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Physical review. B./Physical review. B

Magnetic properties of the spiral spin liquid and surrounding phases in the square lattice XY model

M. G. Gonzalez, Anna Fancelli, Han Yan, Johannes Reuther

Published Aug 5, 2024• 5 citations
Publisher

Abstract

Spiral spin liquids possess a subextensively degenerate ground-state manifold, represented by a continuum of energy minima in reciprocal space. Since a small change of the spiral state wave vector requires a global change of the spin configuration in real space, it is a priori unclear how such systems can fluctuate within the degenerate ground-state manifold. Only recently it was proposed that momentum vortices are responsible for the liquidity of the spiral phase and that these systems are closely related to an emergent rank-2 U(1) gauge theory H. Yan et al. [Phys. Rev. Res. 4, 023175 (2022)]. As a consequence of this gauge structure, fourfold pinch-point singularities were found in a generalized spin correlator. In this paper, we use classical Monte Carlo and molecular dynamics calculations to embed the previously studied spiral spin liquid into a broader phase diagram of the square lattice XY model. We find a multitude of unusual phases and phase transitions surrounding the spiral spin liquid such as an effective four-state Potts transition into a collinear double-striped phase resulting from the spontaneous breaking of two coupled ${\mathbb{Z}}_{2}$ symmetries. Since this phase is stabilized by entropic effects selecting the momenta away from the spiral manifold, it undergoes a second phase transition at low temperatures into a nematic spiral phase which only breaks one ${\mathbb{Z}}_{2}$ symmetry. We also observe a region of parameters where the phase transition into the spiral spin liquid does not break any symmetries and where the critical exponents do not match those of standard universality classes. We study the importance of momentum vortices in driving this phase transition and discuss the possibility of a Kosterlitz-Thouless transition of momentum vortices. Finally, we explore the regime where the rank-2 U(1) gauge theory is valid by investigating the fourfold pinch-point singularities across the phase diagram.

