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Photonics

Determination of the Effective Lifetime of a Spinor Bose–Einstein Condensate

Xin Wang, Yong Kun Qin, Jun Jian, Wenliang Liu, Jizhou Wu, Yuqing Li, V. B. Sovkov, Jie Ma

Published Jan 30, 2025• 0 citations
Publisher

Abstract

The effective lifetime of ultra-cold atoms in specific quantum states plays a crucial role in studying interaction parameters within quantum systems. Measuring the effective lifetime of various quantum states within ultra-cold atoms is a fundamental task in quantum operations. In this paper, the effective lifetimes of the excited electronic states F=2,mF=−2, F=2,mF=−1, and F=2,mF=0 for a sodium atomic Bose–Einstein condensate (BEC) are investigated in both the optical dipole trap (ODT) and one-dimensional optical lattice. Through the analysis of experimental data, we demonstrate the significant advantage of lattice loading over the optical dipole trap in terms of atomic lifetimes. The results provide crucial insights into the temporal scales relevant for investigating the evolution of boson gases in optical lattices, facilitating the realization of quantum simulations pertaining to unique quantum phases, and providing an important experimental basis for the research of non-equilibrium dynamics between different spin states.

DOI
10.3390/photonics12020124

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The effective lifetime of ultra-cold atoms in specific quantum states plays a crucial role in studying interaction parameters within quantum systems. Measuring the effective lifetime of various quantum states within ultra-cold atoms is a fundamental task in quantum operations. In this paper, the effective lifetimes of the excited electronic states F=2,mF=−2, F=2,mF=−1, and F=2,mF=0 for a sodium atomic Bose–Einstein condensate (BEC) are investigated in both the optical dipole trap (ODT) and one-dimensional optical lattice. Through the analysis of experimental data, we demonstrate the significant advantage of lattice loading over the optical dipole trap in terms of atomic lifetimes. The results provide crucial insights into the temporal scales relevant for investigating the evolution of boson gases in optical lattices, facilitating the realization of quantum simulations pertaining to unique quantum phases, and providing an important experimental basis for the research of non-equilibrium dynamics between different spin states.
In this thesis, we study theoretically and in experimentally the properties of spin-1 Bose-Einstein condensates with antiferromagnetic interactions realized in the ultra-cold sodium gases confined in optical dipole traps. We present in detail how to realize, diagnose and control the spinor Bose-Einstein condensates in our experiment. In order to describe the condensate, a mean-field theory is first adopted. This theory predicts a phase transition when changing the magnetic field BBB. The predictions of the mean-field theory agree very well with most of our experimental results, including the values of the critical magnetic field BcB_cBc​, asymptotic values of n0n_0n0​ (relative atom number in mF=0m_F=0mF​=0 state) at large BBB and the phase diagram of n0n_0n0​. However, for small magnetization and small magnetic fields, we find abnormally large fluctuations (super-Poissonian) of n0n_0n0​. In order to describe these large fluctuations, we develop a full quantum statistical description for the spinor condensate at finite temperature. To describe uncondensed thermal atoms (also present in the same trap), we use the ``semi-ideal" Hartree-Fock approximation to deal with the interactions between the condensate atoms and the thermal ones. The experimental results lead us to introduce two kinds of temperatures, the ``spin temperature" TsT_sTs​ and the ``kinetic temperature" TkT_kTk​ with Ts≪TkT_s\ll T_kTs​≪Tk​, characterizing respectively the fluctuaitons of the condensate spin and the thermal gas. We conclude that the system is reaching a quasi-equilibrium states, where different degrees of freedom reach equilibrium by separate mechanisms but where the mutual thermalization does not occur over the lifetime of the cloud.
