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Physical Review A

Optical bistability and Rabi oscillations in a driven two-level semiconductor quantum dot: Effect of dynamical Coulomb interaction between two electrons

İbrahim Karabulut

Published Feb 13, 2025• 2 citations
Publisher

Abstract

We theoretically investigate the influence of dynamic Coulomb interaction on optical bistability and Rabi oscillations in a driven two-level semiconductor quantum dot system under laser irradiation. Using density matrix equations derived from the Coulomb-interaction model proposed by Lu et al. [Phys. Rev. A 103, 043504 (2021)], we obtain analytical solutions for population inversion under the rotating wave approximation. Our analysis shows that the Coulomb interaction induces optical bistability, governed by a cubic equation. The thresholds and the shapes of the hysteresis loops are tunable and can be controlled by various parameters, including electron density, confinement potential, detuning, and dephasing. Additionally, our numerical simulations demonstrate the potential for achieving high-efficiency population inversion and predicting bifurcation and anharmonic regimes in Rabi oscillations under monochromatic excitation.

DOI
10.1103/physreva.111.023511

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We theoretically investigate the influence of dynamic Coulomb interaction on optical bistability and Rabi oscillations in a driven two-level semiconductor quantum dot system under laser irradiation. Using density matrix equations derived from the Coulomb-interaction model proposed by Lu et al. [Phys. Rev. A 103, 043504 (2021)], we obtain analytical solutions for population inversion under the rotating wave approximation. Our analysis shows that the Coulomb interaction induces optical bistability, governed by a cubic equation. The thresholds and the shapes of the hysteresis loops are tunable and can be controlled by various parameters, including electron density, confinement potential, detuning, and dephasing. Additionally, our numerical simulations demonstrate the potential for achieving high-efficiency population inversion and predicting bifurcation and anharmonic regimes in Rabi oscillations under monochromatic excitation.
The influence of electron-hole dipole-dipole interactions (local fields) on the excitonic Rabi oscillations in an isolated quantum dot (QD) has been theoretically investigated. An analysis for the QD interaction with monochromatic field and ultrashort Gaussian pulse has been performed. On the basis of optical Bloch equations the Rabi oscillation dynamics has been investigated. As a result, the bifurcation and essentially anharmonic regimes in the Rabi oscillations in a QD exposed to the monochromatic field have been predicted. The strong dependence of the period of Rabi oscillations on the QD depolarization has been revealed. For the Gaussian pulse it has been shown that the final state of inversion as a function of the pulse peak strength demonstrates step-like transitions.
We provide a theoretical study for the dynamical behavior of two-photon Rabi oscillations in two coupled quantum dots. Each dot is a three-level quantum system (ground, one-exciton, and biexciton states). We describe the optical dynamics within the density matrix formalism framework. The two-photon Rabi oscillations are found to be significantly affected by the strength of the interdot dipolar interaction. Using a detuned laser pulse with an exciton state of the driven quantum dot in our numerical simulations, a direct coherent excitation between the biexciton states can be established, but whether Rabi oscillations can be observed depend mainly on the strength of the dipolar interaction and bandwidth of the excitation laser. When the strength of the dipolar coupling is less than the excitation laser bandwidth, the time-dependent populations of the various two biexciton states of the system exhibit coherent oscillations with several frequencies. However, as we increase the dipolar coupling strength, the population transfer between the quantum dots levels amazingly becomes forbidden, and the excitation gets trapped at the initial state. The reduction of the influence of the dipolar interaction leads to a manipulation of two-photon Rabi oscillation in an ultrashort timescale (∼ps), opening possibilities to achieve ultrafast quantum state control and quantum logic gate generation.
We investigate the optical properties of a Coulomb-coupled double-quantum dot system excited by coherent light pulses. Basic effects of Coulomb coupling regarding linear and nonlinear optical processes are discussed. By numerically solving the Heisenberg equation of motion we are able to present the temporal evolution of the system's density matrix for a wide range of coupling parameters. The two main coupling effects in dipole approximation, biexcitonic shift and F\"orster energy transfer, are investigated and their qualitative and quantitative influence on absorption spectra, Rabi oscillations, and single- and two-pulse excitation is discussed. We present simulated differential transmission spectra to allow for comparison with recent experimental studies.
