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arXiv:1801.01518 · Applied Physics Letters

A stable wavelength-tunable triggered source of single photons and cascaded photon pairs at the telecom C-band

Katharina D. Zeuner, Matthias Paul, Thomas Lettner, Carl Reuterskiöld-Hedlund, Lucas Schweickert, Stephan Steinhauer, Lily Yang, Julien Zichi, Mattias Hammar, Klaus D. Jöns, Val Zwiller

Published Apr 23, 2018• 32 citations
arXivHTMLPDF

Abstract

The implementation of fiber-based long-range quantum communication requires tunable sources of single photons at the telecom C-band. Stable and easy-to-implement wavelength-tunability of individual sources is crucial to (i) bring remote sources into resonance, (ii) define a wavelength standard, and (iii) ensure scalability to operate a quantum repeater. So far, the most promising sources for true, telecom single photons are semiconductor quantum dots, due to their ability to deterministically and reliably emit single and entangled photons. However, the required wavelength-tunability is hard to attain. Here, we show a stable wavelength-tunable quantum light source by integrating strain-released InAs quantum dots on piezoelectric substrates. We present triggered single-photon emission at 1.55 μm with a multi-photon emission probability as low as 0.097, as well as photon pair emission from the radiative biexciton–exciton cascade. We achieve a tuning range of 0.25 nm which will allow us to spectrally overlap remote quantum dots or tuning distant quantum dots into resonance with quantum memories. This opens up realistic avenues for the implementation of photonic quantum information processing applications at telecom wavelengths.

