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Optics Express

Dispersion-engineered optical fibers for mid-infrared entangled single-photon generation

Shruti Jain, Deepak Jain

Published Jul 4, 2025• 0 citations
Publisher

Abstract

Near-infrared (NIR) single-photon sources have become the backbone of quantum technology. There is further potential to demonstrate the next-generation quantum technology applications by extending the wavelengths to the mid-infrared (mid-IR) region. This interest is driven by the extraordinary characteristics of the mid-IR wavelength spectrum. In this paper, we propose germania-doped and ZBLAN fibers that exploit spontaneous four-wave mixing (SpFWM) to generate a single photon-pair in the ∼2 µm to ∼3.5 µm wavelength range. The phase-matching conditions at different wavelengths can be achieved by employing both the same-mode and mixed-mode schemes (intra and intermodal) for the idler, pump, and signal wavelengths. For the intramodal scheme, we exploited the fiber’s high NA to produce closely spaced non-degenerate modes (such as LP 11a /LP 11b and LP 21a /LP 21b ) and then used combinations of these modes (from LP 11a to LP 11b or LP 21a to LP 21b ) for all three signal, pump, and idler wavelengths to achieve the phase-matching. For the intermodal scheme, we borrowed different modes for the signal, pump (including different modes for both pump photons), and idler wavelengths. The mixed-mode schemes allow for a larger core and provide greater flexibility in tuning the idler and signal wavelengths to mitigate the effects of Raman scattering and residual pump photons (∼20–25 THz from the pump frequency), albeit with increased complexity and reduced efficiency. We developed an understanding of the mixed-mode phase-matching scheme and built a model to optimize mode selection for phase-matching. Our investigations reveal, for the first time, the untapped potential of fiber-based mid-IR entangled single photon-pair generation.

DOI
10.1364/oe.564426

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Near-infrared (NIR) single-photon sources have become the backbone of quantum technology. There is further potential to demonstrate the next-generation quantum technology applications by extending the wavelengths to the mid-infrared (mid-IR) region. This interest is driven by the extraordinary characteristics of the mid-IR wavelength spectrum. In this paper, we propose germania-doped and ZBLAN fibers that exploit spontaneous four-wave mixing (SpFWM) to generate a single photon-pair in the ∼2 µm to ∼3.5 µm wavelength range. The phase-matching conditions at different wavelengths can be achieved by employing both the same-mode and mixed-mode schemes (intra and intermodal) for the idler, pump, and signal wavelengths. For the intramodal scheme, we exploited the fiber’s high NA to produce closely spaced non-degenerate modes (such as LP 11a /LP 11b and LP 21a /LP 21b ) and then used combinations of these modes (from LP 11a to LP 11b or LP 21a to LP 21b ) for all three signal, pump, and idler wavelengths to achieve the phase-matching. For the intermodal scheme, we borrowed different modes for the signal, pump (including different modes for both pump photons), and idler wavelengths. The mixed-mode schemes allow for a larger core and provide greater flexibility in tuning the idler and signal wavelengths to mitigate the effects of Raman scattering and residual pump photons (∼20–25 THz from the pump frequency), albeit with increased complexity and reduced efficiency. We developed an understanding of the mixed-mode phase-matching scheme and built a model to optimize mode selection for phase-matching. Our investigations reveal, for the first time, the untapped potential of fiber-based mid-IR entangled single photon-pair generation.
We report novel ZBLAN fibers exploiting SpFWM, generating single-photons in the 3 to4μ m4 \mu\ \mathrm{m}4μ mrange. The phase-matching condition can be fulfilled by choosing suitable spatial mode profiles for signal, pump, and idler wavelengths.
We model the spectral quantum-mechanical purity of heralded single photons from a photon-pair source based on nondegenerate spontaneous four-wave mixing taking the impact of distributed dispersion fluctuations into account. The considered photon-pair-generation scheme utilizes pump-pulse walk-off to produce pure heralded photons and phase matching is achieved through the dispersion properties of distinct spatial modes in a few-mode silica step-index fiber. We show that fiber-core-radius fluctuations in general severely impact the single-photon purity. Furthermore, by optimizing the fiber design we show that generation of single photons with very high spectral purity is feasible even in the presence of large core-radius fluctuations. At the same time, contamination from spontaneous Raman scattering is greatly mitigated by separating the single-photon frequency by more than 32 THz from the pump frequency. (C) 2017 Optical Society of America
Optical fiber-based sources of photon pairs with hybrid entanglement across multiple degrees of freedom are essential for a wide range of quantum technologies, while remaining compatible with existing communication networks. In this paper, we use a birefringent few-mode fiber to demonstrate an intermodal-vectorial four-wave mixing process that generates two pairs of spectrally overlapping signal-idler bands. Using phase-matching conditions, we show that the pairs of bands become spectrally indistinguishable when the group refractive indices of the signal and idler modes intersect at the pump wavelength. Our theoretical predictions are confirmed through experimental observations and corroborated by numerical simulations. Furthermore, we introduce the two-photon state associated with the overlapping bands, which simultaneously exhibits entanglement in a single degree of freedom and hybrid entanglement across multiple degrees of freedom. We also explain how the type and degree of entanglement can be controlled by tailoring the spectral overlap between the signal-idler bands. This study presents a promising scheme for a fiber-based source of photon pairs with entanglement spanning the spatial, polarization, and frequency degrees of freedom.
We model the spectral quantum-mechanical purity of heralded single photons from a photon-pair source based on nondegenerate spontaneous four-wave mixing taking the impact of distributed dispersion fluctuations into account. The considered photon-pair-generation scheme utilizes pump-pulse walk-off to produce pure heralded photons and phase matching is achieved through the dispersion properties of distinct spatial modes in a few-mode silica step-index fiber. We show that fiber-core-radius fluctuations in general severely impact the single-photon purity. Furthermore, by optimizing the fiber design we show that generation of single photons with very high spectral purity is feasible even in the presence of large core-radius fluctuations. At the same time, contamination from spontaneous Raman scattering is greatly mitigated by separating the single-photon frequency by more than 32 THz from the pump frequency.
Abstract We experimentally demonstrate frequency non-degenerate photon-pair generation via spontaneous four-wave mixing from a novel CS 2 -filled microstructured optical fiber. CS 2 has high nonlinearity, narrow Raman lines, a broad transmission spectrum, and also has a large index contrast with the microstructured silica fiber. We can achieve phase matching over a large spectral range by tuning the pump wavelength, allowing the generation of idler photons in the infrared region, which is suitable for applications in quantum spectroscopy. Moreover, we demonstrate a coincidence-to-accidental ratio of larger than 90 and a pair generation efficiency of about 10−210^{-2}10−2 10 - 2 per pump pulse, which shows the viability of this fiber-based platform as a photon-pair source for quantum technology applications.