This work is focused on the optical dynamics of mesoscopic semiconductor heterostructures, using as prototypes zero-dimensional quantum dots and quantum cascade lasers which consist of quasitwo-dimensional quantum wells. Within a density matrix theory, a microscopic many-particle theory is applied to study scattering effects in these structures: the coupling to external as well as local fields, electron-phonon coupling, coupling to impurities, and Coulomb coupling. For both systems, the investigated effects are compared to experimentally observed results obtained during the past years. In quantum dots, the three-dimensional spatial confinement leads to the necessity to consider a quantum kinetic description of the dynamics, resulting in non-Markovian electron-phonon effects. This can be seen in the spectral phonon sidebands due to interaction with acoustic phonons as well as a damping of nonlinear Rabi oscillations which shows a nonmonotonous intensity and pulse duration dependence. An analysis of the inclusion of the self-interaction of the quantum dot shows that no dynamical local field terms appear for the simple two-level model. Considering local fields which have their origin in many quantum dots, consequences for a two-level quantum dot such as a zero-phonon line broadening and an increasing signal in photon echo experiments are found. For the use of quantum dots in an optical spin control scheme, it is found that the dephasing due to the electron-phonon interaction can be dominant in certain regimes. Furthermore, soliton and breather solutions are studied analytically in nonlinear quantum dot ensembles. Generalizing to quasi-two-dimensional structures, the intersubband dynamics of quantum cascade laser structures is investigated. A dynamical theory is considered in which the temporal evolution of the subband populations and the current density as well as the influence of scattering effects is studied. In the nonlinear regime, the scattering dependence and the importance of coherence for Rabi oscillations is investigated. The optically induced charge dynamics is discussed with respect to coherent effects. Calculations of the electronic density and pump-probe signals within a microscopic theory of dephasing show coherent transport effects such as gain oscillations, in agreement with recent experimental results.
We study the interaction of an ac electric field with a semiconductor quantum well by using the effective nonlinear Bloch equations. Only the first two electron subbands in the well are considered. We apply the rotating wave approximation and derive analytical solutions for the Bloch equations for two different values of the detuning. At exact resonance we find a critical value of the Rabi frequency around which the dynamics of the system changes abruptly. Above this critical value one obtains electron oscillations with complete inversion in the two-subband system, while below this value we obtain electron oscillations without complete inversion and with the majority of the electron population on average in the lower subband. We also present numerical calculations for a specific quantum well structure and assess the limits of validity of the analytical results.
In this work, we develop a physically transparent Coulomb-interaction model from simplification of a general many-body theory and apply this model to study interacting electron dynamics for transient occupation and quantum coherence in both single and double quantum dots under laser irradiation. Our theory considers self-consistently the Coulomb-renormalized Rabi coupling to light by using an induced optical-depolarization field, corresponding to dynamical exchange interaction between two electrons within the same quantum dot. Meanwhile, we employ evanescent-field coupling for dynamical Coulomb interaction between two electrons in different quantum dots based on a surface-plasmon model. In particular, we explore the quantum interference between a pair of laser-induced quantum coherence in three-level quantum-dot systems, which gives rise to indirect transition of electrons for sum- and difference-frequency transient optical responses. By varying laser frequency detuning, the control of laser-dressed electronic states becomes possible and can be utilized for switching among off-state, partial, and complete on-states. This study will be useful for controlling the phase entanglement of two laser-dressed states of quantum dots, as well as for enhancing the electro-optical performance through sum- and difference-frequency transitions in many optoelectronic devices.