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Journal of the Optical Society of America B

Low-light-level ladder-type electromagnetically induced transparency and two-photon absorption

Zong-Syun He, Jing-Yuan Su, Hong-Ren Chen, Wei‐Fu Chen, Meng-Huang Sie, Jyun-Yan Ye, Chin‐Chun Tsai

Published Sep 26, 2014• 4 citations
Publisher

Abstract

Ladder-type electromagnetically induced transparency (EIT) and two-photon absorption (TPA) under a low-light level of probe (0.2 μW/cm2(0.06Γ2)) and weak coupling power for a cesium atom at room temperature are investigated. Reduction of the fluorescence on the TPA in a three-level system via EIT interference is clearly observed and analyzed under the low probe Rabi frequency of about 0.30 MHz to avoid the affects from the vicinity of intermediate hyperfine states. The transparency ratio of EIT derived from the reduction of fluorescence is about 25%. Additionally, the EIT linewidth observed can be as narrow as 2.64 MHz, while the coupling Rabi frequency is around 2.66 MHz. By solving the steady-state optical Bloch equations, the numerical simulation spectra are in good agreement with EIT and TPA. According to our investigations, the Doppler velocity averaging effect over the thermal atoms reducing the linewidth of the EIT signal proves the advantage of observing the EIT in the room-temperature cell.

DOI
10.1364/josab.31.002485

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Ladder-type electromagnetically induced transparency (EIT) and two-photon absorption (TPA) under a low-light level of probe (0.2 μW/cm2(0.06Γ2)) and weak coupling power for a cesium atom at room temperature are investigated. Reduction of the fluorescence on the TPA in a three-level system via EIT interference is clearly observed and analyzed under the low probe Rabi frequency of about 0.30 MHz to avoid the affects from the vicinity of intermediate hyperfine states. The transparency ratio of EIT derived from the reduction of fluorescence is about 25%. Additionally, the EIT linewidth observed can be as narrow as 2.64 MHz, while the coupling Rabi frequency is around 2.66 MHz. By solving the steady-state optical Bloch equations, the numerical simulation spectra are in good agreement with EIT and TPA. According to our investigations, the Doppler velocity averaging effect over the thermal atoms reducing the linewidth of the EIT signal proves the advantage of observing the EIT in the room-temperature cell.
This investigation clarifies the transition phenomenon between the electromagnetically induced transparency (EIT) and Raman absorption in a ladder-type system of Doppler-broadened cesium vapor. A competition window of this transition was found to be as narrow as 2 MHz defined by the probe Rabi frequency. For a weak probe, the spectrum of EIT associated with quantum interference suggests that the effect of the Doppler velocity on the spectrum is negligible. When the Rabi frequency of the probe becomes comparable with the effective decay rate, an electromagnetically induced absorption (EIA) dip emerges at the center of the power broadened EIT peak. While the Rabi frequency of the probe exceeds the effective decay rate, decoherence that is generated by the intensified probe field occurs and Raman absorption dominates the interaction process, yielding a pure absorption spectrum; the Doppler velocity plays an important role in the interaction. A theory that is based on density matrix simulation, with or without the Doppler effect, can qualitatively fit the experimental data. In this work, the coherence of atom-photon interactions is created or destroyed using the probe Rabi frequency as a decoherence source.
A high sensitivity spectroscopy of Rydberg atoms is presented by using electromagnetically induced transparency (EIT) in the 6S(1/2)-6P(3/2)-n D ladder-type system of cesium vapor cell at room temperature. The EIT spectra of 40 D Rydberg state are measured and the dependences of the EIT magnitude and linewidth on the coupling laser power are investigated in detail. The Rydberg EIT linewidth is measured to be about 5.6 MHz when the powers of probe and coupling lasers are 50 microW and 5.2 mW, respectively, and which is close to the natural linewidth of cesium atoms. The effect of double resonance optical pumping on EIT is also investigated. The fine structures of nD (n = 39-55) are measured and the experimental result is in agreement with quantum defect theory.
In a Doppler-broadened ladder-type cesium atomic system (6S 1/2 -6P 3/2 -8S 1/2 ), this paper characterizes electromagnetically induced transparency (EIT) in two different experimental arrangements, and investigates the influence of the double-resonance optical-pumping (DROP) effect on EIT in both arrangements. When the probe laser is weak, DROP is explicitly suppressed. When the probe laser is moderate, population of the intermediate level (6P 3/2 F ' = 5) is remarkable, therefore DROP is mixed with EIT. An interesting bimodal spectrum with the broad component due to DROP and the narrow part due to EIT has been clearly observed in cesium 6S 1/2 F = 4−6P 3/2 F ' = 5−8S 1/2 F '' = 4 transitions.
We present an investigation of electromagnetically induced transparency (EIT) without Doppler background due to a locked probe laser. The EIT is theoretically studied based on a multilevel ladder-type cesium atomic system 6S1/2{S}_{1/2}S1/2​--6P3/2{P}_{3/2}P3/2​--8S1/2{S}_{1/2}S1/2​ in a room-temperature vapor cell. The experimental results agree with the theoretical calculations. Compared with the traditional EIT spectra with a Doppler profile limiting the spectral resolution for keeping the coupling laser locked and scanning the probe laser, these EIT spectra with the probe laser locked and the coupling laser scanned have a flat background, which seem be of great benefit for applications such as the measurement of hyperfine intervals between excited states, the study of highly excited Rydberg states, laser-frequency stabilization, etc.
Based on the cesium 6S1/26{S}_{1/2}6S1/2​-6P3/26{P}_{3/2}6P3/2​-8S1/28{S}_{1/2}8S1/2​ ladder-type atomic system, double-resonance optical pumping (DROP) spectra including electromagnetically induced transparency (EIT) effects have been investigated with a room-temperature cesium vapor cell. For both cases of the probe and the coupling laser beams passing through the cesium vapor cell with the counter-propagation (CTP) and co-propagation (CP) configurations, the DROP spectra measured in the experiment display explicitly different linewidths. Thanks to the EIT effect, the linewidth of the DROP spectrum is explicitly narrower for the CTP configuration than for the CP configuration. Experimental results agree with the theoretical analysis considering Doppler averaging. Furthermore, when the coupling laser has moderate power, the DROP spectrum for the CTP configuration clearly shows two components: the narrow part due to the EIT effect and the broad part caused by optical pumping (but these two different components are never seen in the CP configuration). Also, the effect of the intensity of the coupling and probe lasers on the DROP spectra is investigated.
Experimental results of the study of processes of electromagnetically induced transparency (EIT) and two-photon absorption (TPA) are presented for the ladder Ξ-system obtained using the 5 S -5 P - nD , mS system of levels of the 85 Rb and 87 Rb atoms with n = 5, 26, and 27 and m = 39 and 48. To perform these studies, a high-temperature optical cell was designed with several regions with the following thicknesses L : 2 mm, 0.7 mm, and the region of 2–6 μm. The advantages of using thin cells over ordinary cells several centimeters thick are demonstrated. It is shown that the EIT resonance parameters for n = 5, 26, and 27 deteriorate insignificantly for thickness down to 700 μm. The TPA is recorded with the cell thickness decreasing down to L = 6 μm. It is shown that using the EIT and TPA processes makes it possible to measure the hyperfine and fine structures of highlying atomic levels. The influence of the cell walls is appreciable in recording the EIT resonances in the system 5 S -5 P -39 S with L = 0.7 mm and in the system 5 S -5 P -48 S with L = 2 mm. Possible applications of the processes studied are indicated.