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Physical Review Letters

Many-Body Gap Protection against Motional Dephasing of an Optical Clock Transition

Zhijing Niu, Vera M. Schäfer, Haoqing Zhang, Cameron Wagner, Nathan R. Taylor, Dylan J. Young, Eric Yilun Song, Anjun Chu, Ana María Rey, James K. Thompson

Published Mar 20, 2025• 3 citations
Publisher

Abstract

Quantum simulation and metrology with atoms, ions, and molecules often rely on using light fields to manipulate their internal states. The absorbed momentum from the light fields can induce spin-orbit coupling and associated motional-induced (Doppler) dephasing, which may limit the coherence time available for metrology and simulation. We experimentally demonstrate the suppression of Doppler dephasing on a strontium optical clock transition by enabling atomic interactions through a shared mode in a high-finesse optical ring cavity. The interactions create a many-body energy gap that increases with atom number, suppressing motional dephasing when it surpasses the dephasing energy scale. This collective approach offers an alternative to traditional methods, like Lamb-Dicke confinement or Mössbauer spectroscopy, for advancing optical quantum sensors and simulations.

DOI
10.1103/physrevlett.134.113403

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Quantum simulation and metrology with atoms, ions, and molecules often rely on using light fields to manipulate their internal states. The absorbed momentum from the light fields can induce spin-orbit coupling and associated motional-induced (Doppler) dephasing, which may limit the coherence time available for metrology and simulation. We experimentally demonstrate the suppression of Doppler dephasing on a strontium optical clock transition by enabling atomic interactions through a shared mode in a high-finesse optical ring cavity. The interactions create a many-body energy gap that increases with atom number, suppressing motional dephasing when it surpasses the dephasing energy scale. This collective approach offers an alternative to traditional methods, like Lamb-Dicke confinement or Mössbauer spectroscopy, for advancing optical quantum sensors and simulations.
Quantum simulation and metrology with atoms, ions, and molecules often rely on using light fields to manipulate their internal states. The absorbed momentum from the light fields can induce spin-orbit coupling and associated motional-induced (Doppler) dephasing, which may limit the coherence time available for metrology and simulation. We experimentally demonstrate the suppression of Doppler dephasing on a strontium optical clock transition by enabling atomic interactions through a shared mode in a high-finesse optical ring cavity. The interactions create a many-body energy gap that increases with atom number, suppressing motional dephasing when it surpasses the dephasing energy scale. This collective approach offers an alternative to traditional methods, like Lamb-Dicke confinement or Mössbauer spectroscopy, for advancing optical quantum sensors and simulations.
Laser-cooled and quantum degenerate atoms are being pursued as quantum simulators and form the basis of today's most precise sensors. A key challenge toward these goals is to understand and control coherent interactions between the atoms. We observe long-range exchange interactions mediated by an optical cavity, which manifest as tunable spin-spin interactions on the pseudo spin-½ system composed of the millihertz linewidth clock transition in strontium. This leads to one-axis twisting dynamics, the emergence of a many-body energy gap, and gap protection of the optical coherence against certain sources of decoherence. Our observations will aid in the future design of versatile quantum simulators and the next generation of atomic clocks that use quantum correlations for enhanced metrology.
Laser-cooled and quantum degenerate atoms are being pursued as quantum simulators and form the basis of today’s most precise sensors. A key challenge toward these goals is to understand and control coherent interactions between the atoms. We observe long-range exchange interactions mediated by an optical cavity, which manifest as tunable spin-spin interactions on the pseudo spin-½ system composed of the millihertz linewidth clock transition in strontium. This leads to one-axis twisting dynamics, the emergence of a many-body energy gap, and gap protection of the optical coherence against certain sources of decoherence. Our observations will aid in the future design of versatile quantum simulators and the next generation of atomic clocks that use quantum correlations for enhanced metrology.
Large ensembles of laser-cooled atoms interacting through infinite-range photon-mediated interactions are powerful platforms for quantum simulation and sensing. Here we realize momentum-exchange interactions in which pairs of atoms exchange their momentum states by collective emission and absorption of photons from a common cavity mode, a process equivalent to a spin-exchange or XX collective Heisenberg interaction. The momentum-exchange interaction leads to an observed all-to-all Ising-like interaction in a matter-wave interferometer. A many-body energy gap also emerges, effectively binding interferometer matter-wave packets together to suppress Doppler dephasing in analogy to Mössbauer spectroscopy. The tunable momentum-exchange interaction expands the capabilities of quantum interaction-enhanced matter-wave interferometry and may enable the realization of exotic behaviors, including simulations of superconductors and dynamical gauge fields.
Collective couplings of atomic dipoles to a shared electromagnetic environment produce a wide range of many-body phenomena. We report on the direct observation of resonant electric dipole-dipole interactions in a cubic array of atoms in the many-excitation limit. The interactions produce spatially dependent cooperative Lamb shifts when spectroscopically interrogating the millihertz-wide optical clock transition in strontium-87. We show that the ensemble-averaged shifts can be suppressed below the level of evaluated systematic uncertainties for optical atomic clocks. Additionally, we demonstrate that excitation of the atomic dipoles near a Bragg angle can enhance these effects by nearly an order of magnitude compared with nonresonant geometries. Our work demonstrates a platform for precise studies of the quantum many-body physics of spins with long-range interactions mediated by propagating photons.
Quantum simulation and sensing hold great promise for providing new insights into nature, from understanding complex interacting systems to searching for undiscovered physics. Large ensembles of laser-cooled atoms interacting via infinite-range photon mediated interactions are a powerful platform for both endeavours. Here, we realize for the first time momentum-exchange interactions in which atoms exchange their momentum states via collective emission and absorption of photons from a common cavity mode. The momentum-exchange interaction leads to an observed all-to-all Ising-like interaction in a matter-wave interferometer, which is useful for entanglement generation. A many-body energy gap also emerges, effectively binding interferometer matter-wave packets together to suppress Doppler dephasing, akin to Mössbauer spectroscopy. The tunable momentum-exchange interaction provides a new capability for quantum interaction-enhanced matter-wave interferometry and for realizing exotic behaviors including simulations of superconductors and dynamical gauge fields.