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arXiv:2304.01411

Cavity-Mediated Collective Momentum-Exchange Interactions

Chengyi Luo, Haoqing Zhang, Vanessa P. W. Koh, Wilson, John D., Anjun Chu, Murray Holland, Ana María Rey, James K. Thompson

Published Apr 3, 2023• 0 citations
arXivHTMLPDF

Abstract

Quantum simulation and sensing hold great promise for providing new insights into nature, from understanding complex interacting systems to searching for undiscovered physics. Large ensembles of laser-cooled atoms interacting via infinite-range photon mediated interactions are a powerful platform for both endeavours. Here, we realize for the first time momentum-exchange interactions in which atoms exchange their momentum states via collective emission and absorption of photons from a common cavity mode. The momentum-exchange interaction leads to an observed all-to-all Ising-like interaction in a matter-wave interferometer, which is useful for entanglement generation. A many-body energy gap also emerges, effectively binding interferometer matter-wave packets together to suppress Doppler dephasing, akin to Mössbauer spectroscopy. The tunable momentum-exchange interaction provides a new capability for quantum interaction-enhanced matter-wave interferometry and for realizing exotic behaviors including simulations of superconductors and dynamical gauge fields.

DOI
10.48550/arxiv.2304.01411

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Quantum simulation and sensing hold great promise for providing new insights into nature, from understanding complex interacting systems to searching for undiscovered physics. Large ensembles of laser-cooled atoms interacting via infinite-range photon mediated interactions are a powerful platform for both endeavours. Here, we realize for the first time momentum-exchange interactions in which atoms exchange their momentum states via collective emission and absorption of photons from a common cavity mode. The momentum-exchange interaction leads to an observed all-to-all Ising-like interaction in a matter-wave interferometer, which is useful for entanglement generation. A many-body energy gap also emerges, effectively binding interferometer matter-wave packets together to suppress Doppler dephasing, akin to Mössbauer spectroscopy. The tunable momentum-exchange interaction provides a new capability for quantum interaction-enhanced matter-wave interferometry and for realizing exotic behaviors including simulations of superconductors and dynamical gauge fields.
Large ensembles of laser-cooled atoms interacting through infinite-range photon-mediated interactions are powerful platforms for quantum simulation and sensing. Here we realize momentum-exchange interactions in which pairs of atoms exchange their momentum states by collective emission and absorption of photons from a common cavity mode, a process equivalent to a spin-exchange or XX collective Heisenberg interaction. The momentum-exchange interaction leads to an observed all-to-all Ising-like interaction in a matter-wave interferometer. A many-body energy gap also emerges, effectively binding interferometer matter-wave packets together to suppress Doppler dephasing in analogy to Mössbauer spectroscopy. The tunable momentum-exchange interaction expands the capabilities of quantum interaction-enhanced matter-wave interferometry and may enable the realization of exotic behaviors, including simulations of superconductors and dynamical gauge fields.
Paradigmatic spin Hamiltonians in condensed matter and quantum sensing typically utilize pair-wise or 2-body interactions between constituents in the material or ensemble. However, there is growing interest in exploring more general nnn-body interactions for n>2n >2n>2, with examples including more efficient quantum gates or the realization of exotic many-body fracton states. Here we realize an effective n=3n=3n=3-body Hamiltonian interaction using an ensemble of laser-cooled atoms in a high finesse optical cavity with the pseudo-spin 1/2 encoded by two atomic momentum states. To realize this interaction, we apply two dressing tones that coax the atoms to exchange photons via the cavity to realize a virtual 6-photon process, while the lower-order interactions destructively interfere. The resulting photon mediated interactions are not only n>2n>2n>2-body but also all-to-all(-to-all) and therefore of great interest for fast entanglement generation and quantum simulation of exotic phases such as the long sought but not yet observed charge-Qe superconductors, with Q=2nQ=2nQ=2n . The versatility of our experimental system can also allow for extending to 3-body interactions in multi-level systems or to higher-order interactions, such as the signature of a n=4n=4n=4-body interaction mediated by a virtual eight photon process that we also observe.
