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Time-bin entangled Bell state generation and tomography on thin-film lithium niobate

Giovanni Finco, Filippo Miserocchi, Andreas Maeder, Jost Kellner, Alessandra Sabatti, Robert J. Chapman, Rachel Grange

Published Dec 30, 2024• 28 citations
Publisher

Abstract

Optical quantum communication technologies are making the prospect of unconditionally secure and efficient information transfer a reality. The possibility of generating and reliably detecting quantum states of light, with the further need of increasing the private data-rate is where most research efforts are focusing. The physical concept of entanglement is a solution guaranteeing the highest degree of security in device-independent schemes, yet its implementation and preservation over long communication links is hard to achieve. Lithium niobate-on-insulator has emerged as a revolutionising platform for high-speed classical telecommunication and is equally suited for quantum information applications owing to the large second-order nonlinearities that can efficiently produce entangled photon pairs. In this work, we generate maximally entangled quantum states in the time-bin basis using lithium niobate-on-insulator photonics at the fibre optics telecommunication wavelength, and reconstruct the density matrix by quantum tomography on a single photonic integrated circuit. We use on-chip periodically-poled lithium niobate as source of entangled qubits with a brightness of 242 MHz/mW and perform quantum tomography with a fidelity of 91.9 ± 1.0 %. Our results, combined with the established large electro-optic bandwidth of lithium niobate, showcase the platform as perfect candidate to realise fibre-coupled, high-speed time-bin quantum communication modules that exploit entanglement to achieve information security.

DOI
10.1038/s41534-024-00925-7

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Quantum photonics has advanced rapidly and become a leading approach for developing a broad range of quantum technologies, including quantum communications, quantum information processing, quantum computing, and quantum sensing. Besides, the emerging photonic integrated circuits (PIC) technology has been widely used to implement versatile optical elements advantageous for different quantum applications. For example, PIC-based devices have functioned as building blocks, such as photonic qubit sources, linear optical circuits, modulators, and even single-photon detectors, for realizing highly integrated, large-scale quantum computing schemes. In such a powerful quantum photonic integrated circuits (QPIC) scheme, the creation, manipulation, and testing of quantum entanglement states from the generated qubits via a reconfigurable photonic circuitry are essential. Though the state-of-the-art PIC technology is established based on Si photonics due to its widely mature nanophotonic circuit (waveguide) fabrication technology supported by the existing immense semiconductor industry, Si-based PIC has limitations in implementing efficient and fast active elements that usually demand a quadratic nonlinearity. Lithium niobate (LN), renowned as “the silicon of photonics”, has long been a popular material widely used in integrated-optical and nonlinear-optical applications. A great variety of passive and active photonic elements have been realized in the LN platform. Recently, a novel material based on high-quality single-crystalline films of LN, known as thin-film LN on insulator (LNOI), has been developed and has soon drawn enormous attention for its greatly promising ability to realize nanoscale PIC/QPIC in this iconic optical material platform. In this presentation, we report our recent studies on several key LN PIC building blocks for developing novel quantum photonic sources and circuits, including highly integrated photonic-circuit periodically poled lithium niobate (PPLN) chips for photon-pair generation and manipulation, for high-dimensional frequency-entangled qudit production, for time-frequency grid-state generation, for continuous-variable squeezed vacuum state generation, and their potential applications to quantum computing/communication/sensing technology. Besides, a PP-LNOI electro-optic (EO) polarization mode converter (PMC) useful for demonstrating fast control of quantum polarization states and other LNOI circuit elements as QPIC building blocks will also be presented.

