Frequency-converted spontaneous parametric down conversion (SPDC) produces polarization entangled photons with high purity, visibility, and heralding efficiency over many wavelengths. Our two-crystal setup simplifies focusing optimization allowing for ideal brightness while achieving 99% purity and visibility.
Modeling and simulations of entanglement-based quantum-networking protocols commonly assume perfect entangled states. Some investigations have been performed, which show how imperfections cause the efficiency of the protocols to rapidly deteriorate. For polarization-entangled states created by spontaneous-parametric down-conversion (SPDC), the fundamentals of phase matching lead to a trade-off problem for the optimal properties of the state. We present a SPDC method, which circumvents the trade-off problem and allows one to obtain degeneracy, indistinguishability, and heralded-single-photon spectral purity greater than $99\mathrm{%}$ for any target SPDC wavelength in the visible and near-infrared spectrum. Therefore, our method can, in principle, generate polarization-entangled states that are optimal for polarization-entanglement-based quantum-networking protocols.
Spontaneous parametric down-conversion (SPDC) is a reliable and robust source of photons for quantum information applications. For applications that involve operations such as entanglement swapping or single-photon heralding, two-photon states are required to be factorable (uncorrelated) in their spectral and spatial degrees of freedom. We report the design and experimental characterization of an SPDC source that has been optimized for high spectral and spatial purity. The source is pumped by the 776 nm output of a mode-locked Ti:Sapphire laser and consists of a periodically-poled Potassium Titanyl Phosphate (PPKTP) crystal phase-matched for collinear type-II SPDC. The dispersive properties of PPKTP at these wavelengths is such that it is possible to minimize the spectral entanglement by matching the widths of the pump to the spectral phase-matching function. The spatial entanglement is minimized through careful control of the pump focus, yielding nearly single-mode emission. An advantage of this approach is that the emission rate into the collection modes is very high, resulting in a very bright SPDC source. We also report a scheme that employs the output of collinear sources such as these to produce polarization-entangled photon pairs. The scheme, which requires only simple polarization elements, can be scaled to N-photon GHZ states.
Photons produced in the process of spontaneous parametric down-conversion (SPDC) are typically entangled in multiple degrees of freedom. Although polarization is often the parameter of interest, the presence of spectral or spatial entanglement can complicate experiments, either by reducing the visibility of certain interference effects or by reducing collection efficiency. Several recent works have shown that the collection efficiency can be improved by focusing the pump beam. This approach has the added benefit of increasing the bandwidths of the emitted photons. We show that, in the case of type II SPDC, a focused pump can result in different spatial profiles for the signal and idler. If the crystal is configured for emission of polarization-entangled photon pairs, this effect will reduce the fidelity of that entanglement. Moreover, this spatial asymmetry leads to different spectral profiles for the two photons, even when the pump is monochromatic. The spectral and spatial asymmetries can be attributed to the difference in the angular dispersion (walk-off) of the two polarizations, along with a strong correlation between wavelength and emission direction. We also examine the link between spatial entanglement and single-mode coupling efficiency. We find that efficiency is maximized when spatial entanglement can be eliminated. For the case in which walk-off does not play a role, this can be accomplished by properly focusing the pump.
The generation of high purity single photons and entangled photon pairs is a crucial first step in many quantum optics experiments, including those that require quantum teleportation [1], entanglement swapping [2], and the generation of multi-photon entanglement [3]. The most widely used and established approach for creating photon pairs is spontaneous parametric down conversion (SPDC) - where pump photons undergo a non-linear optical process to create a down-converted photon pair [4]. Traditionally, the generation of high-purity heralded single photons required severe spectral filtering, introducing additional loss. However, through careful engineering of spectral correlations of the down-converted photon pairs one can circumvent the need for filtering and avoid the accompanying reduction in heralding efficiency.
Single-mode-fiber-coupled spontaneous parametric down-conversion (SPDC) sources are a key resource for photonic quantum technologies, but in single-crystal geometries brightness, heralding efficiency, and spectral purity remain constrained by intrinsic trade-offs. Here, we show how nonlinear interference in a cascaded two-crystal type-II SPDC source can be used to engineer the modal structure of SPDC emission, improving the brightness--heralding-efficiency trade-off by more than one order of magnitude beyond the single-crystal limit. We further demonstrate two routes to near-unity spectral purity while retaining high brightness and/or heralding efficiency, even with standard periodically poled crystals, and study the additional advantages of aperiodic poling with Gaussian phase matching. Using a spectrally resolved Laguerre--Gauss modal decomposition, we show that these improvements arise from mode-selective interference of spatial-spectral SPDC modes within the nonlinear interferometer. We experimentally validate the model through sum-frequency-generation measurements of the spatial-spectral state.