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Nature Electronics

Quantum paraelectric varactors for radiofrequency measurements at millikelvin temperatures

P. Apostolidis, Byron J. Villis, Jacob F. Chittock-Wood, J. M. Powell, Andreas Baumgartner, Visa Vesterinen, Slawomir Simbierowicz, Juha Hassel, Mark R. Buitelaar

Published Aug 5, 2024• 12 citations
Publisher

Abstract

Abstract Radiofrequency reflectometry can provide fast and sensitive electrical read-out of charge and spin qubits in quantum dot devices coupled to resonant circuits. In situ frequency tuning and impedance matching of the resonator circuit using voltage-tunable capacitors (varactors) is needed to optimize read-out sensitivity, but the performance of conventional semiconductor- and ferroelectric-based varactors degrades substantially in the millikelvin temperature range relevant for solid-state quantum devices. Here we show that strontium titanate and potassium tantalate, materials which can exhibit quantum paraelectric behaviour with large field-tunable permittivity at low temperatures, can be used to make varactors with perfect impedance matching and resonator frequency tuning at 6 mK. We characterize the varactors at 6 mK in terms of their capacitance tunability, dissipative losses and magnetic field insensitivity. We use the quantum paraelectric varactors to optimize the radiofrequency read-out of carbon nanotube quantum dot devices, achieving a charge sensitivity of 4.8 μe Hz−1/2 and a capacitance sensitivity of 0.04 aF Hz−1/2.

