velocity transfers Δvx to Δvy. The case of retro‐reflection seen in quasi normal incidence and for values of the ratio R different from zero (φi = −φr) is also examined. In the case where the value of the ratio R is non null, we may demonstrate that the incidence plan is different from the reflection plan (second law of Descartes reflection).
Collective coupling between dipoles can dramatically modify the optical response of a medium. Such effects depend strongly on the geometry of the medium and the polarization of the light. Using a classical coupled dipole model, here we investigate the simplest case of one-dimensional arrays of interacting atomic dipoles driven by a weak laser field. Changing the polarization and direction of the driving field allows us to separately address superradiant, subradiant, redshifted, and blueshifted eigenmodes, as well as observe strong Fano-like interferences between different modes. The cooperative eigenvectors can be characterized by the phase difference between nearest-neighbor dipoles, ranging from all oscillating in phase to all oscillating out of phase with their nearest neighbors. Investigating the eigenvalue behavior as a function of atom number and lattice spacing, we find that certain eigenmodes of an infinite atomic chain have the same decay rate as a single atom between two mirrors. The effects we observe provide a framework for collective control of the optical response of a medium, giving insight into the behavior of more complicated geometries, as well as providing further evidence for the dipolar analog of cavity QED.