DOI
10.1103/physrevb.110.085106

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Spiral spin liquids possess a subextensively degenerate ground-state manifold, represented by a continuum of energy minima in reciprocal space. Since a small change of the spiral state wave vector requires a global change of the spin configuration in real space, it is a priori unclear how such systems can fluctuate within the degenerate ground-state manifold. Only recently it was proposed that momentum vortices are responsible for the liquidity of the spiral phase and that these systems are closely related to an emergent rank-2 U(1) gauge theory H. Yan et al. [Phys. Rev. Res. 4, 023175 (2022)]. As a consequence of this gauge structure, fourfold pinch-point singularities were found in a generalized spin correlator. In this paper, we use classical Monte Carlo and molecular dynamics calculations to embed the previously studied spiral spin liquid into a broader phase diagram of the square lattice XY model. We find a multitude of unusual phases and phase transitions surrounding the spiral spin liquid such as an effective four-state Potts transition into a collinear double-striped phase resulting from the spontaneous breaking of two coupled Z2{\mathbb{Z}}_{2}Z2​ symmetries. Since this phase is stabilized by entropic effects selecting the momenta away from the spiral manifold, it undergoes a second phase transition at low temperatures into a nematic spiral phase which only breaks one Z2{\mathbb{Z}}_{2}Z2​ symmetry. We also observe a region of parameters where the phase transition into the spiral spin liquid does not break any symmetries and where the critical exponents do not match those of standard universality classes. We study the importance of momentum vortices in driving this phase transition and discuss the possibility of a Kosterlitz-Thouless transition of momentum vortices. Finally, we explore the regime where the rank-2 U(1) gauge theory is valid by investigating the fourfold pinch-point singularities across the phase diagram.
Spiral spin liquids possess a subextensively degenerate ground-state manifold, represented by a continuum of energy minima in reciprocal space. Since a small change of the spiral state wavevector requires a global change of the spin configuration in real space, it is a priori unclear how such systems can fluctuate within the degenerate ground state manifold. Only recently it was proposed that momentum vortices are responsible for the liquidity of the spiral phase and that these systems are closely related to an emergent rank-2 U(1) gauge theory [H. Yan and J. Reuther, Phys. Rev. Research 4, 023175 (2022)]. As a consequence of this gauge structure, four-fold pinch-point singularities were found in a generalized spin correlator. In this article, we use classical Monte Carlo and molecular dynamics calculations to embed the previously studied spiral spin liquid into a broader phase diagram of the square lattice XY model. We find a multitude of unusual phases and phase transitions surrounding the spiral spin liquid such as an effective four-state Potts transition into a colinear double-striped phase resulting from the spontaneous breaking of two coupled Z2\mathbb{Z}_2Z2​ symmetries. Since this phase is stabilized by entropic effects selecting the momenta away from the spiral manifold, it undergoes a re-entrance phenomenon at low temperatures into a nematic spiral phase. We also observe a region of parameters where the phase transition into the spiral spin liquid does not break any symmetries and where the critical exponents do not match those of standard universality classes. We study the importance of momentum vortices in driving this phase transition and discuss the possibility of a Kosterlitz-Thouless transition of momentum vortices. Finally, we explore the regime where the rank-2 U(1) gauge theory is valid by investigating the four-fold pinch point singularities across the phase diagram
In this paper we identify a previously unexplored type of topological defect in spiral spin liquids---the momentum vortex---and reveal its dominant role in shaping the low-energy physics of such systems. Spiral spin liquids are a class of classical spin liquids featuring subextensively degenerate ground states. They are distinct from spin liquids on geometrically frustrated lattices, in which the ground-state degeneracy is extensive and connected by local spin flips. Despite a handful of experimental realizations and many theoretical studies, a concrete physical picture of their spin liquidity has not been established so far. In this paper, we study a 2D spiral spin liquid model to answer this question. We find that the local momentum vector field can carry topological defects in the form of vortices, which, however, have very different properties from the commonly known spin vortices. The fluctuations of such vortices lead the system into a liquid phase at intermediate temperatures. Furthermore, the effective low-energy theory of such vortices indicates their equivalence to quadrupoles of fractons in a rank-2 U(1) gauge theory or, alternatively, to quadrupoles of disclinations in elasticity theory. At very low temperatures, the system freezes into a glassy state in which these vortices form a rigid network with straight-line domain walls. Our paper sheds light on the nature of spiral spin liquids and also paves the way toward understanding their quantum limit.
