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Optics Letters

Optical orbital angular momentum analogy to the Stern–Gerlach experiment

Angela L. Dudley, Bereneice Sephton, Thien An Nguyen, Nathan S. Brady, Sergei Slussarenko, R. R. Alfano, Andrew Forbes, Miles J. Padgett, Giovanni Milione, Martin P. J. Lavery

Published Aug 26, 2024• 1 citation
Publisher

Abstract

Symmetry breaking has been shown to reveal interesting phenomena in physical systems. A notable example is the fundamental work of Otto Stern and Walther Gerlach [Stern and Zerlach, Z. Physik9, 349 (1922)10.1007/BF01326983] nearly 100 years ago demonstrating a spin angular momentum (SAM) deflection that differed from classical theory. Here we use non-separable states of SAM and orbital angular momentum (OAM), known as vector vortex modes, to demonstrate how a classical optics analogy can be used to reveal this non-separability, reminiscent of the work carried out by Stern and Gerlach. We show that by implementing a polarization insensitive device to measure the OAM, the SAM states can be deflected to spatially resolved positions.

DOI
10.1364/ol.534320

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Symmetry breaking has been shown to reveal interesting phenomena in physical systems. A notable example is the fundamental work of Otto Stern and Walther Gerlach [Stern and Zerlach, Z. Physik9, 349 (1922)10.1007/BF01326983] nearly 100 years ago demonstrating a spin angular momentum (SAM) deflection that differed from classical theory. Here we use non-separable states of SAM and orbital angular momentum (OAM), known as vector vortex modes, to demonstrate how a classical optics analogy can be used to reveal this non-separability, reminiscent of the work carried out by Stern and Gerlach. We show that by implementing a polarization insensitive device to measure the OAM, the SAM states can be deflected to spatially resolved positions.
The insight that optical vortex beams carry orbital angular momentum (OAM), which emerged in Leiden about 30 years ago, has since led to an ever expanding range of applications and follow-up studies. This paper starts with a short personal account of how these concepts arose. This is followed by a description of some recent ideas where the coupling of transverse orbital and spin angular momentum (SAM) in tightly focused laser beams produces interesting new effects. The deflection of a focused light beam by an atom in the focus is reminiscent of the Magnus effect known from aerodynamics. Momentum conservation dictates an accompanying light force on the atom, transverse to the optical axis. As a consequence, an atom held in an optical tweezer will be trapped at a small distance of up to λ/2π away from the optical axis, which depends on the spin state of the atom and the magnetic field direction. This opens up new avenues to control the state of motion of atoms in optical tweezers as well as potential applications in quantum gates and interferometry.
Abstract In 1921, Otto Stern conceived the idea for an experiment that would decide between a classical and a quantum description of atomic behavior, as epitomized by the Bohr–Sommerfeld–Debye model of the atom. This model entailed not only the quantization of the magnitude of the orbital electronic angular momentum but also of the projection of the angular momentum on an external magnetic field – the so‐called space quantization. Stern recognized that space quantization would have observable consequences: namely, that the magnetic dipole moment due to the orbital angular momentum would be space quantized as well, taking two opposite values for atoms whose only unpaired electron has just one quantum of orbital angular momentum. When acted upon by a suitable inhomogeneous magnetic field, a beam of such atoms would be split into two beams consisting of deflected atoms with opposite projections of the orbital angular momentum on the magnetic field. In contradistinction, if atoms behaved classically, the atomic beam would only broaden along the field gradient and have maximum intensity at zero deflection, i. e., where there would be a minimum or no intensity for a beam split due to space quantization. Stern anticipated that, although simple in principle, the experiment would be difficult to carry out – and invited Walther Gerlach to team up with him. Gerlach's realism and experimental skills together with his sometimes stubborn determination to make things work proved invaluable for the success of the Stern–Gerlach experiment (SGE). After a long struggle, Gerlach finally saw, on 8 February 1922, the splitting of a beam of silver atoms in a magnetic field. The absence of the concept of electron spin confused and confounded the interpretation of the SGE, as the silver atoms were, in fact, in a 2S state, with zero orbital and spin angular momentum. However, a key quantum feature whose existence the SGE was designed to test – namely space quantization of electronic angular momentum – was robust enough to transpire independent of whether the electronic angular momentum was orbital or due to spin. The SGE entails other key aspects of quantum mechanics such as quantum measurement, state preparation, coherence, and entanglement. Confronted with the outcome of the SGE, Stern noted: “I still have objections to the idea of beauty of quantum mechanics. But she is correct.”
