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arXiv:2504.03127 · Physical Review A

Non-Hermitian optical scattering in cold atoms via four-wave mixing

Xiao Liu, M. Artoni, Giuseppe Carlo La Rocca, Jin‐Hui Wu

Published Jun 20, 2025• 2 citations
arXivHTMLPDF

Abstract

Nonlinear effects could play a crucial role in addressing optical nonreciprocal behaviors in scattering media. Such behaviors are, however, typically observed within a single transmission channel and predominantly in media with fixed optical structures, which inherently restrict the tunability of a nonreciprocal response. We suggest to combine the (intrinsic) nonlinearities of a coherent multi-level medium with a tailored driving geometry that relies on two phase-mismatched standing-wave (SW) beams. This combination is essential for creating extra scattering channels over which, in addition, fully tunable optical nonreciprocal reflection can be attained. Our general approach is here adapted to four-level double-$Λ$ atoms that are found to exhibit distinct forms of nonreciprocal multi-channel scattering and quite sensitive to easily tunable parameters of two SW driving beams. The numerical results we present offer valuable insights into the field of non-Hermitian optical scattering and arise indeed from the interplay of interference among scattering processes and Bragg reflection.

DOI
10.1103/fcs4-99zl

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Nonlinear effects could play a crucial role in addressing optical nonreciprocal behaviors in scattering media. Such behaviors are, however, typically observed within a single transmission channel and predominantly in media with fixed optical structures, which inherently restrict the tunability of a nonreciprocal response. We suggest to combine the (intrinsic) nonlinearities of a coherent multi-level medium with a tailored driving geometry that relies on two phase-mismatched standing-wave (SW) beams. This combination is essential for creating extra scattering channels over which, in addition, fully tunable optical nonreciprocal reflection can be attained. Our general approach is here adapted to four-level double-ΛΛΛ atoms that are found to exhibit distinct forms of nonreciprocal multi-channel scattering and quite sensitive to easily tunable parameters of two SW driving beams. The numerical results we present offer valuable insights into the field of non-Hermitian optical scattering and arise indeed from the interplay of interference among scattering processes and Bragg reflection.
We propose a scheme for realizing nonreciprocal optical scattering with non-Hermitian four-wave mixing (FWM) in a double-Λ system of cold atoms driven by coupling and dressing phase-mismatched standing-wave (SW) fields. Four scattering channels—direct transmission, cross transmission, direct reflection, and cross reflection—can be established for a probe and a signal field, some of which are nonreciprocal due to non-Hermitian spatial modulations when the two SW driving fields exhibit a π/4 phase shift. We find in particular that it is viable to attain single-color unidirectional transport, dual-color unidirectional transport, and single-color directional blockade with respect to a probe and a signal field incident upon this atomic sample from the same side, due to perfect destructive interference between direct and cross scattering channels. This work provides a new paradigm for studying non-Hermitian nonlinear optics and offers a theoretical foundation for designing all-optical atomic devices based on multi-channel nonreciprocal scattering.
We present a further investigation on the optical nonreciprocity based on four-wave mixing (FWM) by leveraging coherently driven cold atoms, as a beneficial supplement to the usual cavity-waveguide solution in virtue of the on-demand tunability and broadband advantage. We consider two parameter regimes unexplored yet, where the probe and coupling fields are set with vanishing or large detunings while the dressing field is kept on resonance. Numerical results reveal that the forward (backward) probe exhibits a high transmittance (is strongly absorbed) in the resonant regime, but may be largely converted into an FWM field (propagate almost freely) in the far-detuned regime. The optimization of such a reversible unidirectional transmission featured by large isolation ratios and low insertion losses can be attained only when the coupling and dressing fields fulfill different scaling relations in amplitude, which has been well explained via analytical results. It is also viable to achieve reversible unidirectional transmission for a probe field of fixed large detunings by simply tuning the coupling field in a wide spectral range. Our findings provide additional insights into the FWM-based optical nonreciprocity and may enable more powerful unidirectional devices in quantum networks.