We introduce a geometrically frustrated classical Ising model, dubbed the “spin-vorticity model,” whose ground-state manifold is a classical spin liquid: a 2-form Coulomb phase. We study the thermodynamics of this model both analytically and numerically, exposing the presence of algebraically decaying correlations and an extensive ground-state entropy, and give a comprehensive account of its ground-state properties and excitations. Each classical ground state may be decomposed into collections of closed two-dimensional membranes, supporting fractionalized string excitations attached to the edges of open membranes. At finite temperature, the model can then be described as a gas of closed strings in a background of fluctuating membranes. The emergent gauge structure of this spin liquid is naturally placed in the language of 2-form electrodynamics, which describes one-dimensional charged strings coupled to a rank-2 antisymmetric gauge field. After establishing the classical spin-vorticity model, we consider perturbing it with quantum exchange interactions, deriving an effective “membrane exchange” model of the quantum dynamics, analogous to ring exchange in quantum spin ice. We demonstrate the existence of a Rokhsar-Kivelson point where the quantum ground state is an equal-weight superposition of all classical ground-state configurations, i.e., a quantum spin liquid. The quantum aspects of this spin liquid are exposed by mapping the membrane exchange model to a strongly coupled frustrated 2-form U(1) lattice gauge theory. We further demonstrate how to quantize the string excitations by coupling a 1-form string field to the 2-form U(1) gauge field, thus mapping a quantum spin model to a 2-form U(1) gauge-Higgs model. We discuss the stability of the gapless deconfined phase of this gauge theory and the possibility of realizing a class of quantum phases of matter: 2-form U(1) quantum spin liquids.
We obtain an almost complete understanding of the mean-field phase diagram of the two-dimensional Hubbard model on a square lattice with a sizable next-nearest-neighbor hopping and a moderate interaction strength. In particular, we clarify the nature of the transition region between the spiral and the stripe phase. Complementing previous [] real-space Hartree-Fock calculations on large finite lattices, we solve the mean-field equations for coplanar unidirectional magnetic order directly in the thermodynamic limit, and we determine the nature of the magnetic states right below the mean-field critical temperature T * by a Landau free-energy analysis. While the magnetic order for filling factors n ≥ 1 is always of Néel type, for n ≤ 1 the following sequence of magnetic states is found as a function of increasing hole-doping: Néel, planar circular spiral, multispiral, and collinear spin-charge stripe states. Multispiral states are superpositions of several spirals with distinct wave vectors, and lead to concomitant charge order. We finally point out that nematic and charge orders inherited from the magnetic order can survive even in the presence of fluctuations, and we present a corresponding qualitative phase diagram. Published by the American Physical Society 2024
We study a generalization of the well-known classical two-dimensional square lattice compass model of XY spins (sometimes referred to as the ${90}^{\ensuremath{\circ}}$ compass model), which interpolates between the XY model and the compass model. Our model possesses the combined C4{C}_{4}C4​ lattice and spin rotation symmetry of the compass model but is free of its fine-tuned subsystem symmetries. Using both field theoretic arguments and Monte Carlo simulations, we find that our model possesses a line of critical points with continuously varying exponents of the Ashkin-Teller type terminating at the four-state Potts point. Further, our Monte Carlo study uncovers that beyond the four-state Potts point, the line of phase transition is connected to the lattice-nematic Ising phase transition in the square lattice compass model through a region of first-order transitions.
The algebraic spin liquid is a long-sought-after phase of matter characterized by the absence of quasiparticle excitations, a low-energy description in terms of emergent Dirac fermions and gauge fields interacting according to (2+1)(2+1)(2+1)-dimensional quantum electrodynamics (QED3)({\mathrm{QED}}_{3})(QED3​), and power-law correlations with universal exponents. The prototypical algebraic spin liquid is the Affleck-Marston $\ensuremath{\pi}$-flux phase, originally proposed as a possible ground state of the spin-12\frac{1}{2}21​ Heisenberg model on the two-dimensional square lattice. While the latter model is now known to order antiferromagnetically at zero temperature, recent sign-problem-free quantum Monte Carlo simulations of spin-12\frac{1}{2}21​ fermions coupled to a compact U(1)\text{U}(1)U(1) gauge field on the square lattice have shown that quantum fluctuations can destroy N\'eel order and drive a direct quantum phase transition to the $\ensuremath{\pi}$-flux phase. We show this transition is in the universality class of the chiral Heisenberg QED3{\mathrm{QED}}_{3}QED3​-- Gross-Neveu-Yukawa model with a single SU(2)\text{SU}(2)SU(2) doublet of four-component Dirac fermions (i.e., Nf=1){N}_{f}=1)Nf​=1), pointing out important differences with the corresponding putative transition on the kagome lattice. Using an $\ensuremath{\epsilon}$ expansion below four space-time dimensions to four-loop order, and a large-Nf{N}_{f}Nf​ expansion up to second order, we show the transition is continuous and compute various thermodynamic and susceptibility critical exponents at this transition, setting the stage for future numerical determinations of these quantities. As a by-product of our analysis, we also obtain charge-density-wave and valence-bond-solid susceptibility exponents at the semimetal-N\'eel transition for interacting fermions on the honeycomb lattice.