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Acta Physica Sinica

Experimental research on optical nonreciprocal control of cesium atomic systems at room temperature

Huiling Zhang, Zhongzhu Xie, Jiarui HAO, Yong Fang

Published Jan 1, 2025• 0 citations
Publisher

Abstract

Non-magnetic optical non-reciprocal devices are conducive to constructing optical information processing networks for weak signals without using any external magnetic field. In this work, the non-reciprocal transmission of electromagnetically induced transparency (EIT) in a cesium atomic gas through laser exciting a Λ-type three-level atomic system is observed experimentally. With the help of cesium atoms, which have several advantages over other alkali atoms, such as a rich and readily adjustable energy level structure, bigger ground state hyperfine energy levels, and lower saturation light intensity. An 894.596 nm laser, as probe light, excites energy level from 6S1/2 (F = 4) to 6P3/2 (F = 5), and an 894.594 nm laser, as coupling light, is divided into two beams to excite energy level from 6S1/2 (F = 3) to 6P3/2 (F = 5). The coupling light enters the cesium atomic gas cell in two directions: either collinearly incident in the same direction as the probe light, or in the opposite direction. The probing light that interacts with the coupling light inside the cesium atomic gas and then is detected by the detector avalanche photodiode, and the outcomes are shown and measured on an oscilloscope. The experimentally observed non-reciprocal transmission of EIT proves optical signal isolation in a cesium atomic system. Under the experimental conditions, a series of experiments is conducted on the regulation of the optical non-reciprocal isolation ratio at room temperature by adjusting the power of the probe light and coupling light as well as the detuning. The influence of adjustable parameters on the non-reciprocal isolation ratio is analyzed. The results show that moderate probe light power helps maintain the intensity of EIT in the absorption intensity curve, ensuring a high isolation ratio, which provides a reference for implementing the performance metrics of optical isolators. The observed isolation ratio increases with the increase of coupling power, which is consistent with the theoretical calculation. Within a certain range of coupling light power, a high-performance optical non-reciprocal system is achieved. This trend is exactly in line with that of EIT signal strength variation during co-directional coupling light excitation. A maximum isolation ratio 26 dB is obtained when many parameters are appropriate. The results indicate that in the coherently prepared cesium atom systems, optically tunable parameters can provide an effective means for achieving ideal optical isolation with a high isolation ratio. Compared with existing research on high isolation ratio cavity-free non-reciprocity based on atomic coherence, our proposed experimental scheme can be conducted by using a three-level system at room temperature. With the development of chip-level integrated gas cells, the achieving miniaturization and system integration become easier, which provides experimental support for achieving the miniaturization and integration. This work provides a certain basis for exploring high-performance non-reciprocal devices with high isolation ratios and new perspective for designing the next generation of optical equipment.

