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Physical Review A

Observation of collapse and revival of atomic four-wave mixing in Bose gases

Wei-Tao Wu, Zhi-Xin Duan, Sheng-Jun Yang

Published Jun 11, 2024• 4 citations
Publisher

Abstract

Atomic four-wave mixing (FWM) is an important nonlinear process in ultracold physics. Despite numerous works on atomic FWM, the phase coherence effect has not been extensively studied. Here, by preparing multiple spin-momentum modes with ultracold $^{87}\mathrm{Rb}$ atoms in a crossed dipole trap and applying an external magnetic field to regulate the atomic motions and interactions, we extensively investigate how the coherence fluctuation affects the atomic FWM process. We observe that the atomic motion and spin-exchange collision involve a periodic collapse and revival of the yield fraction of the atomic FWM. The oscillation period is mainly determined by the spin-exchange rate and thus the atomic scattering cross section. