The utilization of light-pulse atom interferometry presents a valuable technique that has found application in both fundamental scientific inquiries, such as investigating constants such as measurements of fine structure constant α and gravitational constant G, and practical endeavors including acceleration sensing and rotation measurements. This thesis delves into our implementation of a dual atom interferometer design involving the clock transition 1S0 → 3P0 in strontium, concurrently conducting the interferometric sequence on atoms in both ground and excited states. To facilitate the dual atom interferometer’s operation, we have firstly established a compact experimental setup with a transversely loaded bi-dimensional magneto-optical-trap (2D-MOT) to create a high flux source of cold strontium atoms. Introducing a novel cross-polarized bi-color atomic beam slower, we simultaneously addresses two excited Zeeman substates of the transition 1S0 → 1P1 in strontium-88, significantly enhancing the number of atoms prepared in the 461 nm MOT by around 10-fold. Following the 461 nm MOT, the atomic ensemble undergoes cooling in a 689 nm MOT, achieving atomic temperatures below 1 µK. We also install a network of eight magnetic field probes arranged around the cold atomic sample, enabling precise three-axis active control of magnetic fields down to the milligauss level. With the atoms confined in a 2D lattice at the magic-wavelength of 813.427 nm after the initial preparation phase, we conduct the magnetically-induced clock transition to create a statistical mixture state of ground and excited states. After a velocity selection stage, implementing a Mach-Zehnder interferometer with Bragg pulses operating at the magic-wavelength along the vertical axis, we conduct tests of the weak equivalence principle (WEP). The Eötvös ratio we found in our system stood at (1.8 ± 3.1) × 10−4, mainly limited by the finite temperature of the atomic cloud constraining the interrogation time. Furthermore, the dual atom interferometer scheme enables the measurement of state-dependent force and eventually polarizability difference via the phase shift between the atoms in different states, and we experimentally demonstrate this by introducing an additional light field gradient.
The utilization of light-pulse atom interferometry presents a valuable technique that has found application in both fundamental scientific inquiries, such as investigating constants such as measurements of fine structure constant α and gravitational constant G, and practical endeavors including acceleration sensing and rotation measurements. This thesis delves into our implementation of a dual atom interferometer design involving the clock transition 1S0 → 3P0 in strontium, concurrently conducting the interferometric sequence on atoms in both ground and excited states. To facilitate the dual atom interferometer’s operation, we have firstly established a compact experimental setup with a transversely loaded bi-dimensional magneto-optical-trap (2D-MOT) to create a high flux source of cold strontium atoms. Introducing a novel cross-polarized bi-color atomic beam slower, we simultaneously addresses two excited Zeeman substates of the transition 1S0 → 1P1 in strontium-88, significantly enhancing the number of atoms prepared in the 461 nm MOT by around 10-fold. Following the 461 nm MOT, the atomic ensemble undergoes cooling in a 689 nm MOT, achieving atomic temperatures below 1 µK. We also install a network of eight magnetic field probes arranged around the cold atomic sample, enabling precise three-axis active control of magnetic fields down to the milligauss level. With the atoms confined in a 2D lattice at the magic-wavelength of 813.427 nm after the initial preparation phase, we conduct the magnetically-induced clock transition to create a statistical mixture state of ground and excited states. After a velocity selection stage, implementing a Mach-Zehnder interferometer with Bragg pulses operating at the magic-wavelength along the vertical axis, we conduct tests of the weak equivalence principle (WEP). The Eötvös ratio we found in our system stood at (1.8 ± 3.1) × 10−4, mainly limited by the finite temperature of the atomic cloud constraining the interrogation time. Furthermore, the dual atom interferometer scheme enables the measurement of state-dependent force and eventually polarizability difference via the phase shift between the atoms in different states, and we experimentally demonstrate this by introducing an additional light field gradient.
Optical clocks and atom interferometers provide complementary ways to measure time, motion and gravity. Combining these capabilities requires matter-wave beam splitters that manipulate different clock states in the same way, so that optical internal energy becomes a controlled degree of freedom rather than a source of systematic phase shifts. Here we realized a dual matter-wave interferometer operating simultaneously on the two states of the 88Sr optical clock transition, 1S0 and 3P0. The interferometer is driven by Bragg pulses at the 813 nm magic wavelength, for which the two clock states experience the same optical coupling strength. This realizes a common matter-wave beam splitter for atoms whose internal energies differ by an optical excitation. With a sensitivity of 30 mrad, our measurement is consistent with a zero differential phase shift between the two clock-state Mach-Zehnder interferometers, translating to an absence of state-dependent acceleration in free fall at the level of 10−5. We further used the same interferometer to measure state-dependent optical dipole forces and determine a tune-out wavelength of the metastable 3P0 state to be 478.95(8) nm. These results establish magic-wavelength clock-state interferometry as a platform for differential force sensing, excited-state polarizability metrology and future quantum-clock tests of gravity.
Atom interferometry is a maturing quantum technology which provides one of the most precise approaches to explore fundamental physics, e.g. to search for dark matter, and one day to observe gravitational waves in the frequency range from 10 mHz - 10 Hz. Standard atom interferometers use Bragg or Raman two-photon transitions for the coherent manipulation of matter waves. In a Michelson configuration for atom-aided gravitational waves detection, two orthogonal arms are built to reject laser noise, in the same way as optical interferometers. Atom interferometers utilizing an optical clock transition for coherent manipulation are less affected by the technical noise of the laser, and as a result that single baseline detectors become feasible.At LP2N, we are building a vertical gravity-gradiometer based on atom interferometry using strontium atoms probed on such a clock transition. The final experimental setup will implement a 6-meter tall atomic fountain to realize gradiometry with two or more separated atomic clouds.In my dissertation, I present the realization of the experimental setup in all its sub-systems, and the first experiments with atoms at millikelvin temperature obtained with the first cooling stage with blue light. The laser system for the second red cooling phase and for the coherent manipulation is ready; meanwhile, we realized a dual-frequency Zeeman slower that improves the atomic flux by a factor of six. We also present a study of an original scheme to achieve pulsed and fast light-atom interaction in a narrow-linewidth cavity by exploiting the Stark shift as a high bandwidth switch; this technique could open to the use of narrow-linewidth cavities – and notably their high power buildup - in several contexts, like atom interferometry and quantum information.
Atom interferometry experiments measuring gravitational redshift require access to long-lived internal states, such as the 1S0-3P0 optical transition in group II atoms. An E1-M1 two-photon excitation directly access the clock state from the ground state by coupling to a far detuned intermediate state through a pair of electric and magnetic dipole allowed transitions [1]. This avoids state mixing, enhancing the excited state’s lifetime. Moreover, using counter-propagating photons with degenerate frequencies eliminates first-order Doppler effects. We report the progress of our experimental setup to drive the clock transition. We prepare an ultra-cold atomic ensemble of 174Yb through a dual-stage magneto-optical trap sequence, followed by evaporative cooling in a crossed optical dipole trap [2]. To excite the transition, we utilize a high power (10 W), narrow-linewidth l1156 nm laser system referenced to a high-finesse cavity and a frequency comb. We discuss further applications of the two-photon Doppler-free excitation as a beam splliting method for quantum clock interferometry experiments. [1]PRA 90, 012523 (2014). [2]J.Phys.B 54, 035302 (2021)
Atom interferometry has hugely benefitted from advances made in cold atom physics over the past twenty years, and ultra-precise quantum sensors are now available for a wide range of applications [1]. In particular, cold atom interferometers have shown excellent performances in the field of acceleration and rotation measurements [2,3], and are foreseen as promising candidates for navigation, geophysics, geo-prospecting and tests of fundamental physics such as the Universality of Free Fall (UFF). In order to carry out a test of the UFF with atoms as test masses, one needs to compare precisely the accelerations of two atoms with different masses as they fall in the Earth’s gravitational field. The sensitivity of atom interferometers scales like the square of the time during which the atoms are in free fall, and on ground this interrogation time is limited by the size of the experimental setup to a fraction of a second. Sending an atom interferometer in space would allow for several seconds of excellent free-fall conditions, and tests of the UFF could be carried out with precisions as low as 10-15 [4]. However, cold atoms experiments rely on complex laser systems, which are needed to cool down and manipulate the atoms, and these systems are usually very sensitive to temperature fluctuations and vibrations. In addition, when operating an inertial sensor, vibrations are a major issue, as they deteriorate the performances of the instrument. This is why cold atom interferometers are usually used in ground based facilities, which provide stable enough environments. In order to carry out airborne or space-borne measurements, one has to design an instrument which is both compact and stable, and such that vibrations induced by the platform will not deteriorate the sensitivity of the sensor. We report on the operation of an atom interferometer on board a plane carrying out parabolic flights (Airbus A300 Zero-G, operated by Novespace). We have constructed a compact and stable laser setup, which is well suited for onboard applications. Our goal is to implement a dual-species Rb-K atom interferometer in order to carry out a test of the UFF in the plane. In this perspective, we are designing a dual-wavelength laser source, which will enable us to cool down and coherently manipulate the quantum states of both atoms. We have successfully tested a preliminary version of the source and obtained a double species magneto-optical trap (MOT).
The use of strontium in an atom interferometer presents the opportunity to perform detailed measurements of gravitational fields, rotation rates, and clock transitions as well as other natural phenomena. Strontium can be particularly effective in atom interferometry experiments for two reasons. The first is that the intrinsic magnetic properties of strontium result in less sensitivity of the transition frequencies to magnetic noise, allowing for better measurements. Second, strontium atoms can be cooled to a lower temperature just through ordinary Doppler cooling than other atoms typically used in interferometry (e.g., rubidium). A lower temperature means less initial kinetic energy and hence lower spatial dispersion over the course of an experiment. A magneto-optical trap consisting of two primary cooling lasers and two repump lasers cools and confines strontium atoms for use in the interferometer. This thesis focuses on the repump lasers and includes the design and performance of the optical system that frequency stabilizes each laser. The system demonstrated the ability to simultaneously frequency lock the two repump lasers to the degree necessary to form a strontium magneto-optical trap.
We demonstrate a closed-loop light-pulse atom-interferometer inertial sensor that can realize continuous decoupled measurements of acceleration and rotation rate. The sensor operates with double-loop atom interferometers, which share the same Raman light pulses in a spatially separated Mach-Zehnder configuration and use continuous cold atomic beams propagating in opposite directions from two 2D+ magneto-optical trappings. Acceleration and the rotation rate are decoupled and simultaneously measured by the sum and difference of dual-atom-interferometer signals, respectively. The sensitivities of inertial measurements are also increased to be approximately 1.86 times higher than that of a single atom interferometer. The acceleration phase shift is compensated in real time by phase locking these interferometers via the Raman laser phases from the sum-interferometer signal, and the gyroscope performance is improved. We achieve long-term stabilities of $6.1\phantom{\rule{0.2em}{0ex}}\text{\ensuremath{\mu}}\text{g}$ and 840 nrad/s for the acceleration and the rotation rate, respectively, using a short interrogation time of 0.87 ms (interference area A=0.097mm2). This work provides a building block for an atomic interferometer-based inertial measurement unit for use in field applications that require a high data rate and high stability.