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AIP Advances

Electric field measurement using a three-photon double-dark-state model in Rydberg atoms

Dongping Xiao, Xutao Wei, Sheng Yan, Huaiqing Zhang

Published Jul 1, 2025• 2 citations
Publisher

Abstract

Rydberg atoms, leveraging their unique properties, have been increasingly investigated and applied in the field of electric field measurement, demonstrating significant advantages. Nevertheless, challenges persist in measuring low-frequency electric fields below kHz, including difficulties in field loading and weak field effects. To address these issues and enable the measurement of weak low-frequency electric fields below kHz, we propose a novel measurement scheme based on a Double-Dark State Three-Photon System (DDSTPS). The proposed scheme overcomes the shielding effect of the glass vapor cell by employing a built-in electrode plate sampling technique and adjusting the electric field loading method. A three-photon double-dark-state system model was established, utilizing an inverted Y-type system structure. This configuration ensures that the dark state generated during the excitation of the atomic ground state is further excited to the intermediate state through photon interactions. The increased population of atoms in the intermediate state significantly enhances the resolution of the transmission spectrum. Compared to conventional two-photon three-level systems, the proposed scheme improves the maximum slope of the electromagnetically induced transparency (EIT) spectral peak by 122.53% and reduces the full width at half maximum (FWHM) of the spectral peak by more than half. When compared to experimental data from two-photon systems, the FWHM is narrowed by a factor of eight, substantially improving the resolution of the EIT spectrum and further advancing the performance of Rydberg atom-based electric field measurements. In addition, this study investigates the response of DDSTPS under low-frequency electric fields and analyzes its optimal operational region.

