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Kharkov University Bulletin Chemical Series

On structural invariants of energy spectrum of S=1 Heisenberg antiferromagnets with single-ion anisotropy

Victor Tokariev, Mariia Fedorenko

Published Jun 21, 2024• 0 citations
Publisher

Abstract

We study the relationship of the energy spectrum of finite S=1 Heisenberg antiferromagnets with their structure in the presence of single-ion anisotropy. We show that in the limit of strong easy-plane anisotropy magnets with the structure of adjacency cospectral graphs have equal ground state energies with magnetization M=0. We derive additional necessary condition for equality of lowest energy levels with M=±1. For strong easy-axis anisotropy we found that bipartite S=1 magnets with structures, for which S=1/2 Ising models have equal spectra for arbitrary longitudinal magnetic field, have close energy spectra of S=1 antiferromagnets for arbitrary parameter of single-ion anisotropy. For moderate easy-axis anisotropy bipartite S=1 antiferromagnets with equal energies of spin waves in linear approximation are also approximately isoenergetic. Overall, this explains the remarkable similarity of energy spectra in M=0 subspace for S=1 antiferromagnetic Heisenberg model on bipartite cospectral regular graphs.

DOI
10.26565/2220-637x-2024-42-06

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We calculate ground state properties (energy, magnetization, susceptibility) and one-particle spectra for the S=1S=1S=1 Heisenberg antiferromagnet with easy-axis or easy-plane single-site anisotropy on the square lattice. Series expansions are used, in each of three phases of the system, to obtain systematic and accurate results. The location of the quantum phase transition in the easy-plane sector is determined. The results are compared to spin-wave theory.
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We calculate ground state properties (energy, magnetization, susceptibility) and one-particle spectra for the S=1S = 1S=1 Heisenberg antiferromagnet with easy-axis or easy-plane single site anisotropy, on the square lattice. Series expansions are used, in each of three phases of the system, to obtain systematic and accurate results. The location of the quantum phase transition in the easy-plane sector is determined. The results are compared with spin-wave theory.
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The S=1S=1S=1 bilinear-biquadratic Heisenberg exchange model on the triangular lattice with a single-ion anisotropy has previously been shown to host a number of exotic magnetic and nematic orders [Moreno-Cardoner et al., Phys. Rev. B 90, 144409 (2014)], including an extensive region of ``supersolid'' order. In this work, we amend the model by an XXZXXZXXZ anisotropy in the exchange interactions. Tuning to the limit of an exactly solvable S=1S=1S=1 generalized Ising-/Blume-Capel-type model provides a controlled limit to access phases at finite transverse exchange. Notably, we find an additional macroscopically degenerate region in the phase diagram and study its fate under perturbation theory. We further map out phase diagrams as a function of the XXZXXZXXZ anisotropy parameter, the ratio of bilinear and biquadratic interactions, and single-ion anisotropy, and we compute corrections to the total ordered moment in various phases using systematically constructed linear flavor-wave theory. We also present linear flavor-wave spectra of various states, finding that the lowest-energy band in three-sublattice generalized (i.e., with ${S}^{z}=\ifmmode\pm\else\textpm\fi{}1,0)$ Ising/Blume-Capel states, stabilized by strong exchange anisotropies, is remarkably flat, opening up the way to flat-band engineering of magnetic excitation via stabilizing nontrivial Ising-ordered ground states.