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Tin as a nuclear spin qubit in silicon

Wayne M. Witzel

Published Mar 1, 2024• 0 citations
Publisher

Abstract

for single-qubit Clifford gates Micromagnet Array of 6 Loss-DiVincenzo qubits Combining nuclear and electron qubits 5
DOI
10.2172/2540383

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Micromagnet-free operation of electron spin qubits in Si/Si1−x_{1-x}1−x​Gex_xx​ vertical double quantum dots
We study a vertical double quantum dot (DQD) in a Si/Si1−x_{1-x}1−x​Gex_xx​/Si double-well heterostructure for full electrical control of electron Loss-DiVincenzo (LD) spin qubits, using realistic device modeling and numerical simulations. Due to the emerging spin-orbit interaction in the DQD, as well as strain from the gate electrodes, small (percentage range) but finite ggg tensor variations emerge. In addition, we find a large valley splitting, on the order of Ev∼250 μE_v{\sim}250\,μEv​∼250μeV. As a result, multiple avenues for fast electrical single qubit rotations emerge. An ac electric field gives rise to electric dipole spin resonance (EDSR), while electron spin resonance (ESR) in the presence of an ac magnetic field can be electrically controlled by local gates due to varying ggg factors in DQDs. We also show that shuttling between neighboring dots, in vertical and horizontal direction, results in ultrafast single qubit gates of less than a nanosecond. Remarkably, this DQD architecture completely eliminates the need for micromagnets, significantly facilitating the scalability of LD spin qubits in semiconductor foundries.
Abstract Single electron spins bound to multi-phosphorus nuclear spin registers in silicon have demonstrated fast (0.8 ns) two-qubit SWAP\sqrt{\mathrm{SWAP}}SWAP​ SWAP gates and long spin relaxation times (~30 s). In these spin registers, when the donors are ionized, the nuclear spins remain weakly coupled to their environment, allowing exceptionally long coherence times. When the electron is present, the hyperfine interaction allows coupling of the spin and charge degrees of freedom for fast qubit operation and control. Here we demonstrate the use of the hyperfine interaction to enact electric dipole spin resonance to realize high-fidelity ( F=100−6+0F=10{0}_{-6}^{+0}F=100−6+0​ F = 10 0 − 6 + 0 %) initialization of all the nuclear spins within a four-qubit nuclear spin register. By controllably initializing the nuclear spins to ∣⇓⇓⇓⟩\left\vert \Downarrow \Downarrow \Downarrow \right\rangle∣⇓⇓⇓⟩ ⇓ ⇓ ⇓ , we achieve single-electron qubit gate fidelities of F = 99.78 ± 0.07% (Clifford gate fidelities of 99.58 ± 0.14%), above the fault-tolerant threshold for the surface code with a coherence time of $${T}_{2}^{\,* }=12\,\upmu {{{\rm{s}}}}$$ T 2 * = 12 μ s .
Spin-12\frac{1}{2}21​ 119^{119}119Sn nuclei in a silicon semiconductor could make excellent qubits. Nuclear spins in silicon are known to have long coherence times. Tin is isoelectronic with silicon, so we expect electrons can easily shuttle from one Sn atom to another to propagate quantum information via a hyperfine interaction that we predict, from all-electron linearized augmented plane wave density functional theory calculations, to be roughly ten times larger than intrinsic 29^{29}29Si. A hyperfine-induced electro-nuclear controlled-phase (e-n-CPhase) gate operation, generated (up to local rotations) by merely holding an electron at a sweet-spot of maximum hyperfine strength for a specific duration of time, is predicted to be exceptionally resilient to charge/voltage noise. Diabatic spin flips are suppressed with a modest magnetic field (>15 >15~>15 mT for <10−6<10^{-6}<10−6 flip probabilities) and nuclear spin bath noise may be avoided via isotopic enrichment or mitigated using dynamical decoupling or through monitoring and compensation. Combined with magnetic resonance control, this operation enables universal quantum computation.