Quantum memory devices with high storage efficiency and bandwidth are essential elements for future quantum networks. Solid-state quantum memories can provide broadband storage, but they primarily suffer from low storage efficiency. We use passive optimization and machine learning techniques to demonstrate nearly a 6-fold enhancement in quantum memory efficiency. In this regime, we demonstrate coherent and single-photon-level storage with a high signal-to-noise ratio. The optimization technique presented here can be applied to most solid-state quantum memories to significantly improve the storage efficiency without compromising the memory bandwidth.
Quantum memory devices with high storage efficiency and bandwidth are essential elements for future quantum networks. Solid-state quantum memories can provide broadband storage, but they primarily suffer from low storage efficiency. We use passive optimization and algorithmic optimization techniques to demonstrate nearly a sixfold enhancement in quantum memory efficiency. In this regime, we demonstrate coherent and single-photon-level storage with a high signal-to-noise ratio. The optimization technique presented here can be applied to most solid-state quantum memories to significantly improve the storage efficiency without compromising the memory bandwidth. Published by the American Physical Society 2024
We present a detailed analysis of a high-bandwidth quantum memory protocol for storing single photons in a rare-earth-ion doped crystal. The basic idea is to benefit from a coherent free-induced decay type re-emission which occurs naturally when a photon with a broadband spectrum is absorbed by a narrow atomic transition in an optically dense ensemble. This allows for a high-bandwidth memory for realistic material parameters. Long storage time and on-demand readout are obtained by means of spin states in a lambda-type configuration, through the transfer of the optical coherence to a spin coherence (so-called spin-wave storage). We give explicit formulae and show numerical results which make it possible to gain insight into the dependence of the memory efficiency on the optical depth and on the width and the shape of stored photons. We present a feasibility study in rare-earth doped crystals and show that high efficiencies and high bandwidth can be obtained with realistic parameters. High-bandwidth memories using spin-wave storage offers the possibility of very high time-bandwidth products, which is important for experiments where high repetition rates are needed.
Future optical quantum technologies, such as quantum networks, distributed quantum computing and sensing, demand efficient, broadband quantum memories. However, achieving high efficiency without introducing noise, reducing bandwidth, or limiting scalability remains a challenge. Here, we present a new approach to enhance quantum memory protocols by leveraging constructive light-matter interference, leading to an increase in memory efficiency without increasing atomic density or laser intensity. We implement this method in a Raman quantum memory in warm Cesium vapor, and achieve more than a three-fold improvement in total efficiency reaching
(34.3±8.4)%, while retaining GHz-bandwidth operation and low noise levels. Numerical simulations predict that this approach can boost efficiencies in systems limited by atomic density, such as cold atomic ensembles, from
65% to beyond
96%, while in warm atomic vapors it could reduce the laser intensity needed to reach a given efficiency by over an order-of-magnitude, exceeding
95% total efficiency. Furthermore, our method preserves the single-mode nature of the memory at high efficiencies. This new protocol is applicable to various memory architectures, paving the way toward scalable, efficient, low-noise, and high-bandwidth quantum memories.
This thesis demonstrates an efficient quantum memory that for the first time preserves more quantum information than it loses. Beyond this, it describes how even higher efficiency may be realised without sacrificing the other performance characteristics that are required for a practical device. A quantum memory is a device to store and recall the quantum state of light. Such a memory will be required for most applications of the emerging field of quantum information. The closest practical application is quantum repeaters for long distance encryption. A more distant target is quantum computing. Yet demonstrations of quantum memory to date fall far short of the performance required for repeaters, and further short of that for quantum computing. For these applications, high performance will be required in terms of 3 parameters: long storage time, high efficiency, and a large mode-capacity. Prior to this work, the storage time was the only paramter to have been demonstrated near the required level[1], and that only in a classical regime. The primary result of this thesis is to demonst rate a memory with an efficiency close the required level (70% is measured), and confirm its quantum nature with noise measurements. This represents the first quantum memory with efficiency greater than 50% and the first to operate unconditionally above the "no-cloning limit". The demonstration used the same storage medium as for the previous long-term storage experiment (Pr{u00B3}{u207A}:Y{u2082}Si0{u2085} (PrYSO)), and could in principle reach the same long storage times. The technique used is an optical "gradient echo", an optical equivalent to the long studied gradient echo technique used in Nuclear Magnetic Resonance (NMR). Aside from it's practicality for demonstrations, a gradient-echo also offers a powerful handle for manipulating stored light. However it is more complex than related memory techniques because it employs a spatially-varying medium. This becomes crucial when the optical depth (and memory efficiency) is increased; propagation effects mean the light is stored very differently than in other techniques. A simple linear-response model is used to gain insight into this high optical depth regime. As a result, some new properties are identified which may increase the efficiency in practical circumstances and improve flexibility. Of particular note, it's found that the space-dependence can be used to hide one narrow transition with another. This allows the somewhat unintuitive notion that a light pulse can fully traverse a medium without exciting a transition that it is resonant with. The spectral-hiding property has promise to overcome the problem with simultaneously acheiving all three parameters required for quantum memories. The problem is related to the preparation of available rare-earth ion doped materials. To acheive high efficiency and storage times, these require spectral holeburning whose bandwidth is limited by the splittings of spin levels. Methods exist to create high bandwidth delays lines with holeburning[2], but they cannot be efficient or long-lived. By utilising the spectral-hiding property of the gradient echo, methods to overcome this limitation are described for the first time.