A scheme for magnetic-free optical nonreciprocity in an ensemble of four-level cold atoms is proposed by exploiting the directional four-wave mixing effect. Using experimentally achievable parameters, the nonreciprocal optical responses of the system can be observed and the conversion on nonreciprocal transmission and nonreciprocal phase shift can be implemented. These nonreciprocal phenomena originate from the directional phase matching, which breaks the time-reversal symmetry and dynamic reciprocity of the cold atomic system. Moreover, by embedding the cold atoms into a Mach-Zehnder interferometer and choosing proper parameters, a two-port optical isolator with an isolation ratio of 79.70 dB and an insertion loss of 0.35 dB and a four-port optical circulator with a fidelity of 0.9985 and a photon survival probability of 0.9278 can be realized, which shows the high performance of isolation and circulation. The proposal may enable a new class of optically controllable cavity-free nonreciprocal devices in optical signal processing at the low light level.
Abstract A waveguide-QED with giant atoms, which is capable of accessing various limits of a small one, provides a new paradigm to study photon scatterings. Thus, how to achieve nonreciprocal photon transmissions via such a giant atom setup is highly desirable. In this study, the nonreciprocal single-photon scattering characteristics of a double-driven Λ-type three-level giant atom, where one of the transition couples to a 1D waveguide at two separate points, and the other is driven by two coherent driving fields, are investigated. It is found that a frequency-tunable single-photon diode with an ideal contrast ratio can be achieved by properly manipulating the local coupling phases between the giant atom and the waveguide, the accumulation phase between the two waveguide coupling points, the Rabi frequencies and phase difference of the two driven fields. Compared to the previous single driving schemes, on the one hand, the presence of the second driving field can provide more tunable parameters to manipulate the nonreciprocal single-photon scattering behavior. On the other hand, here perfect nonreciprocal transmission for photons with arbitrary frequencies is achievable by tuning the driving phases while the two driving fields keep on turning, which provides an alternative way to control the nonreciprocal single-photon scattering. Furthermore, the results reveal that both the location and width of each optimal nonreciprocal transmission window is also sensitive to the driving detuning, and a single-photon diode with wide or narrow bandwidth can be realized based on demand. These results may be beneficial for designing nonreciprocal single-photon devices based on a double-driven giant atom setup.
Optical nonreciprocity has been a popular research topic in recent years. Semiconductor quantum wells (SQWs) play a key role in many high-performance optoelectronic devices. In this paper, we propose a theoretical scheme to achieve nonmagnetic optical nonreciprocity based on the four-wave mixing effect in SQW nanostructures. Using the experimentally available parameters, the nonreciprocal behavior of the probe field in forward direction and backward direction is achieved through this SQW, where both nonreciprocal transmission and nonreciprocal phase shift have high transmission rates. Furthermore, by embedding this SQW nanostructure into a Mach-Zender interferometer, a reconfigurable nonreciprocal device based on high transmission nonreciprocal phase shift that can be used as an isolator or a circulator, is designed and analyzed. The device can be realized as a two-port optical isolator with an isolation ratio of 92.39 dB and an insertion loss of 0.25 dB, and as a four-port optical circulator with a fidelity of 0.9993, a photon survival probability of 0.9518 and a low insertion loss with suitable parameters. Semiconductor media have the advantages of easier integration and tunable parameters, and this scheme can provide theoretical guidance for implementing nonreciprocal and nonreciprocal photonic devices based on semiconductor solid-state media.
Abstract We theoretically investigate single-photon scattering and nonreciprocal transmission in a coupled resonator waveguide which is coupled to a driven three-level giant atom via two distant sites. In our system, the local coupling phases are introduced to induce intriguing interference effects. As a result, the phase difference can serve as a sensitive controller for the photon scattering. It is found that the photon scattering properties can be effectively tailored by the size of the giant atom, the driving field and the phase difference. Intriguingly, by carefully tuning the parameters such as the atomic dissipation and the phase difference, a perfect nonreciprocal single-photon transmission can be realized. Additionally, the photon frequency can be adjusted by modulating Rabi frequency of the driving field. These results have significant potential for the development of nonreciprocal optical devices using the giant-atom configuration.