DOI
10.1063/1.5021483

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•Apr 30, 2015•0 citations
The implementation of fiber-based long-range quantum communication requires tunable sources of single photons at the telecom C-band. Stable and easy-to-implement wavelength-tunability of individual sources is crucial to (i) bring remote sources into resonance, (ii) define a wavelength standard, and (iii) ensure scalability to operate a quantum repeater. So far, the most promising sources for true, telecom single photons are semiconductor quantum dots, due to their ability to deterministically and reliably emit single and entangled photons. However, the required wavelength-tunability is hard to attain. Here, we show a stable wavelength-tunable quantum light source by integrating strain-released InAs quantum dots on piezoelectric substrates. We present triggered single-photon emission at 1.55 μm with a multi-photon emission probability as low as 0.097, as well as photon pair emission from the radiative biexciton–exciton cascade. We achieve a tuning range of 0.25 nm which will allow us to spectrally overlap remote quantum dots or tuning distant quantum dots into resonance with quantum memories. This opens up realistic avenues for the implementation of photonic quantum information processing applications at telecom wavelengths.
Most quantum communication schemes aim at the long-distance transmission of quantum information. In the quantum repeater concept, the transmission line is subdivided into shorter links interconnected by entanglement distribution via Bell-state measurements to overcome inherent channel losses. This concept requires on-demand single-photon sources with a high degree of multi-photon suppression and high indistinguishability within each repeater node. For a successful operation of the repeater, a spectral matching of remote quantum light sources is essential. We present a spectrally tunable single-photon source emitting in the telecom O-band with the potential to function as a building block of a quantum communication network based on optical fibers. A thin membrane of GaAs embedding InGaAs quantum dots (QDs) is attached onto a piezoelectric actuator via gold thermocompression bonding. Here, the thin gold layer acts simultaneously as an electrical contact, strain transmission medium, and broadband backside mirror for the QD-micromesa. The nanofabrication of the QD-micromesa is based on in situ electron-beam lithography, which makes it possible to integrate pre-selected single QDs deterministically into the center of monolithic micromesa structures. The QD pre-selection is based on distinct single-QD properties, signal intensity, and emission energy. In combination with strain-induced fine tuning, this offers a robust method to achieve spectral resonance in the emission of remote QDs. We show that the spectral tuning has no detectable influence on the multi-photon suppression with g(2)(0) as low as 2%–4% and that the emission can be stabilized to an accuracy of 4 μeV using a closed-loop optical feedback.
Abstract Semiconductor quantum dots are leading candidates for the on-demand generation of single photons and entangled photon pairs. High photon quality and indistinguishability of photons from different sources are critical for quantum information applications. The inability to grow perfectly identical quantum dots with ideal optical properties necessitates the application of post-growth tuning techniques via e.g. temperature, electric, magnetic or strain fields. In this review, we summarize the state-of-the-art and highlight the advantages of strain tunable non-classical photon sources based on epitaxial quantum dots. Using piezoelectric crystals like PMN-PT, the wavelength of single photons and entangled photon pairs emitted by InGaAs/GaAs quantum dots can be tuned reversibly. Combining with quantum light-emitting diodes simultaneously allows for electrical triggering and the tuning of wavelength or exciton fine structure. Emission from light hole exciton can be tuned, and quantum dot containing nanostructure such as nanowires have been piezo-integrated. To ensure the indistinguishability of photons from distant emitters, the wavelength drift caused by piezo creep can be compensated by frequency feedback, which is verified by two-photon interference with photons from two stabilized sources. Therefore, strain tuning proves to be a flexible and reliable tool for the development of scalable quantum dots-based non-classical photon sources.
For quantum light sources in everyday telecommunication networks, quantum science needs to be fully transformed into quantum technology. The first necessary step to move outside a well-controlled lab environment requires the use of quantum light sources operating in the technologically relevant telecom O- and C-band. This can be provided using epitaxial quantum dots as deterministic sources of quantum light. Particularly intriguing is that emitters operating at telecom wavelengths are rapidly catching up with their short wavelength counterparts in terms of performances. Here, we make a decisive step forward in the development of quantum communication networks: a state-of-the-art source of quantum light, a semiconductor quantum dot (QD), with record coincidence rate for entangled photon emission in the telecom C-band, is operated inside an optimized rack-based setup. This setup includes a tunable pulsed laser for the QD excitation (from quasi- to fully resonant excitation), all optics for the excitation filtering, and QD signal coupling into single-mode fibers. Overall, the setup allows for above 50%50\%50% transmission for both exciton and biexciton photons. These results show that quantum dots-based telecom light sources can now be transported and integrated into existing fiber infrastructures, an important step to demonstrate the feasibility of the upcoming quantum internet.
On-demand sources of entangled photons for the transmission of quantum information in the telecom C-band are required to realize fiber-based quantum networks. So far, non-deterministic sources of quantum states of light were used for long distance entanglement distribution in this lowest loss wavelength range. However, they are fundamentally limited in either efficiency or security due to their Poissonian emission statistics. Here, we show on-demand generation of entangled photon pairs in the telecom C-band by an InAs/GaAs semiconductor quantum dot. Using a robust phonon-assisted excitation scheme we measure a concurrence of 91.4 %91.4\,\%91.4% and a fidelity of 95.2 %95.2\,\%95.2% to Φ+Φ^+Φ+. On-demand generation of polarization entangled photons will enable secure quantum communication in fiber-based networks. Furthermore, applying this excitation scheme to several remote quantum dots tuned into resonance will enable first on-demand entanglement distribution over large distances for scalable real-life quantum applications.
Many quantum communication schemes require sources of single, indistinguishable and entangled photon pairs with high brightness. Semiconductor quantum dots (QDs) hold great promise to meet these requirements offering the additional key advantage of the possibility of shifting the emission wavelength to the telecom C-band (centered around 1550 nm). This wavelength range is especially sought-after for fiber-based applications due to the global absorption minimum in standard glass fibers which maximizes the attainable communication distance.
On demand single-photon and entangled-photon sources are key building-blocks for many proposed photonic quantum technologies. For practical device applications, epitaxially grown quantum dots (QDs) are of increasing importance due to their bright photon emission with sharp line width. Particularly, they are solid-state systems and can be easily embedded within a light-emitting diode (LED) to achieve electrically driven sources. Therefore, one would expect a full-fledged optoelectronic quantum network that is running on macroscopically separated, QD-based single- and entangled-photon devices. An all-electrically operated wavelength-tunable on demand single-photon source (SPS) is demonstrated first. The device consists of a LED in the form of self-assembled InGaAs QDs containing nanomembrane integrated onto a piezoelectric crystal. Triggered single photons are generated via injection of ultra-short electrical pulses into the diode, while their energy can be precisely tuned over a broad range of about 4.8 meV by varying the voltage applied to the piezoelectric crystal. High speed operation of this single-photon emitting diode up to 0.8 GHz is demonstrated. In the second part of this thesis, a fast strain-tunable entangled-light-emitting diode (ELED) is demonstrated. It has been shown that the fine structure splitting of the exciton can be effectively overcome by employing a specific anisotropic strain field. By injecting ultra-fast electrical pulses to the diode, electrically triggered entangled-photon emission with high degree of entanglement is successfully realized. A statistical investigation reveals that more than 30% of the QDs in the strain-tunable quantum LED emit polarization-entangled photon-pairs with entanglement-fidelities up to f+ = 0.83(5). Driven at the highest operation speed ever reported so far (400 MHz), the strain-tunable quantum LED emerges as unique devices for high-data rate entangled-photon applications. In the end of this thesis, on demand and wavelength-tunable LH single-photon emission from strain engineered GaAs QDs is demonstrated. Fourier-transform spectroscopy is performed, from which the coherence time of the LH single-photon emission is studied. It is envisioned that this new type of LH exciton-based SPS can be applied to realize an all-semiconductor based quantum interface in the foreseeable distributed quantum networks.