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Optics Express

Spatial symmetry-broken atomic magnetometry

S.S. Park, Min-Hwan Lee, Heung‐Sik Kim, Jihyeong Ju, S. A. Lee, Jaeuk Baek, Heung‐Ryoul Noh, Geol Moon

Published Aug 26, 2025• 0 citations
Publisher

Abstract

We report an atomic magnetic sensor that leverages the spatial symmetry-broken (SSB) properties of the four-wave mixing (FWM) process induced by an external weak magnetic field. The dispersive signals around the center of zero magnetic field are obtained from counterpropagating polarization-selective FWM signals in a rubidium vapor cell. The SSB magnetometer has a linear response within −5 μT to 5 μT, and the magnetic sensitivity is about 10 $pT/Hz$ at 10 Hz, and the bandwidth is in the range of 18.25 kHz. This method would open diverse applications ranging from biomagnetic sensing to Earth’s magnetic field mapping as a robust atomic magnetic sensor.

DOI
10.1364/oe.568742

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•Jul 19, 2022•0 citations
We report an atomic magnetic sensor that leverages the spatial symmetry-broken (SSB) properties of the four-wave mixing (FWM) process induced by an external weak magnetic field. The dispersive signals around the center of zero magnetic field are obtained from counterpropagating polarization-selective FWM signals in a rubidium vapor cell. The SSB magnetometer has a linear response within −5 μT to 5 μT, and the magnetic sensitivity is about 10 pT/HzpT/HzpT/Hz at 10 Hz, and the bandwidth is in the range of 18.25 kHz. This method would open diverse applications ranging from biomagnetic sensing to Earth’s magnetic field mapping as a robust atomic magnetic sensor.
The nonlinear magneto-optical effect has significantly impacted modern society with prolific applications ranging from precision mapping of the Earth's magnetic field to bio-magnetic sensing. Pioneering works on collisional spin-exchange effects have led to ultra-high magnetic field detection sensitivities at the level of fT/HzfT/\sqrt{Hz}fT/Hz​ using a single linearly-polarized probe light field. Here we demonstrate a nonlinear Zeeman-coherence parametric wave-mixing optical-atomic magnetometer using room temperature rubidium vapor that results in more than a three-order-of-magnitude optical signal-to-noise ratio (SNR) enhancement for extremely weak magnetic field sensing. This unprecedented enhancement was achieved with nearly a two-order-of-magnitude reduction in laser power while preserving the sensitivity of the widely-used single-probe beam optical-atomic magnetometry method. This new method opens a myriad of applications ranging from bio-magnetic imaging to precision measurement of the magnetic properties of subatomic particles.
We report a rubidium atomic magnetometer based on pump-probe nonlinear magneto-optical rotation. The rubidium vapor cell is placed in a five-layer magnetic shield with inner coils that can generate uniform magnetic fields along the direction of pump beam, and the cell is also placed in the center of a Helmholtz coil that can generate an oscillating magnetic field perpendicular to the direction of pump beam. The atoms are optically pumped by circularly polarized pump beam along a constant magnetic field in a period of time, then the pump beam is turned off and a /2 pulse of oscillating magnetic field for 87Rb atoms is applied. After the above process, the individual atomic magnetic moments become phase coherent, resulting in a transverse magnetization vector precessing at the Larmor frequency in the magnetic field. The linearly polarized probing beam is perpendicular to the direction of magnetic field, and can be seen as a superposition of the left and right circularly polarized light. Because of the different absorptions and dispersions of the left and right circularly polarized light by rubidium atoms, the polarization direction of probing beam rotates when probing beam passes through rubidium vapor cell. The rotation of the polarization is subsequently converted into an electric signal through a polarizing beam splitter. Finally, the decay signal related to the transverse magnetization vector is measured. The Larmor frequency proportional to magnetic field is obtained by the Fourier transform of the decay signal. The value of magnetic field is calculated from the formula:B=(2/) f, where and f are the gyromagnetic ratio and Larmor frequency, respectively. In order to measure the magnetic field in a wide range, the tracking lock mode is proposed and tested. The atomic magnetometer can track the magnetic field jump of 1000 nT or 10000 nT, indicating that the atomic magnetometer has strong locking ability