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arXiv:2112.10676 · Physical Review Research

Low-energy structure of spiral spin liquids

Han Yan, Johannes Reuther

Published Jun 1, 2022• 27 citations
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Abstract

In this paper we identify a previously unexplored type of topological defect in spiral spin liquids---the momentum vortex---and reveal its dominant role in shaping the low-energy physics of such systems. Spiral spin liquids are a class of classical spin liquids featuring subextensively degenerate ground states. They are distinct from spin liquids on geometrically frustrated lattices, in which the ground-state degeneracy is extensive and connected by local spin flips. Despite a handful of experimental realizations and many theoretical studies, a concrete physical picture of their spin liquidity has not been established so far. In this paper, we study a 2D spiral spin liquid model to answer this question. We find that the local momentum vector field can carry topological defects in the form of vortices, which, however, have very different properties from the commonly known spin vortices. The fluctuations of such vortices lead the system into a liquid phase at intermediate temperatures. Furthermore, the effective low-energy theory of such vortices indicates their equivalence to quadrupoles of fractons in a rank-2 U(1) gauge theory or, alternatively, to quadrupoles of disclinations in elasticity theory. At very low temperatures, the system freezes into a glassy state in which these vortices form a rigid network with straight-line domain walls. Our paper sheds light on the nature of spiral spin liquids and also paves the way toward understanding their quantum limit.