DOI
10.1038/s41928-024-01214-z

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Abstract Radiofrequency reflectometry can provide fast and sensitive electrical read-out of charge and spin qubits in quantum dot devices coupled to resonant circuits. In situ frequency tuning and impedance matching of the resonator circuit using voltage-tunable capacitors (varactors) is needed to optimize read-out sensitivity, but the performance of conventional semiconductor- and ferroelectric-based varactors degrades substantially in the millikelvin temperature range relevant for solid-state quantum devices. Here we show that strontium titanate and potassium tantalate, materials which can exhibit quantum paraelectric behaviour with large field-tunable permittivity at low temperatures, can be used to make varactors with perfect impedance matching and resonator frequency tuning at 6 mK. We characterize the varactors at 6 mK in terms of their capacitance tunability, dissipative losses and magnetic field insensitivity. We use the quantum paraelectric varactors to optimize the radiofrequency read-out of carbon nanotube quantum dot devices, achieving a charge sensitivity of 4.8 μe Hz−1/2 and a capacitance sensitivity of 0.04 aF Hz−1/2.
Radio-frequency reflectometry allows for fast and sensitive electrical readout of charge and spin qubits hosted in quantum dot devices coupled to resonant circuits. Optimizing readout, however, requires frequency tuning of the resonators and impedance matching. This is difficult to achieve using conventional semiconductor or ferroelectric-based varactors in the detection circuit as their performance degrades significantly in the mK temperature range relevant for solid-state quantum devices. Here we explore a different type of material, strontium titanate, a quantum paraelectric with exceptionally large field-tunable permittivity at low temperatures. Using strontium titanate varactors we demonstrate perfect impedance matching and resonator frequency tuning at 6 mK and characterize the varactors at this temperature in terms of their capacitance tunability, dissipative losses and magnetic field sensitivity. We show that this allows us to optimize the radio-frequency readout signal-to-noise ratio of carbon nanotube quantum dot devices to achieve a charge sensitivity of 4.8 μμμe/Hz1/2^{1/2}1/2 and capacitance sensitivity of 0.04 aF/Hz1/2^{1/2}1/2.
Radio-frequency reflectometry techniques enable high-bandwidth readout of semiconductor quantum dots. Careful impedance matching of the resonant circuit is required to achieve high sensitivity, which, however, proves challenging at cryogenic temperatures. Gallium arsenide--based voltage-tunable capacitors, so-called varactor diodes, can be used for in situ tuning of the circuit impedance but deteriorate and fail at temperatures below 10 K and in magnetic fields. Here, we investigate a varactor based on strontium titanate with a hyperabrupt capacitance-voltage characteristic, i.e., a capacitance tunability similar to the best gallium arsenide--based devices. The varactor design introduced here is compact, scalable, and easy to wire bond, with an accessible capacitance range from 45 pF to 3.2 pF. We tune a resonant inductor-capacitor circuit to perfect impedance matching and observe robust temperature- and field-independent matching down to 11 mK and up to 2 T in-plane field. Finally, we perform gate-dispersive charge sensing on a germanium-silicon core-shell nanowire hole double quantum dot, paving the way toward gate-based single-shot spin readout. Our results bring small magnetic field--resilient highly tunable varactors to mK temperatures, expanding the toolbox of cryo-radio-frequency applications.
Electrical readout of spin qubits requires fast and sensitive measurements, which are hindered by poor impedance matching to the device. We demonstrate perfect impedance matching in a radio-frequency readout circuit, using voltage-tunable varactors to cancel out parasitic capacitances. An optimized capacitance sensitivity of 1.6 aF/√Hz is achieved at a maximum source-drain bias of 170−μV root-mean-square and with a bandwidth of 18 MHz. Coulomb blockade in a quantum-dot is measured in both conductance and capacitance, and the two contributions are found to be proportional as expected from a quasistatic tunneling model. We benchmark our results against the requirements for single-shot qubit readout using quantum capacitance, a goal that has so far been elusive.
Frequency tuning enables both high-sensitivity and wide-bandwidth detection in the resonator. Potassium tantalate (KTO) is a quantum paraelectric with tunable permittivity and low microwave loss at cryogenic temperature, making it promising for tunable devices. Here, we demonstrate a superconducting microwave resonator on a KTO substrate. The resonant frequency can be tuned by ∼40 MHz using a 9 V bias at 20 mK, with no observable hysteresis. The absence of hysteresis is a key metric for practical devices, addressing one of the major obstacles in other paraelectric-based tunable resonators. More interestingly, we observed that the quality factor oscillates during voltage tuning, arising from the competition between phonon hardening and charge injection. Therefore, our work provides a practical tunable resonator platform and offers a potential approach to study energy-loss characteristics in quantum paraelectrics.
We present a sensitive, tunable radio-frequency resonator designed to detect reactive changes in nanoelectronic devices down to dilution refrigerator temperatures. The resonator incorporates GaAs varicap diodes to allow electrical tuning of the resonant frequency and the coupling to the input line. We find a resonant frequency tuning range of 8.4 MHz at 55 mK that increases to 29 MHz at 1.5 K. To assess the impact on performance of different tuning conditions, we connect a quantum dot in a silicon nanowire field-effect transistor to the resonator and measure changes in the device capacitance caused by cyclic electron tunneling. At 250 mK, we obtain an equivalent charge sensitivity of 43 μe/Hz when the resonator and the line are impedance-matched and show that this sensitivity can be further improved to 31 μe/Hz by re-tuning the resonator. We understand this improvement by using an equivalent circuit model and demonstrate that for maximum sensitivity to capacitance changes, in addition to impedance matching, a high-quality resonator with low parasitic capacitance is desired.
Fault-tolerant spin-based quantum computers will require fast and accurate qubit read out. This can be achieved using radiofrequency reflectometry given sufficient sensitivity to the change in quantum capacitance associated with the qubit states. Here, we demonstrate a 23-fold improvement in capacitance sensitivity by supplementing a cryogenic semiconductor amplifier with a SQUID preamplifier. The SQUID amplifier operates at a frequency near 200 MHz and achieves a noise temperature below 600 mK when integrated into a reflectometry circuit, which is within a factor 120 of the quantum limit. It enables a record sensitivity to capacitance of 0.07aF/Hz. The setup is used to acquire charge stability diagrams of a gate-defined double quantum dot in a short time with a signal-to-noise ration of about 38 in 1μs of integration time.