DOI
10.7498/aps.74.20241463

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Acta Physica Sinica•Jan 1, 2017•4 citations
Non-magnetic optical non-reciprocal devices are conducive to constructing optical information processing networks for weak signals without using any external magnetic field. In this work, the non-reciprocal transmission of electromagnetically induced transparency (EIT) in a cesium atomic gas through laser exciting a Λ-type three-level atomic system is observed experimentally. With the help of cesium atoms, which have several advantages over other alkali atoms, such as a rich and readily adjustable energy level structure, bigger ground state hyperfine energy levels, and lower saturation light intensity. An 894.596 nm laser, as probe light, excites energy level from 6S1/2 (F = 4) to 6P3/2 (F = 5), and an 894.594 nm laser, as coupling light, is divided into two beams to excite energy level from 6S1/2 (F = 3) to 6P3/2 (F = 5). The coupling light enters the cesium atomic gas cell in two directions: either collinearly incident in the same direction as the probe light, or in the opposite direction. The probing light that interacts with the coupling light inside the cesium atomic gas and then is detected by the detector avalanche photodiode, and the outcomes are shown and measured on an oscilloscope. The experimentally observed non-reciprocal transmission of EIT proves optical signal isolation in a cesium atomic system. Under the experimental conditions, a series of experiments is conducted on the regulation of the optical non-reciprocal isolation ratio at room temperature by adjusting the power of the probe light and coupling light as well as the detuning. The influence of adjustable parameters on the non-reciprocal isolation ratio is analyzed. The results show that moderate probe light power helps maintain the intensity of EIT in the absorption intensity curve, ensuring a high isolation ratio, which provides a reference for implementing the performance metrics of optical isolators. The observed isolation ratio increases with the increase of coupling power, which is consistent with the theoretical calculation. Within a certain range of coupling light power, a high-performance optical non-reciprocal system is achieved. This trend is exactly in line with that of EIT signal strength variation during co-directional coupling light excitation. A maximum isolation ratio 26 dB is obtained when many parameters are appropriate. The results indicate that in the coherently prepared cesium atom systems, optically tunable parameters can provide an effective means for achieving ideal optical isolation with a high isolation ratio. Compared with existing research on high isolation ratio cavity-free non-reciprocity based on atomic coherence, our proposed experimental scheme can be conducted by using a three-level system at room temperature. With the development of chip-level integrated gas cells, the achieving miniaturization and system integration become easier, which provides experimental support for achieving the miniaturization and integration. This work provides a certain basis for exploring high-performance non-reciprocal devices with high isolation ratios and new perspective for designing the next generation of optical equipment.
Electromagnetically induced transparency (EIT) is observed in a three-level multi-V-type system in cesium vapor at room temperature. The absorption and dispersion properties are measured under the condition that the coupling frequency is exactly resonance with transition 6S1/2(F=4) to 6P3/2(F'=3) while the probe frequency is scanned across the transitions from the 6S1/2(F=4) to all structures of the 6P3/2. The effects of the intensity of the pumping beam on EIT signal are investigated. The simple theory model was presented and the results of the experiment agree with the simple theoretical analysis.
For multi-level systems in hot atomic vapors the interplay between the Doppler shift due to atom velocity and the wavenubmer mismatch between driving laser fields strongly influences transmission and absorption properties of the atomic medium. In a three-level atomic ladder-system, Doppler broadening limits the visibility of electromagnetically-induced transparency (EIT) when the probe and control fields are co-propagating, while EIT is recovered under the opposite condition of counter-propagating geometry and kp<kck_{p} < k_{c}kp​<kc​, with kpk_{p}kp​ and kck_{c}kc​ being the wavenumbers of the probe and control fields, respectively. This effect has been studied and experimentally demonstrated as an efficient mechanism to realize non-reciprocal probe light transmission, opening promising avenues for example for realization of magnetic-field free optical isolators. In this tutorial we discuss the theoretical derivation of this effect and show the underlying mechanism to be an avoided crossing of the states dressed by the coupling laser as a function of atomic velocities when $k_{p}