DOI
10.1103/physrevresearch.4.023175

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In this paper we identify a previously unexplored type of topological defect in spiral spin liquids---the momentum vortex---and reveal its dominant role in shaping the low-energy physics of such systems. Spiral spin liquids are a class of classical spin liquids featuring subextensively degenerate ground states. They are distinct from spin liquids on geometrically frustrated lattices, in which the ground-state degeneracy is extensive and connected by local spin flips. Despite a handful of experimental realizations and many theoretical studies, a concrete physical picture of their spin liquidity has not been established so far. In this paper, we study a 2D spiral spin liquid model to answer this question. We find that the local momentum vector field can carry topological defects in the form of vortices, which, however, have very different properties from the commonly known spin vortices. The fluctuations of such vortices lead the system into a liquid phase at intermediate temperatures. Furthermore, the effective low-energy theory of such vortices indicates their equivalence to quadrupoles of fractons in a rank-2 U(1) gauge theory or, alternatively, to quadrupoles of disclinations in elasticity theory. At very low temperatures, the system freezes into a glassy state in which these vortices form a rigid network with straight-line domain walls. Our paper sheds light on the nature of spiral spin liquids and also paves the way toward understanding their quantum limit.
Spiral spin liquids possess a subextensively degenerate ground-state manifold, represented by a continuum of energy minima in reciprocal space. Since a small change of the spiral state wave vector requires a global change of the spin configuration in real space, it is a priori unclear how such systems can fluctuate within the degenerate ground-state manifold. Only recently it was proposed that momentum vortices are responsible for the liquidity of the spiral phase and that these systems are closely related to an emergent rank-2 U(1) gauge theory H. Yan et al. [Phys. Rev. Res. 4, 023175 (2022)]. As a consequence of this gauge structure, fourfold pinch-point singularities were found in a generalized spin correlator. In this paper, we use classical Monte Carlo and molecular dynamics calculations to embed the previously studied spiral spin liquid into a broader phase diagram of the square lattice XY model. We find a multitude of unusual phases and phase transitions surrounding the spiral spin liquid such as an effective four-state Potts transition into a collinear double-striped phase resulting from the spontaneous breaking of two coupled Z2{\mathbb{Z}}_{2}Z2​ symmetries. Since this phase is stabilized by entropic effects selecting the momenta away from the spiral manifold, it undergoes a second phase transition at low temperatures into a nematic spiral phase which only breaks one Z2{\mathbb{Z}}_{2}Z2​ symmetry. We also observe a region of parameters where the phase transition into the spiral spin liquid does not break any symmetries and where the critical exponents do not match those of standard universality classes. We study the importance of momentum vortices in driving this phase transition and discuss the possibility of a Kosterlitz-Thouless transition of momentum vortices. Finally, we explore the regime where the rank-2 U(1) gauge theory is valid by investigating the fourfold pinch-point singularities across the phase diagram.
Spiral spin liquids possess a subextensively degenerate ground-state manifold, represented by a continuum of energy minima in reciprocal space. Since a small change of the spiral state wavevector requires a global change of the spin configuration in real space, it is a priori unclear how such systems can fluctuate within the degenerate ground state manifold. Only recently it was proposed that momentum vortices are responsible for the liquidity of the spiral phase and that these systems are closely related to an emergent rank-2 U(1) gauge theory [H. Yan and J. Reuther, Phys. Rev. Research 4, 023175 (2022)]. As a consequence of this gauge structure, four-fold pinch-point singularities were found in a generalized spin correlator. In this article, we use classical Monte Carlo and molecular dynamics calculations to embed the previously studied spiral spin liquid into a broader phase diagram of the square lattice XY model. We find a multitude of unusual phases and phase transitions surrounding the spiral spin liquid such as an effective four-state Potts transition into a colinear double-striped phase resulting from the spontaneous breaking of two coupled Z2\mathbb{Z}_2Z2​ symmetries. Since this phase is stabilized by entropic effects selecting the momenta away from the spiral manifold, it undergoes a re-entrance phenomenon at low temperatures into a nematic spiral phase. We also observe a region of parameters where the phase transition into the spiral spin liquid does not break any symmetries and where the critical exponents do not match those of standard universality classes. We study the importance of momentum vortices in driving this phase transition and discuss the possibility of a Kosterlitz-Thouless transition of momentum vortices. Finally, we explore the regime where the rank-2 U(1) gauge theory is valid by investigating the four-fold pinch point singularities across the phase diagram
We introduce a geometrically frustrated classical Ising model, dubbed the “spin-vorticity model,” whose ground-state manifold is a classical spin liquid: a 2-form Coulomb phase. We study the thermodynamics of this model both analytically and numerically, exposing the presence of algebraically decaying correlations and an extensive ground-state entropy, and give a comprehensive account of its ground-state properties and excitations. Each classical ground state may be decomposed into collections of closed two-dimensional membranes, supporting fractionalized string excitations attached to the edges of open membranes. At finite temperature, the model can then be described as a gas of closed strings in a background of fluctuating membranes. The emergent gauge structure of this spin liquid is naturally placed in the language of 2-form electrodynamics, which describes one-dimensional charged strings coupled to a rank-2 antisymmetric gauge field. After establishing the classical spin-vorticity model, we consider perturbing it with quantum exchange interactions, deriving an effective “membrane exchange” model of the quantum dynamics, analogous to ring exchange in quantum spin ice. We demonstrate the existence of a Rokhsar-Kivelson point where the quantum ground state is an equal-weight superposition of all classical ground-state configurations, i.e., a quantum spin liquid. The quantum aspects of this spin liquid are exposed by mapping the membrane exchange model to a strongly coupled frustrated 2-form U(1) lattice gauge theory. We further demonstrate how to quantize the string excitations by coupling a 1-form string field to the 2-form U(1) gauge field, thus mapping a quantum spin model to a 2-form U(1) gauge-Higgs model. We discuss the stability of the gapless deconfined phase of this gauge theory and the possibility of realizing a class of quantum phases of matter: 2-form U(1) quantum spin liquids.
Classical U(1) fracton spin liquids feature an extensive ground state degeneracy and follow an effective description in terms of a tensor Gauss's law where charges, so-called fractons, have restricted mobility. Here we introduce a simple spin model that realizes such a state by straightforward discretization of the higher-rank gauge theory on a square lattice. The simplicity of this construction offers direct insights into the system's fundamental fractonic properties, such as real-space fracton configurations, height-field representation of the classical ground state manifold as well as properties of local and nonlocal fluctuations within the fracton-free subspace. By sampling classical Ising states from the extensive ground state manifold, we show that the effective tensor Gauss's law remains intact when explicitly enforcing the spin-1/2 length constraint, demonstrating the existence of a classical Ising fracton spin liquid. However, we observe that perturbative quantum effects are insufficient to efficiently tunnel between classical ground states, leading to severe Hilbert space fragmentation which obscures fractonic quantum behavior. Specifically, by simulating the spin-1/2 quantum model with Green's function Monte Carlo as a function of the Rokhsar-Kivelson potential, we find that the system supports either magnetic long-range order or a classical spin liquid. Our findings highlight the crucial role of Hilbert-space fragmentation in fractonic spin systems but also indicate ways to mitigate such effects via increasing the spin magnitude to S = 1 , investigated in a companion paper.
The hallmark of highly frustrated systems is the presence of many states close in energy to the ground state. Fluctuations between these states can preclude the emergence of any form of order and lead to the appearance of spin liquids. Even on the classical level, spin liquids are not all alike: they may have algebraic or exponential correlation decay, and various forms of long wavelength description, including vector or tensor gauge theories. Here, we introduce a classification scheme, allowing us to fit the diversity of classical spin liquids (CSLs) into a general framework as well as predict and construct new kinds. CSLs with either algebraic or exponential correlation-decay can be classified via the properties of the bottom flat band(s) in their soft-spin Hamiltonians. The classification of the former is based on the algebraic structures of gapless points in the spectra, which relate directly to the emergent generalized Gauss's laws that control the low-temperature physics. The second category of CSLs, meanwhile, are classified by the fragile topology of the gapped bottom band(s). Utilizing the classification scheme we construct new models realizing exotic CSLs, including one with anisotropic generalized Gauss's laws and charges with subdimensional mobility, one with a network of pinch-line singularities in its correlation functions and a series of fragile topological CSLs connected by zero-temperature transitions. Published by the American Physical Society 2024
Gapless fracton quantum spin liquids are exotic phases of matter described by higher-rank U(1) gauge theories, which host gapped and immobile fracton matter excitations as well as gapless photons. Despite well-known field theories, no spin models beyond purely classical systems have been identified to realize these phases. Using error-controlled Green function Monte Carlo, here we investigate a square lattice spin-1 model that shows precise signatures of a fracton quantum spin liquid without indications of conventional ordering. Specifically, the magnetic response exhibits characteristic patterns of suppressed pinch points that accurately match the prediction of a rank-2 U(1) field theory and reveals the existence of emergent photon excitations in 2+1 spacetime dimensions. Remarkably, this type of fracton quantum spin liquid is not only identified in the system's ground state but also in generic low-energy sectors of a strongly fragmented Hilbert space.