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SIMULTANEOUS DUAL LASER STABILIZATION FOR STRONTIUM ATOM INTERFEROMETRY

Spakowski, Matthew D.

Published Sep 1, 2022• 0 citations
OpenAlex

Abstract

The use of strontium in an atom interferometer presents the opportunity to perform detailed measurements of gravitational fields, rotation rates, and clock transitions as well as other natural phenomena. Strontium can be particularly effective in atom interferometry experiments for two reasons. The first is that the intrinsic magnetic properties of strontium result in less sensitivity of the transition frequencies to magnetic noise, allowing for better measurements. Second, strontium atoms can be cooled to a lower temperature just through ordinary Doppler cooling than other atoms typically used in interferometry (e.g., rubidium). A lower temperature means less initial kinetic energy and hence lower spatial dispersion over the course of an experiment. A magneto-optical trap consisting of two primary cooling lasers and two repump lasers cools and confines strontium atoms for use in the interferometer. This thesis focuses on the repump lasers and includes the design and performance of the optical system that frequency stabilizes each laser. The system demonstrated the ability to simultaneously frequency lock the two repump lasers to the degree necessary to form a strontium magneto-optical trap.

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The use of strontium in an atom interferometer presents the opportunity to perform detailed measurements of gravitational fields, rotation rates, and clock transitions as well as other natural phenomena. Strontium can be particularly effective in atom interferometry experiments for two reasons. The first is that the intrinsic magnetic properties of strontium result in less sensitivity of the transition frequencies to magnetic noise, allowing for better measurements. Second, strontium atoms can be cooled to a lower temperature just through ordinary Doppler cooling than other atoms typically used in interferometry (e.g., rubidium). A lower temperature means less initial kinetic energy and hence lower spatial dispersion over the course of an experiment. A magneto-optical trap consisting of two primary cooling lasers and two repump lasers cools and confines strontium atoms for use in the interferometer. This thesis focuses on the repump lasers and includes the design and performance of the optical system that frequency stabilizes each laser. The system demonstrated the ability to simultaneously frequency lock the two repump lasers to the degree necessary to form a strontium magneto-optical trap.
The utilization of light-pulse atom interferometry presents a valuable technique that has found application in both fundamental scientific inquiries, such as investigating constants such as measurements of fine structure constant α and gravitational constant G, and practical endeavors including acceleration sensing and rotation measurements. This thesis delves into our implementation of a dual atom interferometer design involving the clock transition 1S0 → 3P0 in strontium, concurrently conducting the interferometric sequence on atoms in both ground and excited states. To facilitate the dual atom interferometer’s operation, we have firstly established a compact experimental setup with a transversely loaded bi-dimensional magneto-optical-trap (2D-MOT) to create a high flux source of cold strontium atoms. Introducing a novel cross-polarized bi-color atomic beam slower, we simultaneously addresses two excited Zeeman substates of the transition 1S0 → 1P1 in strontium-88, significantly enhancing the number of atoms prepared in the 461 nm MOT by around 10-fold. Following the 461 nm MOT, the atomic ensemble undergoes cooling in a 689 nm MOT, achieving atomic temperatures below 1 µK. We also install a network of eight magnetic field probes arranged around the cold atomic sample, enabling precise three-axis active control of magnetic fields down to the milligauss level. With the atoms confined in a 2D lattice at the magic-wavelength of 813.427 nm after the initial preparation phase, we conduct the magnetically-induced clock transition to create a statistical mixture state of ground and excited states. After a velocity selection stage, implementing a Mach-Zehnder interferometer with Bragg pulses operating at the magic-wavelength along the vertical axis, we conduct tests of the weak equivalence principle (WEP). The Eötvös ratio we found in our system stood at (1.8 ± 3.1) × 10−4, mainly limited by the finite temperature of the atomic cloud constraining the interrogation time. Furthermore, the dual atom interferometer scheme enables the measurement of state-dependent force and eventually polarizability difference via the phase shift between the atoms in different states, and we experimentally demonstrate this by introducing an additional light field gradient.
Atomic Caesium clocks have made an astonishing development in the past few decades, with them gaining an order of magnitude in precision every decade. A new generation of atomic optical clocks is now emerging, which is moving to the forefront of timekeeping. By going from microwave to optical frequencies these clocks are now reaching fractional uncertainty levels in the 10\\(^-\\)\\(^1\\)\\(^8\\), opening a whole new range of exciting applications. This thesis presents the design and implementation of an experiment for laser cooling of strontium atoms, focusing on the mobility of the setup, opening a range of new applications as a mobile clock. The experimental apparatus applies a range of new techniques for strontium, such as the use of a two dimensional magneto-optical trap for pre cooling atoms, allowing for a compact and transportable system. A mobile laser system for laser cooling strontium atoms was realized. This includes a frequency doubling system for the main cooling transition. The constructed monolithic frequency doubling cavity has generated 300 mW of blue light and proven to be a stable setup suitable for a mobile system. The 3D-MOT was able to capture 4 * 10\\(^5\\) atoms with a long lifetime of 5.5 s, with further improvements for a significant increase in atom number currently being implemented.
