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Photonics

Optical Unidirectional Transport and Directional Blockade in Cold Atoms via Non-Hermitian Four-Wave Mixing

Xiao Liu, M. Artoni, Giuseppe Carlo La Rocca, Jin‐Hui Wu

Published May 21, 2025• 2 citations
Publisher

Abstract

We propose a scheme for realizing nonreciprocal optical scattering with non-Hermitian four-wave mixing (FWM) in a double-Λ system of cold atoms driven by coupling and dressing phase-mismatched standing-wave (SW) fields. Four scattering channels—direct transmission, cross transmission, direct reflection, and cross reflection—can be established for a probe and a signal field, some of which are nonreciprocal due to non-Hermitian spatial modulations when the two SW driving fields exhibit a π/4 phase shift. We find in particular that it is viable to attain single-color unidirectional transport, dual-color unidirectional transport, and single-color directional blockade with respect to a probe and a signal field incident upon this atomic sample from the same side, due to perfect destructive interference between direct and cross scattering channels. This work provides a new paradigm for studying non-Hermitian nonlinear optics and offers a theoretical foundation for designing all-optical atomic devices based on multi-channel nonreciprocal scattering.

DOI
10.3390/photonics12050521

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We propose a scheme for realizing nonreciprocal optical scattering with non-Hermitian four-wave mixing (FWM) in a double-Λ system of cold atoms driven by coupling and dressing phase-mismatched standing-wave (SW) fields. Four scattering channels—direct transmission, cross transmission, direct reflection, and cross reflection—can be established for a probe and a signal field, some of which are nonreciprocal due to non-Hermitian spatial modulations when the two SW driving fields exhibit a π/4 phase shift. We find in particular that it is viable to attain single-color unidirectional transport, dual-color unidirectional transport, and single-color directional blockade with respect to a probe and a signal field incident upon this atomic sample from the same side, due to perfect destructive interference between direct and cross scattering channels. This work provides a new paradigm for studying non-Hermitian nonlinear optics and offers a theoretical foundation for designing all-optical atomic devices based on multi-channel nonreciprocal scattering.
Nonlinear effects could play a crucial role in addressing optical nonreciprocal behaviors in scattering media. Such behaviors are, however, typically observed within a single transmission channel and predominantly in media with fixed optical structures, which inherently restrict the tunability of a nonreciprocal response. We suggest to combine the (intrinsic) nonlinearities of a coherent multi-level medium with a tailored driving geometry that relies on two phase-mismatched standing-wave (SW) beams. This combination is essential for creating extra scattering channels over which, in addition, fully tunable optical nonreciprocal reflection can be attained. Our general approach is here adapted to four-level double-ΛΛΛ atoms that are found to exhibit distinct forms of nonreciprocal multi-channel scattering and quite sensitive to easily tunable parameters of two SW driving beams. The numerical results we present offer valuable insights into the field of non-Hermitian optical scattering and arise indeed from the interplay of interference among scattering processes and Bragg reflection.
We present a further investigation on the optical nonreciprocity based on four-wave mixing (FWM) by leveraging coherently driven cold atoms, as a beneficial supplement to the usual cavity-waveguide solution in virtue of the on-demand tunability and broadband advantage. We consider two parameter regimes unexplored yet, where the probe and coupling fields are set with vanishing or large detunings while the dressing field is kept on resonance. Numerical results reveal that the forward (backward) probe exhibits a high transmittance (is strongly absorbed) in the resonant regime, but may be largely converted into an FWM field (propagate almost freely) in the far-detuned regime. The optimization of such a reversible unidirectional transmission featured by large isolation ratios and low insertion losses can be attained only when the coupling and dressing fields fulfill different scaling relations in amplitude, which has been well explained via analytical results. It is also viable to achieve reversible unidirectional transmission for a probe field of fixed large detunings by simply tuning the coupling field in a wide spectral range. Our findings provide additional insights into the FWM-based optical nonreciprocity and may enable more powerful unidirectional devices in quantum networks.
Control of unidirectional light propagation is of paramount importantance to optical signal processing and optical communication. Especially, the amplified optical signal can isolate noise well that may provide more applications. In this work, we propose a dynamically modulated regime to realize unidirectional reflection amplification in a short and dense uniform atomic medium, and all atoms are driven into four-level double-Λ type by two coupling fields with linearly varied intensities along x direction and two weak probe fields. Based on four-wave mixing resonance and the broken spatial symmetry, the complete nonreciprocal reflection (unidirectional reflection) can be amplified with reflectivity more than 2.0, even to 6.0. In addition, the width, height, and position of the unidirectional reflection bands can be tunable. Thus, our regime is feasible and may inspire further applications in all-optical networks that require controllable unidirectional light amplification.
A scheme for magnetic-free optical nonreciprocity in an ensemble of four-level cold atoms is proposed by exploiting the directional four-wave mixing effect. Using experimentally achievable parameters, the nonreciprocal optical responses of the system can be observed and the conversion on nonreciprocal transmission and nonreciprocal phase shift can be implemented. These nonreciprocal phenomena originate from the directional phase matching, which breaks the time-reversal symmetry and dynamic reciprocity of the cold atomic system. Moreover, by embedding the cold atoms into a Mach-Zehnder interferometer and choosing proper parameters, a two-port optical isolator with an isolation ratio of 79.70 dB and an insertion loss of 0.35 dB and a four-port optical circulator with a fidelity of 0.9985 and a photon survival probability of 0.9278 can be realized, which shows the high performance of isolation and circulation. The proposal may enable a new class of optically controllable cavity-free nonreciprocal devices in optical signal processing at the low light level.
Abstract We propose a scheme for realizing exact parity-time ( P T ) antisymmetry of complex susceptibility in a wide range of probe detuning by considering a one-dimensional lattice of cold atoms driven into the simplest three-level Λ configuration. This is attained by modulating the intensity of a standing-wave coupling field with a proper phase shift to counteract the product of a single-photon detuning and a two-photon detuning. Such a dynamically controlled P T -antisymmetric lattice supports the integration of a few nontrivial scattering behaviors including unidirectional light reflectionless, asymmetric perfect absorption, and directional signal quenching. These behaviors, depending in particular on atomic densities and lattice lengths, facilitate the on-demand realization of unidirectional or bidirectional photon transport blockade.
Optical amplification and spatial multiplexing technologies have important applications in quantum communication, quantum networks, and optical information processing. In this paper, based on the non-reciprocal amplification of a pair of co-propagating conjugate four-wave mixing (FWM) signals induced by a one-way pump field in a double-Λ-type hot atomic system, we demonstrate spatially multiplexed multiple FWM processes by introducing a counter-propagating collinear pump field. This configuration enables simultaneous amplification of bidirectional four-channel FWM signals. Furthermore, when the injected signal and pump beams are modulated to Laguerre-Gaussian beams carrying different optical orbital angular momentum (OAM), the OAM of the pump beam is transferred to each amplified field. Through the tilted lens method, we experimentally demonstrate that the OAM of the amplified signal light remains identical to that of the original injected signal light. In contrast, the OAM of the other three newly generated FWM fields is governed by the angular momentum conservation law of their respective FWM processes, which enables the precise manipulation of the OAM for the other generated amplified fields. Theoretical analysis of the dynamical transport equation for the density operator in light-matter interaction processes fully corroborates the experimental results. These findings establish a robust framework for developing OAM-compatible optical non-reciprocal devices based on complex structured light.