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Europhysics Letters (EPL)

Temporal coherences of atomic chaotic light sources: The Siegert relation and its generalisation to higher-order correlation functions

Martial Morisse, S. Joshi, Jaromír Mika, J. C. C. Capella, Robin Kaiser, Romain Bachelard, L. Slodička, Mathilde Hugbart

Published Jul 1, 2024• 1 citation
Publisher

Abstract

Abstract Light is characterized by its electric field, yet quantum optics has revealed the importance of monitoring photon-photon correlations at all orders. We here present a comparative study of two experimental setups, composed of cold and warm rubidium atoms, respectively, which allow us to probe and compare photon correlations. The former operates in the quantum regime where spontaneous emission dominates, whereas the latter exhibits a temperature-limited coherence time. We demonstrate our capability to measure photon correlations up to the fourth order which could be useful to better characterize light scattered by cold atoms beyond the chaotic statistics.

DOI
10.1209/0295-5075/ad5d87

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Abstract Light is characterized by its electric field, yet quantum optics has revealed the importance of monitoring photon-photon correlations at all orders. We here present a comparative study of two experimental setups, composed of cold and warm rubidium atoms, respectively, which allow us to probe and compare photon correlations. The former operates in the quantum regime where spontaneous emission dominates, whereas the latter exhibits a temperature-limited coherence time. We demonstrate our capability to measure photon correlations up to the fourth order which could be useful to better characterize light scattered by cold atoms beyond the chaotic statistics.
Light is characterized by its electric field, yet quantum optics has revealed the importance of monitoring photon-photon correlations at all orders. We here present a comparative study of two experimental setups, composed of cold and warm Rubidium atoms, respectively, which allow us to probe and compare photon correlations up to the fourth order. The former operates in the quantum regime where spontaneous emission dominates, whereas the latter exhibits a temperature-limited coherence time. While both setups present almost-chaotic light statistics, we discuss how the access to different orders of photon correlations allows one to better characterize the mechanisms responsible for deviations from those statistics.
The Siegert relation relates electric field and intensity correlations of light, under given assumptions. After a brief derivation of the relation, we present an experimental setup that can be implemented in a student laboratory: it allows measuring both field and intensity correlations at the same time, thus providing a direct test of the Siegert relation. Some experimental results are presented when the scattering medium corresponds to a cold atomic cloud. As a conclusion, we discuss typical situations where the relation fails.
In a near-field three-photon correlation measurement, we observed the third-order temporal and spatial correlation functions of chaotic thermal light in the single-photon counting regime. In the study, we found that the probability of jointly detecting three randomly radiated photons from a chaotic thermal source by three individual detectors is 666 times greater if the photodetection events fall in the coherence time and coherence area of the radiation field than if they do not. From the viewpoint of quantum mechanics, the observed phenomenon is the result of three-photon interference. By making use of this property, we measured the three-photon thermal light lensless ghost image of a double spot and achieved higher visibility compared with the two-photon thermal light ghost image.
Abstract We present an experimental technique that can accurately measure the high-order photon correlations of various light fields based on double Hanbury Brown–Twiss scheme. The system consists of four conventional binary response single-photon counting modules which are non-photon-number-resolving detectors. We theoretically analyze the effects of the experimental conditions on the high-order photon correlations of coherent, chaotic thermal, Fock and squeezed vacuum states with considering the overall efficiency and background noise. In experiment, we determine the proper resolution time from 2 9 = 512 ns to 2 11 = 2048 ns and counting rate from 10 kc s −1 to 100 kc s −1 for characterizing the exact second-, third- and fourth-order photon correlations of chaotic thermal state. At complete time delays, we also observe the third- and fourth-order photon correlations of chaotic thermal state, with the maximum high-order correlation values of 5.99 ± 0.02 and 23.9 ± 0.2 respectively, which are in good agreement with the theoretical values of 6 and 24. The demonstrated experimental technique with high accuracy is a promising tool for investigating quantum optical coherence and ghost imaging.
This thesis intends to familiarize the reader with the concepts of photon statistics and correlations in quantum optics. Developing light sources that emit quantum states is central for the realization of quantum technologies. One important step in characterizing these sources is the measurement of field fluctuations and correlations, by coincidence measurements. The expectation value of a coincidence measurement, a simultaneous measurement of two intensities (or, more general, four fields), is represented by the fourth-order correlation function. The value of the correlation function, at zero delay between the detection of two photons, reveals important properties of the state to which they belonged, for example the fluctuations of the photon number. Since predictability is important for many applications, light sources emitting single photons are also characterized by the indistinguishability of consecutively emitted photons, or of two photons from separate emitters. In paper I we investigate blinking behaviour in quantum emitters, and its effect on the interference pattern and photon statistics with photons from two separate emitters. Blinking refers to an emitters transition into a non-emitting state, and subsequent transition back to an emitting state. We show that blinking can not be treated as linear loss, when measuring the fourth-order correlation function for two emitters in a Hong-Ou-Mandel setup. In general, a measurement of the fourth-order correlation function is robust to loss, which makes it a very practical tool. However, the relation between recorded coincidence counts and the correlation function is only direct in the limit of zero detection efficiency, and depends on the detection system. In paper II, we show that by adding a variable attenuation in the beam path, we can trace back to the ''true'' value of the correlation function at zero quantum efficiency. This method improves accuracy in correlation measurements by decreasing a systematic error at the expense of an increased statistical error, which is easier to handle, extending the use of coincidence methods to classical and non-classical multi-photon states.
The use of temporal correlations in scattered photons to probe the microscopic dynamics of ultracold quantum gases has emerged as a powerful, minimally destructive approach for in situ analysis. Here, we demonstrate that temporal coherence spectroscopy can quantitatively characterize atomic motion in a magnetic trap, despite the perturbative effects of the probing light. By measuring the first-order correlation function g (1) (τττ ) of light scattered by a 87 Rb cloud confined in a quadrupole trap, we identify radiation-pressure-induced acceleration and heating as the origin of the apparent discrepancy between coherence spectra and temperatures inferred from time-of-flight measurements. A simple dynamical model incorporating these effects restores agreement between theory and experiment, establishing coherence spectroscopy as a reliable in situ probe of velocity distributions in trapped atomic ensembles. Our results pave the way for time-resolved studies of nonequilibrium dynamics and thermalization processes in confined cold gases, complementing conventional destructive imaging techniques.