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Optical quantum communication technologies are making the prospect of unconditionally secure and efficient information transfer a reality. The possibility of generating and reliably detecting quantum states of light, with the further need of increasing the private data-rate is where most research efforts are focusing. The physical concept of entanglement is a solution guaranteeing the highest degree of security in device-independent schemes, yet its implementation and preservation over long communication links is hard to achieve. Lithium niobate-on-insulator has emerged as a revolutionising platform for high-speed classical telecommunication and is equally suited for quantum information applications owing to the large second-order nonlinearities that can efficiently produce entangled photon pairs. In this work, we generate maximally entangled quantum states in the time-bin basis using lithium niobate-on-insulator photonics at the fibre optics telecommunication wavelength, and reconstruct the density matrix by quantum tomography on a single photonic integrated circuit. We use on-chip periodically-poled lithium niobate as source of entangled qubits with a brightness of 242 MHz/mW and perform quantum tomography with a fidelity of 91.9 ± 1.0 %. Our results, combined with the established large electro-optic bandwidth of lithium niobate, showcase the platform as perfect candidate to realise fibre-coupled, high-speed time-bin quantum communication modules that exploit entanglement to achieve information security.
Optical quantum communication technologies are making the prospect of unconditionally secure and efficient information transfer a reality. The possibility of generating and reliably detecting quantum states of light, with the further need of increasing the private data-rate is where most research efforts are focusing. The physical concept of entanglement is a solution guaranteeing the highest degree of security in device-independent schemes, yet its implementation and preservation over long communication links is hard to achieve. Lithium niobate-on-insulator has emerged as a revolutionising platform for high-speed classical telecommunication and is equally suited for quantum information applications owing to the large second-order nonlinearities that can efficiently produce entangled photon pairs. In this work, we generate maximally entangled quantum states in the time-bin basis using lithium niobate-on-insulator photonics at the fibre optics telecommunication wavelength, and reconstruct the density matrix by quantum tomography on a single photonic integrated circuit. We use on-chip periodically-poled lithium niobate as source of entangled qubits with a brightness of 242 MHz/mW and perform quantum tomography with a fidelity of 91.9+-1.0 %. Our results, combined with the established large electro-optic bandwidth of lithium niobate, showcase the platform as perfect candidate to realise fibre-coupled, high-speed time-bin quantum communication modules that exploit entanglement to achieve information security.
Lithium niobate-on-insulator (LNOI) is a leading platform for high-speed optical communication technologies owing to its large electro-optic bandwidth, which enables light modulation above 100 GHz [1]. The wide transparency window is being leveraged to produce photonic integrated circuits operating at different wavelengths, and the strong second-order nonlinearity allows efficient frequency conversion via periodic poling of the crystal on the same waveguide network [2]. LNOI has potential to revolutionise optical communication, and nonlinear conversion processes can be used to generate highly pure quantum states acting as bits of information for the next generation of optical quantum information technologies.
Time-bin encoded quantum states of light are crucial for quantum technology applications. The integration of manipulation functionalities into chip-scale devices is essential for deploying scalable, high-performance, and cost-effective quantum networks. Here we develop a fully integrated, high-throughput quantum receiver based on the thin-film lithium niobate (TFLN) platform, capable of high-speed electro-optic manipulation of time-bin encoded quantum states. The device's novel architecture enables active switching of time-bin quantum states with an electro-optic bandwidth exceeding 30 Ghz, while supporting real-time arbitrary projective measurements with a bandwidth of over 1 GHz. We showcase its versatility and performance through several applications, including the certification of entanglement with Bell's inequality violation by 38 standard deviations and with >95% visibility. We then apply it to a fiber-based quantum communication scenario, where we experimentally demonstrate an entanglement-based quantum key distribution (QKD) protocol, achieving stable finite-size secure key rates exceeding 25 kbit/s over 12 hours of continuous operation. By leveraging a high-speed active switching scheme, the system overcomes the need for temporal post-selection, eliminating a fundamental loophole that compromises the security of time-bin entanglement-based QKD protocols and relaxes the temporal resolution requirements of single-photon detectors. Moreover, it enables active selection of the projection basis, increasing the flexibility for communication parties. This approach establishes a versatile and scalable architecture for time-bin encoded quantum communication, enabling practical protocols on industry-grade photonic technology.