Rydberg atoms, with large principal quantum number n, have been widely investigated in recent years due to their peculiar properties, such as big sizes, long lifetimes and strong interactions with fields and other Rydberg atoms. Rydberg atoms are very sensitive to external fields due to their large polarizabilities scaling as n7.These make Rydberg atoms an ideal candidate for the quantum information, the many-body interaction, etc.In this work, we investigate the Rydberg atoms using electromagneticlly induced transparency (EIT) in a ladder three-level system. The EIT is a quantum interference effect between two excitation path-ways driven by two laser fields. The main idea is performed in a room temperature cesium vapor cell, where the probe laser frequency is modulated. The ground state (6P1/2), excited state (6P3/2), and Rydberg state (nS1/2) constitute a Rydberg three-level system, in which the probe laser is fixed to the 6S1/2 (F = 4)6P3/2 (F = 5) transition by saturated absorption spectrum technique, whereas the coupling laser is scanned across the 6P3/249S1/2 transition. We detect the demodulated EIT signal with the lock-in amplifier (SR830). The modulated EIT signal shows a two-peak structure. The measured spacing between two peaks increases with the frequency detuning, caused by the modulation amplitude, and half the spacing between the peak-to-peak is nearly 1.67 times the modulation amplitude of the probe laser; the measured result shows that the splitting is independent of the modulation frequency. The experimental results are in agreement with the theoretical calculations. The results in our work can be used for real-time monitoring of the laser-line profiles and the fluctuation of laser frequency.
Abstract For multi-level systems in hot atomic vapors the interplay between the Doppler shift due to atomic motion and the wavenumber mismatch between driving laser fields strongly influences transmission and absorption properties of the atomic medium. In a three-level atomic ladder-system, Doppler broadening limits the visibility of electromagnetically-induced transparency (EIT) when the probe and control fields are co-propagating, while EIT is recovered under the opposite condition of counter-propagating geometry and k p < k c , with k p and k c being the wavenumbers of the probe and control fields, respectively. This effect has been studied and experimentally demonstrated as an efficient mechanism to realize non-reciprocal probe light transmission, which may enable applications as magnetic-field free optical isolators. Here, we describe the basics of this effect and discuss a simple picture for the underlying mechanism. We illustrate how the non-reciprocity scales with wavelength mismatch and show how to experimentally demonstrate the effect in a simple Rydberg-EIT system using thermal Rubidium atoms.
Ladder-type electromagnetically induced transparency (EIT) and two-photon absorption (TPA) under a low-light level of probe (0.2 μW/cm2(0.06Γ2)) and weak coupling power for a cesium atom at room temperature are investigated. Reduction of the fluorescence on the TPA in a three-level system via EIT interference is clearly observed and analyzed under the low probe Rabi frequency of about 0.30 MHz to avoid the affects from the vicinity of intermediate hyperfine states. The transparency ratio of EIT derived from the reduction of fluorescence is about 25%. Additionally, the EIT linewidth observed can be as narrow as 2.64 MHz, while the coupling Rabi frequency is around 2.66 MHz. By solving the steady-state optical Bloch equations, the numerical simulation spectra are in good agreement with EIT and TPA. According to our investigations, the Doppler velocity averaging effect over the thermal atoms reducing the linewidth of the EIT signal proves the advantage of observing the EIT in the room-temperature cell.
Rydberg atoms are highly excited atoms with large principal quantum number n, big sizes (~n2) and long lifetimes (~n3). Rydberg atoms are very sensitive to an external field due to the large polarizabilities of Rydberg atoms (~n7). Electromagnetically induced transparency (EIT) of Rydberg atom provides an ideal method to detect Rydberg atoms without destroying atoms, and can be used to measure the external direct current and radio frequency (RF) field. In this paper, we study the EIT effect of a cesium ladder-type three-level atom involving Rydberg state exposed to a weak RF field. The ground state (6S1/2), the excited state (6P3/2) and Rydberg state (48D5/2) constitute the Rydberg three-level system, in which the probe laser couples 6S1/2(F=4)6P3/2(F'=5) transition, whereas the coupling laser scans across the 6P3/248D5/2 Rydberg transition. The coupling laser (510 nm laser, propagating in the z-axis direction and linear polarization in the y-axis direction) and the probe laser (852 nm laser, linear polarization in the y-axis direction) counter-propagate through a 50-mm-long cesium vapor cell at room temperature, yielding Rydberg EIT spectra. Rydberg EIT signal is detected as a function of the detuning of the coupling laser. When a weak RF (80 MHz) electric field polarized in the x-axis direction is applied to a pair of electrode plates located on both sides of the cesium cell, the EIT spectrum of Rydberg 48D5/2 shows the Stark splitting and the even order harmonic sidebands. The experimental results are analyzed by using the Floquet theory. The simulation results accord well with the experimentally measured results. Furthermore, we also investigate the influence of the self-ionization effect of Rydberg atom on the Stark spectrum by changing the RF frequency. We put forward a proposal to avoid the effect of ionization by placing electrode plates in the cesium cell. In the weak RF-field domain, mj=5/2 Stark line crosses mj=1/2, 3/2 sidebands, these cross points provide an antenna-free method of accurately calibrating the RF electric field based on Rydberg atoms.