and can be easily locked after start-up. The main performances in different magnetic fields are tested. The results show that the measurement range of the atomic magnetometer is from 100 nT to 100000 nT, the extreme sensitivity is 0.2 pT/Hz1/2, and the magnetic field resolution is 0.1 pT. The transverse relaxation times of the transverse magnetization vector in different magnetic fields are obtained, and the relaxation time decreases with the increase of the magnetic field. When the measurement range is from 5000 nT to 100000 nT, the magnetic field sampling rate of the atomic magnetometer can be adjusted in a range from 1 Hz to 1000 Hz. The atomic magnetometer in high sampling rate can measure weak alternating magnetic field at low frequency. This paper provides an important reference for developing the atomic magnetometer with large measurement range, high sensitivity and high sampling rate.
We demonstrated a scalar atomic magnetometer using a microfabricated Cs vapor cell. The atomic spin precession is driven by an amplitude-modulated circularly-polarized pump laser resonant on the D1 transition of Cs atoms and detected by an off-resonant linearly-polarized probe laser using a balanced polarimeter setup. Under a magnetic field with amplitude in the Earth's magnetic field range, the magnetometer in the gradiometer mode can reach sensitivities below 150fT/√Hz, which shows that the magnetometer by itself can achieve sub-100fT/√Hz sensitivities. In addition to its high sensitivity, the magnetometer has a bandwidth close to 1 kHz due to the broad magnetic resonance inside the small vapor cell. Our experiment suggests the feasibility of a portable low-power and high-performance magnetometer which can be operated in the Earth's magnetic field. Such a device will greatly reduce the restrictions on the operating environment and expand the range of applications for atomic magnetometers, such as detection of nuclear magnetic resonance in low magnetic fields
We demonstrated a scalar atomic magnetometer using a microfabricated Cs vapor cell. The atomic spin precession is driven by an amplitude-modulated circularly-polarized pump laser resonant on the D1 transition of Cs atoms and detected by an off-resonant linearly-polarized probe laser using a balanced polarimeter setup. Under a magnetic field with amplitude in the Earth's magnetic field range, the magnetometer in the gradiometer mode can reach sensitivities below 150fT/Hz, which shows that the magnetometer by itself can achieve sub-100fT/Hz sensitivities. In addition to its high sensitivity, the magnetometer has a bandwidth close to 1 kHz due to the broad magnetic resonance inside the small vapor cell. Our experiment suggests the feasibility of a portable low-power and high-performance magnetometer which can be operated in the Earth's magnetic field. Such a device will greatly reduce the restrictions on the operating environment and expand the range of applications for atomic magnetometers, such as detection of nuclear magnetic resonance in low magnetic fields.
Here we demonstrate an atomic magnetometer that has a bandwidth of more than 100 kHz and a sensitivity of $180\phantom{\rule{0.2em}{0ex}}\mathrm{fT/}\ensuremath{\surd}\mathrm{Hz}$ at a Fourier frequency of 8 Hz, and $0.7\phantom{\rule{0.2em}{0ex}}\mathrm{nT/}\ensuremath{\surd}\mathrm{Hz}$ at 100 kHz. These sensitivity measurements are achieved at geophysically useful magnetic field magnitudes (approximately $50\phantom{\rule{0.2em}{0ex}}\ensuremath{\mu}\mathrm{T}$ inside a three-layer $\ensuremath{\mu}$-metal shield) and are limited by the photon shot noise for frequencies above 8 Hz. This device is based on a nonlinear magneto-optical rotation sensor that is operated with an active feedback to the pump modulation frequency. We present a theoretical description of the response functions of the components in the magnetometer. We show that the range of operation of atomic magnetometers can thus be expanded beyond the conventional high-sensitivity, low-bandwidth domain, to provide a high-linearity, high-bandwidth, and high-sensitivity sensor.
We demonstrate an ultra-high sensitivity rf optical magnetometer based on a compact 5×5×8 mm3 Rubidium-87 vapor cell in a mu-metal shielded environment. The rf field is detected via a Faraday rotation effect on the linear polarization of a probe beam, and the resonance frequency is tuned via Zeeman effect by applying a static bias magnetic field to the cell. Sensitivities down to 3 fT/√Hz are achieved between 10 kHz and 100 kHz, which is a performance comparable to that of prior larger cells. An increase in the sensitivity with frequency and temperature has been observed.