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Research on degenerate quantum gases of dilute atomic gases has become a well established field in modern physics and revealed many astonishing phenomena. The first experiments on Bose and Fermi gases at low temperatures aimed to prove the predictions of quantum mechanics on a macroscopic scale. Since then we make use of Bose and Fermi gases and mixtures of any combination to model other many body systems. A property of Bose Einstein condensates is superfluidity which we want to investigate further in toroidal potentials with a new apparatus which can produce an all-optical BEC. This means trapping thermal atoms in an optical dipole trap and cooling the sample by evaporation into the quantum degenerate regime. This new technique was first successfully demonstrated by M.D. Barrett et al. in 2001 and promises to be faster and simpler than the well established and common way of evaporation in magnetic traps. A new apparatus was built by the author and we report on the experimental details of the trapping of 87Rb atoms from a hot vapour and cooling them in a magneto-optical trap, and further evaporation to quantum degeneracy in a crossed optical dipole trap operating at a wavelength of l = 1064nm, with accurate control of the power in both beams via a feedback loop. The evaporation of neutral atoms of 87Rb in far red detuned optical dipole traps using linearly polarised laser light is spin independent, and mixed spinor condensates of the F=1 manifold can be formed. As an empirical technique we found by applying a magnetic gradient field during the final evaporation that we can selectively populate mF spin states or prepare mixtures. This intriguing mechanism was found earlier as well by M. S. Chang, but is yet not fully understood and subject of our future research. We can now routinely prepare an almost pure condensate containing up to 7000 atoms in the condensed phase purely in the mF = 0 spin state. This thesis contains the theoretical framework of Bose-Einstein condensation with in mean-field theory, the concepts of cooling of atoms in magneto-optical traps, the trapping and evaporation in optical dipole traps and the experimental realisation. In the future this experiment will be extended by a fast scanning dipole trap to apply arbitrary time averaged potentials of more complex geometries, such as toroidal traps to study the effects of superfluidity in a periodic potential. The production of toroidal traps and cold atoms in such a trap are outlined in this thesis.
Cold atoms trapped in optical lattices (crystals of light) provide a pristine platform for exploring quantum many body physics. Motivated by several recent experiments, this thesis examines the equilibrium and non-equilibrium dynamics of a Bose-Einstein condensate (BEC) loaded in a low dimensional optical lattice in order to realize novel quantum phases. There are two main research directions in this thesis. The first one involves the possibility that exotic order spontaneously forms when two-component bosons are trapped in a honeycomb lattice. My studies on this theme is motivated by the observation of a “twisted superfluid” state in Prof. Klaus Sengstock’s group at Hamburg (Soltan-Panahi et al., Nat. Phys. 8, 71 (2012)). A twisted superfluid involves Bose-Einstein condensation into a state whose order parameter has a spatially varying phase. In chapter 3, I study the stability of a Bose-Einstein condensate towards forming a twisted superfluid within the framework of mean field theory. Despite a exhaustive numerical search I do not find a parameter regime with a twisted superfluid. This search involved all experimentally relevant parameter regimes and therefore mean field theory predicted that the experimentalists should not observe a twisted superfluid. I conclude that the experimental observations were either a manifestation of counter superfluidity or due to interactions during time-of-flight. Subsequent experiments showed that the observations were an artifact of the measurement process. The second research direction in this thesis is an exploration of the stability of periodically driven quantum systems (also known as Floquet systems). Floquet systems can be used to realize exotic non-equilibrium quantum phases which do not have a counterpart in static systems. However, the driving can cause these systems to heat up which presents a major obstacle to creating exotic states. To explore this issue in a concrete example, I model an experiment (Parker, Ha, and Chin, Nat. Phys. 9, 769 (2013)) where a Bose-Einstein condensate loaded in an optical lattice is subjected to periodic shaking. I investigate the stability of this Floquet BEC to interactions. This research direction consists of 3 studies. In chapter 4, I first do this analysis for a purely one-dimensional system and identify a large parameter regime where the BEC is stable. In the next two chapters, I go beyond 1D and consider the role of transverse degrees of freedom. This is because the shaken lattice experiments that I model involves a 1D array of pancakes. I find that this