Quantum networks based on wavelength-multiplexed entanglement enable parallel distribution of quantum correlations, increasing channel capacity for secure communication and distributed quantum information processing. However, broadband integrated sources capable of generating multipartite entanglement beyond photon pairs remain scarce. Here we report on-chip generation of telecom-band four-photon entanglement in a periodically poled thin-film lithium niobate on insulator (LNOI) waveguide. Type-0 spontaneous parametric down-conversion provides a phase-matching bandwidth exceeding 200 nm, enabling spectrally separable generation of multi-photon entanglement across the telecom band. The generated photons are encoded in time bins for robust fiber compatibility, and a coherent interface enabling reversible conversion between time-bin and polarization degrees of freedom allows complete quantum state tomography. We measure two-photon entanglement with a brightness of 6.7 MHz/mW/nm and a fidelity of 0.874±0.0020.874 \pm 0.0020.874±0.002. At a pump power of 0.08 mW, the four-photon state exhibits a fourfold coincidence rate of 1 Hz and a fidelity of 0.74±0.010.74 \pm 0.010.74±0.01, representing a threefold improvement over previous integrated platforms. Our results establish LNOI as a scalable platform for broadband multi-photon entanglement and provide a practical route toward dense wavelength-multiplexed quantum networks.
Abstract Entanglement is central to quantum technologies such as cryptography, sensing, and computing. Photon pairs generated via nonlinear optical processes are excellent for preparing entangled states due to their long coherence times and compatibility with fiber optic networks. Steady progress in nanofabrication has positioned lithium niobate-on-insulator (LNOI) as a leading platform for monolithic integration of photon pair sources into optical circuits, leveraging its strong second-order nonlinearity. Here, we present a reconfigurable photonic integrated circuit on LNOI, which combines two on-chip photon pair sources with programmable interferometers, enabling the generation of entangled states. The photon pair sources achieve a source brightness of 26 MHz nm −1 mW −1 while maintaining a coincidence-to-accidental ratio above 100. We successfully interfere the two sources with 99.0 ± 0.7% visibility, demonstrating the indistinguishability required for producing entanglement on-chip. We show the preparation of any of the maximally entangled Bell states with fidelity above 90% verified by quantum state tomography. These results establish LNOI as a compelling, scalable platform to explore integrated quantum photonic technologies enabled by high-brightness sources of entangled quantum states.
Quantum photonics has advanced rapidly and become a leading approach for developing a broad range of quantum technologies, including quantum communications, quantum information processing, quantum computing, and quantum sensing. Besides, the emerging photonic integrated circuits (PIC) technology has been widely used to implement versatile optical elements advantageous for different quantum applications. For example, PIC-based devices have functioned as building blocks, such as photonic qubit sources, linear optical circuits, modulators, and even single-photon detectors, for realizing highly integrated, large-scale quantum computing schemes. In such a powerful quantum photonic integrated circuits (QPIC) scheme, the creation, manipulation, and testing of quantum entanglement states from the generated qubits via a reconfigurable photonic circuitry are essential. Though the state-of-the-art PIC technology is established based on Si photonics due to its widely mature nanophotonic circuit (waveguide) fabrication technology supported by the existing immense semiconductor industry, Si-based PIC has limitations in implementing efficient and fast active elements that usually demand a quadratic nonlinearity. Lithium niobate (LN), renowned as “the silicon of photonics”, has long been a popular material widely used in integrated-optical and nonlinear-optical applications. A great variety of passive and active photonic elements have been realized in the LN platform. Recently, a novel material based on high-quality single-crystalline films of LN, known as thin-film LN on insulator (LNOI), has been developed and has soon drawn enormous attention for its greatly promising ability to realize nanoscale PIC/QPIC in this iconic optical material platform. In this presentation, we report our recent studies on several key LN PIC building blocks for developing novel quantum photonic sources and circuits, including highly integrated photonic-circuit periodically poled lithium niobate (PPLN) chips for photon-pair generation and manipulation, for high-dimensional frequency-entangled qudit production, for time-frequency grid-state generation, for continuous-variable squeezed vacuum state generation, and their potential applications to quantum computing/communication/sensing technology. Besides, a PP-LNOI electro-optic (EO) polarization mode converter (PMC) useful for demonstrating fast control of quantum polarization states and other LNOI circuit elements as QPIC building blocks will also be presented.