Abstract The insight that optical vortex beams carry orbital angular momentum (OAM), which emerged in Leiden about 30 years ago, has since led to an ever expanding range of applications and follow‐up studies. This paper starts with a short personal account of how these concepts arose. This is followed by a description of some recent ideas where the coupling of transverse orbital and spin angular momentum (SAM) in tightly focused laser beams produces interesting new effects. The deflection of a focused light beam by an atom in the focus is reminiscent of the Magnus effect known from aerodynamics. Momentum conservation dictates an accompanying light force on the atom, transverse to the optical axis. As a consequence, an atom held in an optical tweezer will be trapped at a small distance of up to λ /2 π away from the optical axis, which depends on the spin state of the atom and the magnetic field direction. This opens up new avenues to control the state of motion of atoms in optical tweezers as well as potential applications in quantum gates and interferometry.
The identification of orbital angular momentum (OAM) as a fundamental property of a beam of light nearly 25 years ago has led to an extensive body of research around this topic. The possibility that single photons can carry OAM has made this degree of freedom an ideal candidate for the investigation of complex quantum phenomena and their applications. Research in this direction has ranged from experiments on complex forms of quantum entanglement to the interaction between light and quantum states of matter. Furthermore, the use of OAM in quantum information has generated a lot of excitement, as it allows for encoding large amounts of information on a single photon. Here, we explain the intuition that led to the first quantum experiment with OAM 15 years ago. We continue by reviewing some key experiments investigating fundamental questions on photonic OAM and the first steps to applying these properties in novel quantum protocols. At the end, we identify several interesting open questions that could form the subject of future investigations with OAM.This article is part of the themed issue 'Optical orbital angular momentum'.
Thus far we have concentrated on the postulates, on their ramifications, and on the means and methods by which they are applied. Connections with classical physics have been featured, and primary notions other than those of Chapter 5 have not been needed. We deviate from this path in the present chapter, introducing a new and extremely important concept; it is based on one of the most significant and fruitful experiments of the quantal era. This experiment was performed by O. Stern and W. Gerlach (1921) and subsequently interpreted by G. Uhlenbeck and S. Goudsmit (1925). The experiment and its elucidation led to the new concept of “intrinsic spin” (in particular to spin “½”), a development that was one of the major turning points in modern physics. The consequences have been monumental, and include primary theoretical developments; the interpretation of data related to, and an understanding of, empirical rules concerning a wide variety of physical systems (e.g., the periodic table of the elements/atomic structure); and the generation of new experimental techniques and of innovative measurements. Our study of intrinsic spin and its correlative, two-state systems, introduces the reader to one of the most profound topics in quantum theory. The Stern–Gerlach experiment and its interpretation The experiment of Stern and Gerlach was designed to test the “spatial quantization” of neutral atoms, i.e., to determine whether the (orbital) angular momentum was quantized. The basic ideas are as follows. Associated with the atom's orbital angular momentum would be a magnetic moment, as in the Bohr model of hydrogen.
Optical vortices became a hot topic since almost two decades ago, when it was recognized that Laguerre-Gaussian laser modes carry orbital angular momentum [Allen et al. Phys Rev A 45, 8185 (1992)] related with a screw phase dislocation, and different from the spin angular momentum associated to circular polarization. In 1995, this dynamical quantity was transferred to matter in an optical micromanipulation system for the first time [H. He, et al., Phys. Rev. Lett. 75, 826 (1995)], and since then, a number of studies on angular momentum of light have unveiled different interesting aspects on the subject. However, there are still open questions, which have arisen together with the generation of novel light beams, such as vector vortices, for instance. In contrast with scalar vortices, with usual polarization states (linear, circular, elliptical), the orientation and magnitude of the electric field of vector vortices (solutions of the vector wave equation) is a function of space and time. In this work, we present an experimental study of the local angular momentum density of a Bessel vector vortex of first order by means of an optical trap. For this purpose, we used different probe particles in order to sense the local contribution to the optical angular momentum in each region of the beam. But optical fields are not the only wave fields that may exhibit phase dislocations or singularities. There are close analogies between light and sound fields that can be exploited in order to get a better understanding of common phenomena and study new aspects in both branches of physics. Here we also present the first experimental demonstration and theoretical analysis of acoustical vortices in free field, with similar properties to those of the optical vortices, including the angular momentum that can be transferred to matter. The corresponding analogies and differences with the optical case turn out to be very enlightening for the understanding of the phenomenon of angular momentum in wave fields.