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IEEE Ultrasonics, Ferroelectrics, and Frequency Control Joint Symposium (UFFC-JS)

The 1529 nm Laser Stabilization Based on Dual-wavelength Modulation Transfer Spectroscopy

Jie Miao, Jingming Chen, Jiqing Lian, Qiaohui Yang, Zhendong Chen, Duo Pan, Jingbiao Chen

Published Sep 22, 2024• 0 citations
Publisher

Abstract

Modulation transfer spectroscopy (MTS) is a widely adopted sub-Doppler spectroscopic technique used for laser stabilization. In conventional MTS, modulation of the pump light is transferred to the probe light within a single atomic transition. A high population of atoms in the ground state is essential for achieving a high signal-to-noise ratio in MTS. Consequently, traditional MTS cannot be effectively applied to atomic transitions between higher energy levels, where the population of atoms is significantly lower. This work proposes a novel approach to stabilize a 1529 nm laser using dual-wavelength MTS. In this scheme, the pump and probe lights are generated by separate lasers, allowing for the modulation transfer process to occur between a 780 nm laser and a 1529 nm laser. Specifically, a prestabilized and modulated 780 nm laser is used as the pump light to interact with atoms, while the 1529 nm laser acts as the probe light to generate the servo signal necessary for locking the 1529 nm laser. This technique is versatile and can be applied to various atomic ensembles, including potassium (K), cesium (Cs), and lithium (Li).