geometry leads to much more dissipation than a purely 1D system. This extra dissipation arises because interactions can transfer energy between different directions. In chapter 5, I consider the extreme case where there is no transverse confinement. I find that in the absence of transverse confinement, a one-dimensional Floquet BEC is generically unstable. Finally, in chapter 6, I consider harmonic transverse confinement modeling the crossover between chapters 4 and 5. I find that as the transverse confinement is made stronger, the atom loss rate initially increases, but beyond a critical transverse confinement, the atom loss disappears due to unavailability of phase space for scattering. I also predict that if the transverse confinement is tuned to the vicinity of certain magic values, the heating rate exhibits a sharp drop. I perform similar analyses for a shaken square lattice and find that generically a low-dimensional Floquet BEC can be stabilized by suitably designing the transverse confinement.
Bose-Einstein condensation (BEC) is a phenomenon in which identical bosons occupy the same quantum state below a certain critical temperature. A hallmark of BEC is the coherence between particles every particle shares the same quantum wavefunction and phase. This coherence has been demonstrated for the external (motional) degrees of freedom of the atomic condensates by interfering two condensates. In this thesis, the coherence is shown to extend to the internal spin degrees of freedom of a spin-1 Bose gas evidenced by the observed coherent and reversible spin-changing collisions. The observed coherent dynamics are analogous to Josephson oscillations in weakly connected superconductors and represent a type of matter-wave four-wave mixing. Control of the coherent evolution of the system using magnetic fields is also demonstrated. The studies on spinor condensates begin by creating spinor condensates directly using all-optical approaches that were first developed in our laboratory. All-optical formation of Bose-Einstein condensates (BEC) in 1D optical lattice and single focus trap geometries are developed and presented. These techniques offer considerable flexibility and speed compared to magnetic trap approaches, and the trapping potential can be essentially spin-independent and are ideally suited for studying spinor condensates. Using condensates with well-defined initial non-equilibrium spin configuration, spin mixing of F = 1 and F = 2 spinor condensates of rubidium-87 atoms confined in an optical trap is observed. The equilibrium spin configuration in the F = 1 manifold confirms that 87Rb is ferromagnetic. The coherent spinor dynamics are demonstrated by initiating spin mixing deterministically with a non-stationary spin population configuration. Finally, the interplay between the coherent spin mixing and spatial dynamics in spin-1 condensates with ferromagnetic interactions is investigated.
Since the experimental achievement of Bose-Einstein condensation (BEC) in dilute gases, ultra-cold atom systems have proven to be an unparalleled test bed for condensed matter phenomena. With this in mind, our laboratory set out to build an apparatus for the study of the effects of disorder on condensed matter phase transitions using a BEC loaded into one, two, and three-dimensional lattices. My thesis is divided into two main sections. In the first section I describe in detail the design and construction of our apparatus. Our system is designed to form <super>87<\super>Rb condensates of approximately 10<super>5<\super> atoms. We have three possible experimental science chambers. 1. One can perform 1D lattice experiments in the chamber where the condensate is formed. There is a mirror located in vacuum, which is suitable for this purpose. 2. In a glass chamber one can do 1D, 2D, or 3D lattice experiments. Atoms are loaded into a dipole trap (optical tweezer) prior to condensation and transported approximately 20 cm to the glass cell where optical evaporation is performed to form a BEC. 3. One can transfer, using the same techniques as (2), to a chamber with a multi-channel plate detector for Rydberg atom experiments. The experimental results described in my thesis pertain to situation (1). However, I describe some details of (2) in the construction section. The first experiment presented in my thesis demonstrates the effect of disorder on the time-dependent dynamics of lattice systems. We observe that a small perturbation produces a dramatic change in the adiabaticity criteria for loading a BEC into one-dimensional optical lattice. I conclude with experiments that we expect to perform on this apparatus.