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Materials Horizons

Fault-tolerant computing with single-qudit encoding in a molecular spin

Matteo Mezzadri, Alessandro Chiesa, Luca Lepori, Stefano Carretta

Published Jan 1, 2024• 16 citations
Publisher

Abstract

We show how to perform fault-tolerant quantum computing by using a simple d-level molecular spin qudit. We demonstrate a nearly exponential error reduction with linear growth in the number of single-qudit levels and loose coherence requirements.
DOI
10.1039/d4mh00454j

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Universal quantum computers require fault-tolerant logical qudits, as qudits naturally align with the simulation of multi-level physical systems. Here, we present a general framework and working examples for encoding fault-tolerant logical qudits in finite-dimensional spin systems. We construct distance-333, distance-555 codewords, and general 2t+12t+12t+1-distance codes that can be implemented using a single physical qudit or a small number of coupled qudits for higher distances, while requiring a Hilbert space dimension significantly smaller than conventional constructions based on multiple logical qubits. Logical operations and error correction protocols can be implemented with polynomial scaling in the number of elementary operations. We further discuss schematic designs for physical implementation and required single-gate fidelities, which are compatible with current spin qudit platforms. This strategy provides a resource-efficient path toward realizing fault-tolerant logical qudits in finite multi-level physical systems.
We construct a fault-tolerant quantum error-correcting protocol based on a qubit encoded in a large spin qudit using a spin-cat code, analogous to the continuous-variable cat encoding. With this, we can correct the dominant error sources, namely processes that can be expressed as error operators that are linear or quadratic in the components of angular momentum. Such codes tailored to dominant error sources can exhibit superior thresholds and lower resource overheads when compared to those designed for unstructured noise models. A key component is the gate that preserves the rank of spherical tensor operators. Categorizing the dominant errors as phase and amplitude errors, we demonstrate how phase errors, analogous to phase-flip errors for qubits, can be effectively corrected. Furthermore, we propose a measurement-free error-correction scheme to address amplitude errors without relying on syndrome measurements. Through an in-depth analysis of logical gate errors, we establish that the fault-tolerant threshold for error correction in the spin-cat encoding surpasses that of standard qubit-based encodings. We consider a specific implementation based on neutral-atom quantum computing, with qudits encoded in the nuclear spin of 87 Sr , and show how to generate the universal gate set, including the rank-preserving gate, using quantum control and the Rydberg blockade. These findings pave the way for encoding a qubit in a large spin with the potential to achieve fault tolerance, high threshold, and reduced resource overhead in quantum information processing. Published by the American Physical Society 2024
We propose multi-spin molecules as a viable architecture for fault-tolerant quantum computing. To this aim, we introduce a correction protocol handling both diagonal and off-diagonal errors, typically associated with dephasing and relaxation. The scheme is based on a hybrid encoding which combines dephasing-tolerant units suppressing the leading pure dephasing error into a multi-spin molecule implementing a multi-qubit code for residual off-diagonal errors. Our proposal leverages peculiar properties of molecular spins, i.e. the strong hierarchy between different errors and the possibility to engineer multi-spin molecules at the synthetic level. Moreover, it addresses the important issue of the loss of coherences in anharmonic systems subject to off-diagonal errors, which hampers their correction at the single spin level. Thanks to the huge suppression of dephasing by the first-level code, we numerically demonstrate the potential performance of this strategy even with a limited number of spins per logical unit.
We prove a fault-tolerance theorem for quantum computation against adversarial noise. For every quantum circuit on Nˉ\bar{N}Nˉ logical qudits of depth Tˉ\bar{T}Tˉ, we construct a fault-tolerant circuit on N=poly(Nˉ)N=\text{poly}(\bar{N})N=poly(Nˉ) physical qudits of depth Tˉ⋅Nˉo(1)\bar{T}\cdot\bar{N}^{o(1)}Tˉ⋅Nˉo(1), which is robust against an adversary who may arbitrarily choose and corrupt an almost-linear number N1−o(1)N^{1-o(1)}N1−o(1) of physical qudits at each time step. This robustness significantly improves upon prior fault-tolerance theorems, which assumed corruptions were either local and stochastic, or else only act on a polynomially vanishing fraction of qudits. Our fault-tolerance scheme addresses a key bottleneck towards constructing quantum PCPs via the circuit-to-Hamiltonian mapping of Anshu, Breuckmann, and Nguyen (STOC'24). More fundamentally, our result demonstrates that fault-tolerant quantum computation remains possible under noise models that are global, worst-case, and non-Markovian over the full duration of the computation, directly countering concerns that correlated noise could fundamentally undermine quantum fault tolerance. Our construction is based on a new family of subsystem product codes we develop, which have large dimension and distance along with low-weight parity-checks, and which support transversal non-Clifford gates. We show how to perform single-shot fault-tolerant error correction on these codes using a Floquet-like procedure based on the local testability of classical tensor codes. We then obtain a universal fault-tolerance scheme using repeated code switching in a hypercubic qudit architecture. Finally, we recursively compose our scheme with itself to reduce an initially exponential qudit dimension down to a constant.
A quantum computer is a powerful machine that provides a new approach to information processing based on quantum mechanics. However, basically, qubits are very vulnerable to errors, thus a quantum error correction code (QECC) is needed to build a reliable quantum computer. Moreover, simply using QECCs is not sufficient in order that a quantum computer can tolerate errors. In quantum computation, each operation must be performed on the encoded states. Even when the gates used to perform these operations are noisy, the quantum computation must be tolerable to the errors. This is called fault-tolerant quantum computation and it is an essential condition for implementing a quantum computer. However, considering the fault tolerance, the overhead of the quantum computer increases exponentially. In this paper, we introduce fault-tolerant quantum computation and schemes to reduce the its overhead.
The authors propose a quantum memory, implemented on a spin-7/2 nucleus coupled to an electron spin-1/2 qubit, which provides XXX, YYY, and ZZZ error correction using fewer quantum resources than the equivalently effective qubit-based protocols.