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Nanophotonics

Electro‐optic frequency shift of single photons from a quantum dot

Sanjay Kapoor, Aleksander Rodek, Michał Mikołajczyk, Jerzy Szuniewicz, Filip Sośnicki, T. Kazimierczuk, P. Kossacki, Michał Karpiński

Published Jan 20, 2025• 7 citations
Publisher

Abstract

Quantum dots (QDs) are a promising source of single photons mainly due to their on-demand operation. However, their emission wavelength depends on their size and immediate surroundings in the solid-state environment. By applying a serrodyne electro-optic phase modulation, we achieve a spectral shift up to 0.01 nm (3.5 GHz) while preserving the purity and indistinguishability of the photons. This method provides an efficient and scalable approach for tuning the emission wavelength of QDs without relying on nonlinear frequency mixing or probabilistic processes. Our results show that the electro-optic phase modulation enables stable and tunable spectral shifts, making it suitable for applications such as quantum communication, quantum key distribution, and primarily integrating remote quantum dot sources into large-scale quantum networks.

DOI
10.1515/nanoph-2024-0550

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Quantum dots (QDs) are a promising source of single photons mainly due to their on-demand operation. However, their emission wavelength depends on their size and immediate surroundings in the solid-state environment. By applying a serrodyne electro-optic phase modulation, we achieve a spectral shift up to 0.01 nm (3.5 GHz) while preserving the purity and indistinguishability of the photons. This method provides an efficient and scalable approach for tuning the emission wavelength of QDs without relying on nonlinear frequency mixing or probabilistic processes. Our results show that the electro-optic phase modulation enables stable and tunable spectral shifts, making it suitable for applications such as quantum communication, quantum key distribution, and primarily integrating remote quantum dot sources into large-scale quantum networks.
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Abstract Quantum networks typically operate in the telecom wavelengths to take advantage of low-loss transmission in optical fibres. However, bright quantum dots (QDs) emitting highly indistinguishable quantum states of light, such as InGaAs QDs, often emit photons in the near infrared thus necessitating frequency conversion (FC) to the telecom band. Furthermore, the signal quality of quantum emissions is crucial for the effective performance of these networks. In this work we report a method for simultaneously implementing spectral purification and frequency shifting of single photons from QD sources to the c-band in a periodically poled lithium niobate waveguide. We consider difference frequency generation in the counter-propagating configuration to implement FC with the output emission bandwidth in units of GHz. Our approach establishes a clear path to integrating high-performance single-emitter sources in a hybrid quantum network.
On-demand indistinguishable single-photon sources are essential for quantum networking and communication. Semiconductor quantum dots are among the most promising candidates, but their typical emission wavelength renders them unsuitable for use in fiber networks. Here, we present quantum frequency conversion of near-infrared photons from a bright quantum dot to the telecommunication C-band, allowing integration with existing fiber architectures. We use a custom-built, tunable 2400 nm seed laser to convert single photons from 942 nm to 1550 nm in a difference-frequency generation process. We achieve an end-to-end conversion efficiency of ≃35%, demonstrate count rates approaching 1 MHz at 1550 nm with g(2)(0)=0.043(1), and achieve Hong-Ou-Mandel (HOM) visibilities of 60%. We expect this scheme to be preferable to quantum dot sources directly emitting at telecom wavelengths for fiber-based quantum networking.
Fiber-optical networks are well established to accommodate global data traffic via coherent information transmission. The next generation of telecommunications will require the integration of quantum information into fiber-optic networks, e.g., for quantum key distribution. A promising and scalable route to enable quantum networking is encoding quantum information into the frequency of photons. While the cointegration of frequency-entangled photons with coherent information transmission is achieved via spectral multiplexing, more resource-efficient approaches are required. In this work, we introduce and experimentally demonstrate a transceiver concept that enables the transmission of coherent and frequency-entangled photons over a single-frequency channel. Our concept leverages the serrodyne technique via electro-optic phase modulation leading to very different dynamics for entangled and coherent photons. This enables temporal multiplexing of the respective signals. We demonstrate the preservation of entanglement over the channel in the presence of coherent light. Our approach reveals a strong potential for efficient bandwidth use in hybrid networks.