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Physical Review Letters

Conditional Dynamics in Heterodyne Detection of Superradiant Lasing with Incoherently Pumped Atoms

Huihui Yu, Yuan Zhang, Qilong Wu, Chongxin Shan, Klaus Mølmer

Published Aug 12, 2024• 8 citations
Publisher

Abstract

In this Letter, we use quantum trajectory theory to simulate heterodyne detection of narrow bandwidth superradiant lasing from an incoherently excited atomic ensemble. To this end, we describe the system dynamics and account for stochastic measurement backaction by second-order mean-field theory. Our simulations show how heterodyne measurements break the phase symmetry, and initiate the atomic coherence with a random phase and a long temporal phase coherence. More importantly, our theory allows direct simulation of experimental procedures for extraction of spectral information which do not lend themselves to evaluation with the quantum regression theorem.

DOI
10.1103/physrevlett.133.073601

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In this Letter, we use quantum trajectory theory to simulate heterodyne detection of narrow bandwidth superradiant lasing from an incoherently excited atomic ensemble. To this end, we describe the system dynamics and account for stochastic measurement backaction by second-order mean-field theory. Our simulations show how heterodyne measurements break the phase symmetry, and initiate the atomic coherence with a random phase and a long temporal phase coherence. More importantly, our theory allows direct simulation of experimental procedures for extraction of spectral information which do not lend themselves to evaluation with the quantum regression theorem.
A recent experiment demonstrated heterodyne detection-based frequency measurements with superradiant pulses from coherently pumped strontium atoms in an optical lattice clock system, while another experiment has analyzed the statistics of superradiant pulses from incoherently pumped calcium atoms in a similar system. In this article, we propose to perform heterodyne detection of the superradiant pulses from the calcium atoms, and analyze theoretically the corresponding atomic ensemble dynamics in terms of the rotation of a collective spin vector and the incoherent quantum jumps among superradiant Dicke states. We examine the effect of quantum measurement backaction on the emitted field and the collective spin vector dynamics, and we demonstrate that it plays an essential role in the modelling of the frequency measurements. We develop a stochastic mean field theory, which is also applicable to model frequency measurements with steady-state superradiance signals, and to explore quantum measurement effects in the dynamics of atomic ensembles.
Background: Theoretical studies of superradiant lasing on optical clock transitions predict a superb frequency accuracy and precision closely tied to the bare atomic linewidth. Such a superradiant laser is also robust against cavity fluctuations when the spectral width of the lasing mode is much larger than that of the atomic medium. Recent predictions suggest that this unique feature persists even for a hot and thus strongly broadened ensemble, provided the effective atom number is large enough. Methods: Here we use a second-order cumulant expansion approach to study the power, linewidth and lineshifts of such a superradiant laser as a function of the inhomogeneous width of the ensemble including variations of the spatial atom-field coupling within the resonator. Results: We present conditions on the atom numbers, the pump and coupling strengths required to reach the buildup of collective atomic coherence as well as scaling and limitations for the achievable laser linewidth. Conclusions: We show how sufficiently large numbers of atoms subject to strong optical pumping can induce synchronization of the atomic dipoles over a large bandwidth. This generates collective stimulated emission of light into the cavity mode leading to narrow-band laser emission at the average of the atomic frequency distribution. The linewidth is orders of magnitudes smaller than that of the cavity as well as the inhomogeneous gain broadening and exhibits reduced sensitivity to cavity frequency noise.
We simulate the superradiant dynamics of ensembles of atoms in the presence of collective and individual atomic decay processes. We apply the Monte-Carlo wave-function method and identify quantum jumps in a reduced Dicke state basis, which reflects the permutation symmetry of the system. While the number of density matrix elements in the Dicke representation increases polynomially with atom number, the quantum jump dynamics populates only a single Dicke state at the time and thus efficient simulations can be carried out for tens of thousands of atoms. The superradiant pulses from initially excited atoms agree quantitatively with recent experimental results of strontium atoms but rapid atom loss in these experiments does not permit steady-state superradiance. By introducing an incident flux of new atoms to maintain a large average atom number, our theoretical calculations predict lasing with a millihertz linewidth despite rapid atom number fluctuations.
The stochastic dynamics of the quantum state of a laser conditioned on continuous intensity and phase-sensitive measurements on its output are examined. We first develop the essential model for a Poissonian laser, and then generalize it for regularly pumped lasers. We show that the rate of phase diffusion (which gives the laser linewidth) is not affected by the regularity of the pump. In both cases, heterodyne detection causes the phase variance in the conditioned laser state to become very small, yet remain significantly above (at least three times) that of a coherent state. The phase diffusion is manifest by a random walk undertaken by the mean phase, with the stochasticity arising from the local-oscillator shot noise. In contrast, intensity measurements have no effect on a Poissonian laser. For a perfectly regularly pumped laser, coarse-grained intensity measurements (for which an approximate theory is developed here) collapse the state to one with an arbitrarily small photon-number variance-to-mean ratio.
We use the quantum trajectory (stochastic wave function) approach to simulate the dynamics of a cavity QED system. The system consists of one atom interacting on resonance with one mode of a coherently driven optical cavity. We simulate a variety of different measurements on this system. The simulation of direct photoelectric detection produces trajectories that illustrate the collapse of the wave function in delayed photon coincidence measurements. It also allows us to calculate waiting-time distributions, pho­toelectron counting distributions, and the mean transmitted intensity as a function of the excitation frequency and field strength. A simulation with frequency filtering of the stochastic wave fuction gives results for optical spectra. From a simulation of homodyne detection we obtain trajectories showing the fluctuations in the quadrature phase amplitudes of the intracavity field and the atomic dipole. These simulations are used to calculate spectra of squeezing. We show that when the cavity is excited near one of the "vacuum" Rabi resonances, the composite atom-cavity system behaves like a two-state system. Under these conditions the optical spectrum shows Mollow sidebands caused by a dynamic Stark shift of the Jaynes-Cummings eigenstates. Thus, in this measurement we are observing the "dressing" of the (one-quantum) dressed states.
We develop a stochastic mean-field theory to describe active frequency measurements of pulsed superradiant emission, studied in a recent experiment with strontium-87 atoms trapped in an optical lattice inside an optical cavity [M. Norcia et al., Phys. Rev. X 8, 021036 (2018)PRXHAE2160-330810.1103/PhysRevX.8.021036]. Our theory reveals the intriguing dynamics of atomic ensembles with multiple transition frequencies, and it reproduces the superradiant beats signal, noisy power spectra, and frequency uncertainty in remarkable agreement with the experiments. Moreover, using longer superradiant pulses of similar strength and shortening the experimental duty cycle, we predict a short-term frequency uncertainty 7×10^{-17}/sqrt[τ/s], which makes active frequency measurements with superradiant transitions comparable with the record performance of current frequency standards [M. Schioppo et al., Nat. Photonics 11, 48 (2017)NPAHBY1749-488510.1038/nphoton.2016.231]. Our theory combines cavity quantum electrodynamics and quantum measurement theory, and it can be readily applied to explore conditional quantum dynamics and describe frequency measurements for other processes such as steady-state superradiance and superradiant Raman lasing.