DOI
10.1109/uffc-js60046.2024.10793864

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Modulation transfer spectroscopy (MTS) is a widely adopted sub-Doppler spectroscopic technique used for laser stabilization. In conventional MTS, modulation of the pump light is transferred to the probe light within a single atomic transition. A high population of atoms in the ground state is essential for achieving a high signal-to-noise ratio in MTS. Consequently, traditional MTS cannot be effectively applied to atomic transitions between higher energy levels, where the population of atoms is significantly lower. This work proposes a novel approach to stabilize a 1529 nm laser using dual-wavelength MTS. In this scheme, the pump and probe lights are generated by separate lasers, allowing for the modulation transfer process to occur between a 780 nm laser and a 1529 nm laser. Specifically, a prestabilized and modulated 780 nm laser is used as the pump light to interact with atoms, while the 1529 nm laser acts as the probe light to generate the servo signal necessary for locking the 1529 nm laser. This technique is versatile and can be applied to various atomic ensembles, including potassium (K), cesium (Cs), and lithium (Li).
We demonstrate a dual-wavelength optical frequency standard based on the dual-optical-transition modulation transfer spectroscopy (DOT-MTS) between different quantum transitions of the rubidium D1 (795 nm) and D2 (780 nm) lines. In a single rubidium atomic ensemble, modulation frequency sidebands from the 780 nm pump beam are simultaneously transferred to both the 780 and 795 nm probe lasers. The DOT-MTS enables the simultaneous stabilization of 780 and 795 nm lasers on a single vapor cell. Both lasers exhibit a frequency instability in the low 10 −14 range at 1 s of averaging, as estimated from the residual error signal. A theoretical model is developed based on the V-type atomic level structure to illustrate the dual-wavelength spectroscopy. This approach can be extended to develop a multi-wavelength optical frequency standard within a single atomic ensemble, broadening its applicability in fields such as precision metrology, Rydberg atoms, wavelength standards, optical networks, and beyond.
Modulation transfer spectroscopy (MTS) provides a high-resolution, Doppler-free method for laser frequency stabilization, offering excellent signal-to-noise ratio and robustness, particularly suited for compact thermal atomic clocks. Extending this approach, dual-optical-transition MTS (DOT-MTS) enables the simultaneous stabilization of two optical transitions within a single atomic ensemble, paving the way for multi-wavelength frequency references in integrated systems. Despite its potential, DOT-MTS remains relatively unexplored. In this work, we demonstrate DOT-MTS in a ladder-type configuration using87Rb atoms. Both optical-optical double resonance (OODR) and double-resonance optical pumping (DROP) signals are clearly observed. Through systematic optimization of experimental parameters, the system achieves a self-evaluated short-term frequency stability at the 1E-13 level. These results demonstrate the feasibility of DOT-MTS as a high-performance, compact frequency reference and open a promising avenue toward the development of portable optical clocks.
We make a detailed comparison of frequency modulation spectroscopy (FMS) and modulation transfer spectroscopy (MTS) and of their applications in stabilizing laser frequency. In both FMS and MTS, intensity modulations of probe beam are observed in saturated absorption spectroscopy of 87Rb atoms. However, the two modulation profiles appear different due to their distinct origins. Demodulation gives rise to frequency discrimination spectra, which can serve as error signals for frequency locking. The optimal error signal of FMS has a larger linear slope but also a slanted baseline, in contrast to that of MTS. We apply FMS and MTS to stabilize two 780 nm external cavity diode lasers to D2 lines of 87Rb atoms. We measure laser linewidth and stability using beat notes of two independently locked lasers. A laser linewidth as narrow as 12.9 kHz is achieved in FMS locking, compared to 70.8 kHz in MTS locking. A laser stability at the level of 10−12 is reached in both schemes. Nevertheless, FMS locking offers a better short-term stability, whereas MTS locking yields a smaller long-term drift. Our investigation of FMS and MTS would be valuable for making a choice of these spectroscopy techniques for laser stabilization as well as other relevant applications.
The modulation transfer spectroscopy (MTS) technique used to stabilize two different transition lines of rubidium, required for laser cooling of atoms, is investigated. The laser source is based on a 1560 nm semiconductor laser diode that is amplified by an erbium doped fiber amplifier (EDFA). The laser output is frequency doubled with a fiber coupled periodically poled Lithium Niobate (PPLN) crystal to 780 nm. To address the weak spectral features of repumping laser, a theoretical study is conducted followed by experimental verification. The 87Rb D2 line F = 1 → F' = 0 transition temperature-enhanced MTS signal is observed, which provides a choice to stabilize the repumping laser frquency on the F = 1 → F ' = 2 transition using frequency shifting with acousto-optic modulators (AOMs). Compared with the orignal MTS signal, this method is shown to be more stable and accurate for laser frequency locking. Laer frequency locking is realized by controlling the driving current of the seed laser using digital PID feedback. After locking, the laser linewidth is 35.36 kHz.
Modulation transfer spectroscopy (MTS) is widely used in an optical laboratory for laser frequency stabilization. There have been many theoretical and experimental papers on this spectroscopic method. However, most of the works focus on the cycling transitions like the D2 line of rubidium. In this paper, the MTS for noncycling transitions is investigated. We consider the D1 line of rubidium whose modulation transfer spectrum has been determined and compared to the polarization spectrum. It is found that the slope of the modulation transfer signal is sharper than the polarization spectrum. The performance of laser frequency locking based on the MTS method is better than that of the polarization spectroscopy method. The dependence of the signal amplitude on the temperature of the vapor cell was analyzed, and the high signal-to-noise-ratio spectra are achieved for D1 open transitions. The obtained results provide an effective spectroscopic method for the robust frequency locking of a laser at a wavelength of 795 nm.
We demonstrate a dual wavelength optical frequency standard based on the dual optical transition modulation transfer spectroscopy (DOTMTS) between different quantum transitions of the rubidium D1 (795 nm) and D2 (780 nm) lines. In a single rubidium atomic ensemble, modulation frequency sidebands from the 780 nm pump beam are simultaneously transferred to both the 780 nm and 795 nm probe lasers. The DOTMTS enables the simultaneous stabilization of 780 nm and 795 nm lasers on a single vapor cell. Both lasers exhibit a frequency instability in the low 10 ^(-14) range at 1 s of averaging, as estimated from the residual error signal. A theoretical model is developed based on the V type atomic level structure to illustrate the dual-wavelength spectroscopy. This approach can be extended to develop a multiwavelength optical frequency standard within a single atomic ensemble, broadening its applicability in fields such as precision metrology, wavelength standards, optical networks, and beyond.