This thesis describes the first steps to fulfill the main objective of our project: the development of a gravimetry system based on the continuous monitoring of Bloch oscillations performed by ultra-cold strontium atoms.The realization of this project comprises three main stages: the first stage consists in obtaining a magneto-optical trap in the broad transition of 461 nm of strontium, the second stage is the transfer to a magneto-optical trap in the narrow intercombination line of 689 nm, and finally the third stage is the monitoring of Bloch oscillations of the cloud of atoms in a ring cavity.This work details the first stage of the project, the creation of an experimental apparatus which produces ultra-cold strontium atoms in the transition of 461 nm, as well as the characterization of the cloud of atoms, temperature, size, number of atoms, etc.For this project, a new experimental apparatus has been designed and realized.It involves an ultra-high vacuum system, magnetic field sources, laser systems and optical instruments which are required for cooling, trapping and repumping strontium atoms.A novel feature is the implementation of a transversely loaded two-dimensional magneto-optical trap, which serves as a source of a cold strontium atomic beam.A loading rate of the atomic beam into a nearby three-dimensional magneto-optical trap exceeding 10 5 s -1 for the 88 Sr isotope at a moderate dispenser temperature of 600 • C are reported.The temperature of the cloud is about 4 mK and its size 0.3 mm, these characteristics suggest that the state of the atomic trap is in optimal conditions to make the transfer to the optical magneto trap in the intercombination line and thus continue with the second stage of the project.
We report on the progress toward a dual-species cadmium and strontium atom interferometer for fundamental physics tests. We have developed and characterized a complete baseline laser system for cadmium, which provides the high power and narrow linewidth necessary for laser cooling and trapping and for performing atom interferometry, with upgraded systems for strontium also implemented. An overview of a design for cooling cadmium is presented, and we outline the basic design of a Cd–Sr atomic fountain, discussing atom launching techniques and the possible role of blackbody radiation. The excellent properties of cadmium and strontium, both individually and as a test pair, are discussed along with the enabled fundamental physics program of tests of the weak equivalence principle and the measurement of relativistic time dilation effects in quantum superpositions of clocks.
We present a detailed investigation of strontium magneto-optical trap (MOT) dynamics. Relevant physical quantities in the trap, such as temperature, atom number and density, and loss channels and lifetime, are explored with respect to various trap parameters. By studying the oscillatory response of a two-level 1S0–1P1 88Sr MOT, we firmly establish the laser cooling dynamics predicted by Doppler theory. Measurements of the MOT temperature, however, deviate severely from Doppler theory predictions, implying significant additional heating mechanisms. To explore the feasibility of attaining quantum degenerate alkaline-earth samples via evaporative cooling, we also present the first experimental demonstration of magnetically trapped metastable 88Sr. Furthermore, motivated by the goal of establishing the fermionic isotope 87Sr as one of the highest-quality, neutral-atom-based optical frequency standards, we present a preliminary study of sub-Doppler cooling in a 87Sr MOT. A dual-isotope (87Sr and 88Sr) MOT is also demonstrated.
Optical atomic clocks have proven to be the most stable clocks with the lowest systematic uncertainty which has now reached a record level of (9.4 X10/(^{19}/)). Thus optical clocks now surpass the best fountain Cs atomic clocks by three orders of magnitude which opens the prospect of using optical clocks as frequency standards for timekeeping in the near future. \n \nThis thesis describes the progress that has been made towards a stationary optical lattice clock based on strontium atoms, and reports the results of an ongoing characterization. \n \nAn experimental apparatus was designed and built to efficiently slow, cool, and trap the strontium atoms which represent the heart of the strontium optical lattice clock discussed in this thesis. The novel aspects of the experimental development described in the thesis comprise a frequency doubling cavity for producing 461 nm laser light employed for cooling and trapping the strontium atoms in the first stage cooling. This cavity provided sufficient power for cooling and trapping the strontium atoms for up to 300 mW of 461 nm laser light. Furthermore, a new design of Zeeman slower based on spherical permanent magnets was produced, built and characterized. \n \nThe slower is compact, tunable, easy to assemble and maintain, and cost-effective as the permanent magnets do not require any power supply or water cooling. It is suggested that this kind of Zeeman slower constitutes an ideal solution for portable optical clock systems. A blue magneto-optical trap was realized for the first time with such a Zeeman slower. With about 30 mW of a 461 nm laser, up to 6X10/(^8/) atoms were captured.