DOI
10.1063/5.0265975

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Acta Physica Sinica•Jan 1, 2025•0 citations
Rydberg atoms, leveraging their unique properties, have been increasingly investigated and applied in the field of electric field measurement, demonstrating significant advantages. Nevertheless, challenges persist in measuring low-frequency electric fields below kHz, including difficulties in field loading and weak field effects. To address these issues and enable the measurement of weak low-frequency electric fields below kHz, we propose a novel measurement scheme based on a Double-Dark State Three-Photon System (DDSTPS). The proposed scheme overcomes the shielding effect of the glass vapor cell by employing a built-in electrode plate sampling technique and adjusting the electric field loading method. A three-photon double-dark-state system model was established, utilizing an inverted Y-type system structure. This configuration ensures that the dark state generated during the excitation of the atomic ground state is further excited to the intermediate state through photon interactions. The increased population of atoms in the intermediate state significantly enhances the resolution of the transmission spectrum. Compared to conventional two-photon three-level systems, the proposed scheme improves the maximum slope of the electromagnetically induced transparency (EIT) spectral peak by 122.53% and reduces the full width at half maximum (FWHM) of the spectral peak by more than half. When compared to experimental data from two-photon systems, the FWHM is narrowed by a factor of eight, substantially improving the resolution of the EIT spectrum and further advancing the performance of Rydberg atom-based electric field measurements. In addition, this study investigates the response of DDSTPS under low-frequency electric fields and analyzes its optimal operational region.
Introduction: Rydberg atoms are ideal for measuring electric fields due to their unique physical properties. However, low-frequency electric fields below MHz can be challenging due to the accumulation of ionized free electrons on the atomic vapor cell’s surface, acting as a shield. Method: This paper proposes a Cavity-enhanced three-photon system (CETPS) measurement scheme, which uses a long-wavelength laser to excite the Rydberg state, reducing atomic ionization and enhancing detection spectrum resolution. A theoretical model is proposed to explain the quantum coherence effect of the light field, measured electric field, and the atomic system. Result: The results show that the proposed scheme significantly increases the electromagnetically induced transparency (EIT) spectral peak and narrows the spectral width, resulting in the maximum slope increasing by more than an order of magnitude. Discussion: The paper also discusses the impact of the Rabi frequency of the two laser fields and the coupling coefficient of the optical cavity on the transmission spectrum amplitude and linewidth, along with the optimal configuration of these parameters in the CEPTS scheme.
We demonstrate the measurement of super low-frequency electric field using Rydberg atoms in an atomic vapor cell with inside parallel electrodes, thus overcoming the low-frequency electric-field-screening effect at frequencies below a few kHz. Rydberg electromagnetically induced transparency (EIT) spectra involving 52 D 5/2 state is employed to measure the signal electric field. An auxiliary DC field is applied to improve the sensitivity. A DC Stark map is demonstrated, where the utilized 52 D 5/2 exhibits m j = 1/2, 3/2, 5/2 Stark shifts and splittings. The m j = 1/2 state is employed to detect the signal field because of its larger polarizability than that of m j = 3/2, 5/2. Also, we show that the strength of the spectrum is dependent on the angle between the laser polarizations and the electric field. With optimization of the applied DC field to shift the m j = 1/2 Rydberg energy level to a high sensitivity region and the laser polarizations to obtain the maximum m j = 1/2 signal, we achieve the detection of the signal electric field with a frequency of 100 Hz down to 214.8 µ V/cm with a sensitivity of 67.9 µ V cm −1 Hz −1/2 , and the linear dynamic range is over 37 dB. Our work extends the measurement frequency of Rydberg sensors to super low frequency with high sensitivity, which has the advantages of high sensitivity and miniaturization for receiving super low frequency.
The high polarizability of Rydberg atoms enables the multi-parameters measurement of electromagnetic fields. In this paper, we report on an atomic antenna based on Rydberg atoms in a room temperature vapor cell. The EIT is a destructive interference spectroscopy with a narrow linewidth and can be used to detect small electric fields through Autler-Townes splitting or Stark shifts. In our experiments, we employ cascade-type two-photon excitation electromagnetically induced transparency (EIT) spectroscopy to measure the shift of the Rydberg energy level. We introduce a low-frequency electric field (~kHz frequency) using a built-in electrode technique in the cesium cell. The interaction between the Rydberg atom and electric field induces the Stark shifts, where the amplitude of the electric field is converted into corresponding two-photon detuning by the EIT effect. Furthermore, the amplitude of the low-frequency electric field is converted into an intensity signal of EIT probe beam. Under weak field conditions, it is an approximate linear relationship between EIT transmission signal and input electric field amplitude, enabling measurement of waveform, amplitude, and frequency. We have demonstrated optical measurements of low-frequency electric field using Rydberg atoms. By increasing the power of probe beam and coupling beam, the EIT can increase the response bandwidth from ~MHz to hundreds of MHz. This provides a scalable approach for measuring high-frequency electric fields.
Recently, Rydberg atom has emerged as an attractive choice to realize quantum sensing of low-frequency electric field. The progress so far has mostly utilized the intensity and phase changes in probe laser and the corresponding detection mechanism still remains classical. Nevertheless, external field acting on the Rydberg state can induce the polarization variation of probe laser in the Rydberg electromagnetically induced transparency (EIT) system embedded in realistic multi-state atoms. We experimentally observe this phenomenon and realize signal extraction by appropriately utilizing the polarization degrees of freedom. Based on such a mechanism, we further design and implement a quantum weak measurement scheme, which clearly suppresses the technical noise and leads to considerable improvement of performance. Evaluation of the sensitivities across different post-selection angles demonstrates that the weak measurement results agree well with the theoretical model predictions. The advantages of our method are analyzed from multiple aspects, including characterizing the responses over different frequencies and comparing the responses of the weak measurement scheme and the traditional transmission-based method. After accounting for the screening effect of a measured ratio 17\% where the 87^\text{87}87Rb atoms experience a substantially reduced field inside the glass cell, the performance reaches 33 μV cm-1 Hz-1/2μ\text{V}~\text{cm}^\text{-1}~\text{Hz}^\text{-1/2}μV cm-1 Hz-1/2 in sensitivity and 1.0 μV/cmμ\text{V/cm}μV/cm in minimal detectable field for an integration time of 1000 s, as perceived by the atoms.
The large electric dipole moment of the Rydberg atom allows for strong coupling with weak electric fields, and is widely used in electric field measurements because of its reproducibility, precision and stability. The combination of Rydberg atoms and electromagnetically induced transparency (EIT) technology has been used for detecting and characterizing radio-frequency (RF) electric fields. In this work, by selecting probe light (852 nm), dressed light (1470 nm), and coupled light (780 nm), the Rydberg state (49P3/2) of Cs atom is prepared by using a three-photon excitation scheme through using all-infrared light excitation of Rydberg atoms. We experimentally observe the EIT spectra of the Rydberg states decorated by radio-frequency electric fields, which optically detects Rydberg atoms. The effect of the amplitude and frequency of the RF electric field on the spectrum is explored in light of changes in the EIT spectrum. The results show that in the region of weak electric field, only the ac Stark energy shift and spectral broadening occur. As the electric field is further enhanced, the sideband phenomenon occurs in both the primary peak and secondary peak of the EIT. In the region of strong field, the Rydberg energy level produces a series of Floquet states with higher-order terms, as well as state shifting and mixing, resulting in asymmetry in the spectra of the EIT sideband peaks. The effect of frequency on the shielding effect of the Cs vapor cell is further discussed based on the shift of the main peak of the EIT. The demodulation of the electric field in a range of 50 Hz–1 kHz with a fidelity of 95% is achieved by modulating the low-frequency electric field to the RF electric field. The results can provide valuable references for spectral detection and traceable measurements of low-frequency electric fields.
A Rydberg atom is a special type of atom characterized by a high principal quantum number. Electric field sensors based on Rydberg atoms have received widespread attention due to their high polarizability. However, there is currently little research on the use of Rydberg atoms for direct current (DC) or low-frequency electric fields, mainly due to the shielding effect of atomic vapor cells in low-frequency electric fields, which makes accurate measurement of the electric fields extremely challenging. In this paper, we construct a Rydberg ladder configuration by using probe laser at 852 nm and coupling laser at 510 nm in a room-temperature cesium vapor cell with integrated electrode plates, thereby enabling the realizing of a Floquet-EIT (electromagnetically induced transparency) spectrum dressed by a radio frequency (RF) field in the presence of a DC electric field. We further study the influence of DC electric field on spectral characteristic. Experimentally, it is observed that when only the RF electric field is applied, the EIT spectrum displays solely even-order sidebands. Furthermore, when both the RF field and the DC electric field are simultaneously present, the first-order sideband signal of the Floquet-EIT is observed. As the intensity of the DC electric field increases, the amplitude of the first-order sideband gradually increases. However, increasing the DC electric field to a sufficient magnitude induces sideband interference, which leads the sideband amplitudes to decrease. Furthermore, increasing the RF frequency can alleviate the interference effects induced by the DC electric field on the first-order sideband. Finally, comparing the relative standard deviation of the sideband amplitudes of the Floquet-EIT spectra with the frequency shifts of the DC-Stark spectra under weak DC electric fields, we find that the measurement accuracy of the former is significantly superior to that of the latter. This work makes use of a Cs atomic vapor cell with an integrated electrode to avoid shielding effects. By observing Floquet-EIT spectra, the response of the spectra to DC electric fields is investigated. This experiment provides novel insights into the quantum sensing measurements of DC and low-frequency electric fields.