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New Journal of Physics

Interplay of electromagnetically induced transparency and Doppler broadening in hot atomic vapors

Lida Zhang, Nina Stiesdal, Hannes Busche, Mikkel G. Hansen, Thomas Pohl, Sebastian Hofferberth

Published Jul 1, 2024• 10 citations
Publisher

Abstract

Abstract For multi-level systems in hot atomic vapors the interplay between the Doppler shift due to atomic motion and the wavenumber mismatch between driving laser fields strongly influences transmission and absorption properties of the atomic medium. In a three-level atomic ladder-system, Doppler broadening limits the visibility of electromagnetically-induced transparency (EIT) when the probe and control fields are co-propagating, while EIT is recovered under the opposite condition of counter-propagating geometry and k p < k c , with k p and k c being the wavenumbers of the probe and control fields, respectively. This effect has been studied and experimentally demonstrated as an efficient mechanism to realize non-reciprocal probe light transmission, which may enable applications as magnetic-field free optical isolators. Here, we describe the basics of this effect and discuss a simple picture for the underlying mechanism. We illustrate how the non-reciprocity scales with wavelength mismatch and show how to experimentally demonstrate the effect in a simple Rydberg-EIT system using thermal Rubidium atoms.

DOI
10.1088/1367-2630/ad5d83

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Abstract For multi-level systems in hot atomic vapors the interplay between the Doppler shift due to atomic motion and the wavenumber mismatch between driving laser fields strongly influences transmission and absorption properties of the atomic medium. In a three-level atomic ladder-system, Doppler broadening limits the visibility of electromagnetically-induced transparency (EIT) when the probe and control fields are co-propagating, while EIT is recovered under the opposite condition of counter-propagating geometry and k p < k c , with k p and k c being the wavenumbers of the probe and control fields, respectively. This effect has been studied and experimentally demonstrated as an efficient mechanism to realize non-reciprocal probe light transmission, which may enable applications as magnetic-field free optical isolators. Here, we describe the basics of this effect and discuss a simple picture for the underlying mechanism. We illustrate how the non-reciprocity scales with wavelength mismatch and show how to experimentally demonstrate the effect in a simple Rydberg-EIT system using thermal Rubidium atoms.
For multi-level systems in hot atomic vapors the interplay between the Doppler shift due to atom velocity and the wavenubmer mismatch between driving laser fields strongly influences transmission and absorption properties of the atomic medium. In a three-level atomic ladder-system, Doppler broadening limits the visibility of electromagnetically-induced transparency (EIT) when the probe and control fields are co-propagating, while EIT is recovered under the opposite condition of counter-propagating geometry and kp<kck_{p} < k_{c}kp​<kc​, with kpk_{p}kp​ and kck_{c}kc​ being the wavenumbers of the probe and control fields, respectively. This effect has been studied and experimentally demonstrated as an efficient mechanism to realize non-reciprocal probe light transmission, opening promising avenues for example for realization of magnetic-field free optical isolators. In this tutorial we discuss the theoretical derivation of this effect and show the underlying mechanism to be an avoided crossing of the states dressed by the coupling laser as a function of atomic velocities when $k_{p}
Abstract We study the steady optical responses of a cold atomic ensemble driven into the three-level ladder configuration involving a Rydberg state at finite temperatures. By improving the superatom model with thermal movement included, we calculate relevant atomic coherence effects and find that the residual Doppler broadening at the mK–K temperatures will weaken the nonclassical properties of transmitted probe photons. Furthermore, propagation directions of the probe and coupling fields have a great influence on various properties related to electromagnetically induced transparency. That is, the residual Doppler effect is more destructive to relevant atomic coherence effects in the co-propagation case but can be partially eliminated in the counter-propagation case.
In a Doppler-broadened ladder-type Rubidium atomic system [Formula: see text]–[Formula: see text]–[Formula: see text], three-photon electromagnetically induced absorption (EIA) and transparency (EIT) in two schemes of two coupling lasers with different propagation directions are comprehensively studied. Two coupling fields are entangled tightly with each other and induce constructive interference such that we observe EIA as two coupling fields are counter-propagating. Two coupling fields are independent and cause destructive interference such that only enhanced EIT occurs when two coupling fields are co-propagating, although all of the Doppler-broadened atoms satisfy the condition for three-photon resonance. The experimental results are coincided with the numerically calculated spectra using the dressed perturbation method. The mechanisms of EIT and EIA could also be understood by the dressed-state pictures.
The propagation of a probe field through a four-level Y-type atomic system is described in the presence of two additional coherent radiation fields, namely, the control field and the coupling field. An expression for the probe response is derived analytically from the optical Bloch equations under steady state condition to study the absorptive properties of the system under probe field propagation through an ensemble of stationary atoms as well as in a Doppler broadened atomic vapor medium. The most striking result is the conversion of electromagnetically induced transparency (EIT) into electromagnetically induced absorption (EIA) as we start switching from weak probe regime to strong probe regime. The dependence of this conversion on residual Doppler averaging due to wavelength mismatch is also shown by choosing the coupling transition as a Rydberg transition.
The behavior of multilevel atomic ensembles (e.g., alkali-metal atoms) can be influenced significantly by the intensity of a driving field (or controlling/coupling field). The phase coherence between two transition pathways driven by a probe light and a driving field can lead to the effect known as electromagnetically induced transparency (EIT). In EIT, the probe light can pass through a three-level alkali-metal atomic vapor without absorption or reflection when two coherent resonances (transition pathways driven by the driving and probe fields) are present and the linewidths of the transparency windows are sufficiently narrow. The optical characteristics of atomic systems can also be affected by the Doppler broadening of the absorption profile in a spectroscope. Our analysis indicates that both broadenings (related to the transitions excited by the driving and probe fields) can be expanded, leading to an increase in the transmittance and reflectance broadenings when a coupling field with adaptive strength is applied; the corresponding temperature would, thus, be implemented and readable. We show that the most suitable preparation for temperature sensing via an EIT vapor is to provide 80 times the spontaneous decay rate (SDR) of the excited atomic levels. This configuration results in reflectance and transmittance values that range between zero and one and cover a temperature range of 0 K to 600 K. As an example, we demonstrate the integration of specialized coating technologies with EIT ensembles for temperature sensing in the range of dozens of kelvins at and above room temperature. A key advantage of this temperature-sensing system is its ability to use adaptive resonant visible light as the probe field. This novel approach may find applications in providing unprecedented levels of precision and control in temperature sensing for coating processes and in the design of other photonic or optical devices. It can also be used to determine the temperature-dependent behavior of the specific heat of alkali-metal solids and gases (including the latent heats of vaporization or sublimation of alkali-metal solids) through the reflection and transmission spectra of the vaporized EIT atomic vapors.
A three-level lambda system driven by multicolor control, pump, and probe fields is investigated. The pump and probe fields are derived from the same laser with opposite propagating directions. Due to the Doppler effect, the zero group-velocity atoms face bichromatic fields, while other atoms face trichromatic fields. The atomic medium shows distinct characteristics and exhibits simultaneous electromagnetically induced transparency (EIT) and electromagnetically induced absorption (EIA) at two frequencies. EIT and EIA peaks have a fixed relationship with frequency, which is determined by the Doppler shifts.