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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Base-Independent Photon Entanglement in Superradiance of Multilevel Atoms

Amir Sivan, Meir Orenstein

Published Jun 23, 2025• 0 citations
Publisher

Abstract

We propose realization of sources of multiphoton entanglement from atomic ensembles via a fast and deterministic superradiance process [1]. We leverage the collective emission phenomenon of superradiance in order to generate multiphoton states, and entangle them in their frequency degree of freedom by incorporating the dynamics of multilevel atoms. Such deterministic high-yield sources of entangled photons are crucial for applications pertaining to quantum computation, quantum communications and quantum metrology [2]. We emphasize that the original Dicke superradiance model [3] and its extensions have only dealt with the atomic-ensemble entanglement and photonic ensemble-average observables such as intensity and autocorrelation, and photonic entanglement in superradiance has never been considered.

DOI
10.1109/cleo/europe-eqec65582.2025.11109879

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We propose realization of sources of multiphoton entanglement from atomic ensembles via a fast and deterministic superradiance process [1]. We leverage the collective emission phenomenon of superradiance in order to generate multiphoton states, and entangle them in their frequency degree of freedom by incorporating the dynamics of multilevel atoms. Such deterministic high-yield sources of entangled photons are crucial for applications pertaining to quantum computation, quantum communications and quantum metrology [2]. We emphasize that the original Dicke superradiance model [3] and its extensions have only dealt with the atomic-ensemble entanglement and photonic ensemble-average observables such as intensity and autocorrelation, and photonic entanglement in superradiance has never been considered.
We show here that the photonic states emitted by ensembles of multilevel atoms via a superradiance process exhibit entanglement in the modal (frequency) degree of freedom, making this collective emission process a favorable candidate for a fast, bright, and deterministic source of entangled photons. This entanglement is driven by two mechanisms: (i) selective excitation of the atomic ensemble to a superposition state, and (ii) degeneracies of the optical transitions owing to the internal structure of the emitting atoms. The latter induces intricate nonradiative virtual transitions in the ensemble, which create interatomic correlations that are imprinted onto the emitted photons. One of the important outcomes of this complexity is the generation of mode-independent entangled multiphoton states. In addition, we study the dynamics of the correlations of the superradiating multilevel atom ensembles, and demonstrate a case where they exhibit beating in steady state as a result of the aforementioned virtual transitions.
Superradiance is one of the most fundamental collective quantum phenomena in light-matter interactions and has been studied extensively since Dicke's seminal work. However, its practical implementation remains challenging because superradiant enhancement requires strict experiment conditions for strong collective coupling among emitters. Can superradiance emerge in a simple platform, such as an atomic vapor cell composed of thermally moving atoms? To address this question, we identify the key signatures of superradiance in a hot atomic ensemble and find a use case of superradiance using an atomic vapor cell. Here, the Photon-Pair SuperRadiance (PPSR) process in an atomic vapor cell provides a novel approach to generating superradiant quantum light from a practical atomic platform. We experimentally demonstrate a superradiant entangled photon-pair generation via PPSR process in a high-density, 1-mm-long chip-scale Cs vapor cell. The hot, dense atomic vapor cell allows the mean interatomic distance in the Doppler-broadened atomic ensemble to be reduced to 0.29 times the idler-photon wavelength, satisfying the condition for cooperative emission. The thin chip-scale geometry enables high atomic densities while mitigating the reabsorption of emitted photons and maintaining moderate optical depth. In this subwavelength regime, we clearly observe the temporal narrowing of the biphoton wavefunction from 0.60 ns to 0.17 ns due to a superradiant decay. This pronounced temporal compression provides strong evidence of collective superradiant emission in the chip-scale Cs vapor cell. Our PPSR source delivers a detected photon-pair rate exceeding 10^6 pairs/s while maintaining a high coincidence-to-accidental ratio of 280.
The interaction of an ensemble of atoms with common vacuum modes may lead to an enhanced emission into these modes. This phenomenon, known as superradiance, highlights the coherent nature of spontaneous emission, resulting in macroscopic entangled states in mundane situations. The complexity of the typical observations of superradiance, however, masks its quantum nature, allowing alternative classical interpretations. Here we stress how this picture changed with the implementation ten years ago of a new process for single-photon generation from atomic ensembles. We present then the last piece of evidence for the superradiant nature of such a process, reporting the observation of an accelerated emission of the photon with a rate that may be tuned by controllably changing the number of atoms in the ensemble. We hope such an investigation will help open up a new bottom-up approach to the study of superradiance.
Dicke superradiance by an ensemble of quantum emitters produces a collective burst of radiation, but no entanglement in the mixed state of the emitters. We show that adding a local kinetic constraint between the emitters generates extensive mixed-state entanglement, while otherwise preserving all key features of Dicke superradiance. Specifically, for any local Boolean constraint, we analytically derive a lower bound for the emission rate which implies a peak intensity ∝N2\propto N^2∝N2 and a peak time ∝(log⁡N)/N\propto (\log N)/N∝(logN)/N with number of spins NNN. This effect enables the superradiantly accelerated preparation of entangled dark states. Hereby, Hilbert-space fragmentation of the Dicke ladder leads to an exponentially branching decay tree that generates a hierarchy of dark states. Importantly, these disconnected manifolds include exponentially many long-range entangled singlet dark states. The explored kinetic constraints and superradiant dynamics can be realized in neutral-atom arrays coupled to an optical cavity, and we suggest a simple and accessible witness to detect the predicted mixed-state entanglement in such experiments. Moreover, we show that entanglement generation is robust against atomic decay and collective dephasing, and should be observable under recently reported experimental conditions. Our results, thereby, offer a general framework and experimentally viable approach for the dissipative engineering of entangled dark states enhanced by superradiance.