Reducing statistical noise in frequency ratio measurement between Ca + and Sr optical clocks with a frequency-synthesized local oscillator from a Sr optical clock
Haosen Shi, BINGKUN LU, Huaqing Zhang, Ruming Hu, Yuan Qian, Yao Huang, Tao Yang, Yuan Yao, Hongfu Yu, Zhanjun Fang, Kelin Gao, Hua Guan, Yige Lin, Yanyi Jiang, Long-Sheng Ma
Optical frequency ratio measurement between optical atomic clocks is essential to precision measurement as well as the redefinition of the second. Currently, the statistical noise in frequency ratio measurement of most ion clocks is limited by the frequency instability of ion clocks. In this work, we reduce the statistical noise in the frequency ratio measurement between a transportable Ca + optical clock and a Sr optical lattice clock down to 2.2×10 −15 / τ . The local oscillator of the Ca + optical clock is frequency-synthesized from the Sr optical lattice clock, enabling a longer probe time for Ca + clock transition. Compared to previous measurement using independent local oscillators, we achieve 10-fold reduction in comparison campaign duration.
Optical frequency ratio measurement between optical atomic clocks is essential to precision measurement as well as the redefinition of the second. Currently, the statistical noise in frequency ratio measurement of most ion clocks is limited by the frequency instability of ion clocks. In this work, we reduce the statistical noise in the frequency ratio measurement between a transportable Ca + optical clock and a Sr optical lattice clock down to 2.2×10 −15 / τ . The local oscillator of the Ca + optical clock is frequency-synthesized from the Sr optical lattice clock, enabling a longer probe time for Ca + clock transition. Compared to previous measurement using independent local oscillators, we achieve 10-fold reduction in comparison campaign duration.
Laser noise usually limits the stability of optical frequency ratio measurements, limiting the speed and precision one can compare two atomic frequency standards. In this talk I will describe two methods, correlation and differential spectroscopy, which utilize correlations in laser noise to increase the achievable interrogation time and thus increase the frequency comparison stability. Correlation spectroscopy is a technique which uses a parity measurement following a synchronized Ramsey interrogation to measure the relative frequency of two similar frequency atomic clocks. With this technique we achieve a measurement instability of (4×10^(-16))⁄√(τ⁄s) for a comparison of two single 27Al+ ion clocks. Differential spectroscopy uses an atomic clock with low projection noise, here a 171Yb lattice clock, to correct the phase noise of a second, higher frequency clock’s local oscillator thereby reducing the measurement instability to the level of the first. This can be further extended using two lattice clocks in a zero dead time configuration to correct the phase noise beyond the interrogation time reachable for a single Yb lattice clock. With these techniques we achieve measurement stabilities of (2.5×10^(-16))⁄√(τ⁄s) and (2×10^(-16))⁄√(τ⁄s) for a comparison between a single 27Al+ ion clock and a 171Yb lattice clock running as single clock and in a zero dead time configuration respectively. In addition to these techniques, I will also discuss recent progress towards characterizing the systematics of the NIST 40Ca+/27Al+ optical atomic clock.
Atomic clock frequency ratios with fractional uncertainty ≤3.2×10−18
We report high-precision frequency ratio measurements between optical atomic clocks based on 27Al+, 171Yb, and 87Sr. With total fractional uncertainties at or below 3.2×10−18, these measurements meet an important milestone criterion for redefinition of the second in the International System of Units. Discrepancies in 87Sr ratios at approximately 1×10−16 and the Al+/Yb ratio at 1.6×10−17 in fractional units compared to our previous measurements underscore the importance of repeated, high-precision comparisons by different laboratories. A key innovation in this work is the use of a common ultrastable reference delivered to all clocks via a 3.6 km phase-stabilized fiber link between two institutions. Derived from a cryogenic single-crystal silicon cavity, this reference improves comparison stability by a factor of 2 to 3 over previous systems, with an optical lattice clock ratio achieving a fractional instability of 1.3×10−16 at 1 second. By enabling faster comparisons, this stability will improve sensitivity to non-white noise processes and other underlying limits of state-of-the-art optical frequency standards.