Abstract An ensemble of atoms can operate as a quantum sensor by placing atoms in a superposition of two different states. Upon measurement of the sensor, each atom is individually projected into one of the two states. Creating quantum correlations between the atoms, that is entangling them, could lead to resolutions surpassing the standard quantum limit 1–3 set by projections of individual atoms. Large amounts of entanglement 4–6 involving the internal degrees of freedom of laser-cooled atomic ensembles 4–16 have been generated in collective cavity quantum-electrodynamics systems, in which many atoms simultaneously interact with a single optical cavity mode. Here we report a matter-wave interferometer in a cavity quantum-electrodynamics system of 700 atoms that are entangled in their external degrees of freedom. In our system, each individual atom falls freely under gravity and simultaneously traverses two paths through space while entangled with the other atoms. We demonstrate both quantum non-demolition measurements and cavity-mediated spin interactions for generating squeezed momentum states with directly observed sensitivity 3 . 4−0.9+1.13\,.\,{4}_{-0.9}^{+1.1}3.4−0.9+1.1​ 3 . 4 − 0.9 + 1.1 dB and 2 . 5−0.6+0.62\,.\,{5}_{-0.6}^{+0.6}2.5−0.6+0.6​ 2 . 5 − 0.6 + 0.6 dB below the standard quantum limit, respectively. We successfully inject an entangled state into a Mach–Zehnder light-pulse interferometer with directly observed sensitivity 1 . 7−0.5+0.51\,.\,{7}_{-0.5}^{+0.5}1.7−0.5+0.5​ 1 . 7 − 0.5 + 0.5 dB below the standard quantum limit. The combination of particle delocalization and entanglement in our approach may influence developments of enhanced inertial sensors 17,18 , searches for new physics, particles and fields 19–23 , future advanced gravitational wave detectors 24,25 and accessing beyond mean-field quantum many-body physics 26–30 .
Spin Hamiltonians in condensed matter and quantum sensing typically utilize pairwise or two-body interactions between constituents in the material or ensemble. However, there is growing interest in exploring more general n -body interactions for n > 2. In this study, we realized an effective n = 3-body Hamiltonian interaction using an ensemble of laser-cooled atoms in a high-finesse optical cavity with the pseudospin 1 / 2 encoded by two atomic momentum states. We applied two dressing tones that induce the atoms to exchange photons via the cavity to realize a virtual six-photon process; lower-order interactions destructively interfered. We also observed signatures of a n = 4-body interaction mediated by a virtual eight-photon process. Our approach may be extensible to three-body interactions in multilevel systems or to even higher-order interactions.
Laser-cooled and quantum degenerate atoms are being pursued as quantum simulators and form the basis of today’s most precise sensors. A key challenge toward these goals is to understand and control coherent interactions between the atoms. We observe long-range exchange interactions mediated by an optical cavity, which manifest as tunable spin-spin interactions on the pseudo spin-½ system composed of the millihertz linewidth clock transition in strontium. This leads to one-axis twisting dynamics, the emergence of a many-body energy gap, and gap protection of the optical coherence against certain sources of decoherence. Our observations will aid in the future design of versatile quantum simulators and the next generation of atomic clocks that use quantum correlations for enhanced metrology.
Experimental platforms based on ultracold atomic gases have significantly advanced the quantum simulation of complex systems, yet the exploration of phenomena driven by long-range interactions remains a formidable challenge. Currently available methods utilizing dipolar quantum gases or multimode cavities allow us to implement long-range interactions with a 1 / r 3 character or with a spatial profile fixed by the mode structure of the vacuum electromagnetic field surrounding the atoms, respectively. Here, we propose an experimental scheme employing laser-painted cavity-mediated interactions, which enables the realization of atom-atom interactions that are fully tunable in range, shape, and sign. Our approach combines the versatility of cavity quantum electrodynamics with the precision of laser manipulation, thus providing a highly flexible platform for simulating and understanding long-range interactions in quantum many-body systems. Our analytical predictions are supported by numerical simulations describing the full dynamics of the atoms, the laser, and the cavity. These reveal the self-organization of domains in the density of the atomic cloud, confirming the finite-range nature of the induced interactions. We demonstrate that there is a wide and experimentally accessible parameter regime in which our protocol works robustly, with negligible heating of the quantum gas. The methodology not only paves the way for exploring new territories in quantum simulation but also enhances the understanding of fundamental physics, potentially leading to the discovery of novel quantum states and phases. Published by the American Physical Society 2024