We report high-precision frequency ratio measurements between optical atomic clocks based on ^{27}Al^{+}, ^{171}Yb, and ^{87}Sr. With total fractional uncertainties at or below 3.2×10^{-18}, these measurements meet an important milestone criterion for redefinition of the second in the International System of Units. Discrepancies in ^{87}Sr ratios at approximately 1×10^{-16} and the Al^{+}/Yb ratio at 1.6×10^{-17} in fractional units compared to our previous measurements underscore the importance of repeated, high-precision comparisons by different laboratories. A key upgrade from our previous work is the use of a common ultrastable reference delivered to all clocks via a 3.6-km phase-stabilized fiber link between two institutions, enabling better accuracy and stability in frequency transfer. Derived from a cryogenic single-crystal silicon cavity, this reference improves comparison stability by a factor of 2-3 over previous systems, with an optical lattice clock ratio achieving a fractional instability of 1.3×10^{-16} at 1 s. Identifying individual clock stabilities with a three-corner-hat measurement, we demonstrate the most stable optical lattice and trapped-ion clocks used in a multispecies comparison. By enabling faster comparisons, this stability will improve sensitivity to nonwhite noise processes and other underlying limits of state-of-the-art optical frequency standards.
Direct comparison of multi-ion optical clocks based on 40Ca+ and 88Sr+
We report the first direct frequency comparison between two multi-ion optical clocks based on the S1/2 to D5/2 transition in \Ca and \Sr ions. Using linear chains of up to nine \Ca ions and six \Sr ions, we demonstrate improved stability as a function of the number of ions that are contributing to the laser frequency stabilization servo. The measured joint fractional frequency stability of the two clocks reaches 1.37(12)×10−15 at one second, placing an upper bound on the same stability of one of the clocks at 9.6(8)×10−16 in one second. We measured the frequency ratio of the two clocks to be RSr/Ca=1.082076536381896986(18), where the systematic uncertainty is primarily limited by the room temperature blackbody radiation. Our direct measurement represents an order of magnitude improvement compared to existing indirect frequency ratio measurements. Furthermore, by combining our results with recent absolute frequency measurements of the \Sr transition, referenced to a primary frequency standard, we refined the absolute frequency of the \Ca transition to νCa+=411042129776400.21(4) Hz, reducing its uncertainty by a factor of three. This study presents the first direct comparison between two multi-ion optical clocks, highlighting their significant potential for future applications in fundamental physics tests, geodesy, and precision metrology.
Many-particle optical lattice clocks have the potential for unprecedented measurement precision and stability due to their low quantum projection noise. However, this potential has so far never been realized because clock stability has been limited by frequency noise of optical local oscillators. By synchronously probing two 87Sr lattice systems using a laser with a thermal noise floor of $1\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}15}$, we remove classically correlated laser noise from the intercomparison, but this does not demonstrate independent clock performance. With an improved optical oscillator that has a $1\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}16}$ thermal noise floor, we demonstrate an order of magnitude improvement over the best reported stability of any independent clock, achieving a fractional instability of $1\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}17}$ in 1000 s of averaging time for synchronous or asynchronous comparisons. This result is within a factor of 2 of the combined quantum projection noise limit for a 160 ms probe time with $\ensuremath{\sim}{10}^{3}$ atoms in each clock. We further demonstrate that even at this high precision, the overall systematic uncertainty of our clock is not limited by atomic interactions. For the second Sr clock, which has a cavity-enhanced lattice, the atomic-density-dependent frequency shift is evaluated to be $\ensuremath{-}3.11\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}17}$ with an uncertainty of $8.2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}19}$.
Comparisons of high-accuracy optical atomic clocks \cite{Ludlow2015} are essential for precision tests of fundamental physics \cite{Safronova2018}, relativistic geodesy \cite{McGrew2018, Grotti2018, Delva2019}, and the anticipated redefinition of the SI second \cite{Riehle2018}. The scientific reach of these applications is restricted by the statistical precision of interspecies comparison measurements. The instability of individual clocks is limited by the finite coherence time of the optical local oscillator (OLO), which bounds the maximum atomic interrogation time. In this letter, we experimentally demonstrate differential spectroscopy \cite{Hume2016}, a comparison protocol that enables interrogating beyond the OLO coherence time. By phase-coherently linking a zero-dead-time (ZDT) \cite{Schioppo2017} Yb optical lattice clock with an Al+ single-ion clock via an optical frequency comb and performing synchronised Ramsey spectroscopy, we show an improvement in comparison instability relative to our previous result \cite{network2020frequency} of nearly an order of magnitude. To our knowledge, this result represents the most stable interspecies clock comparison to date.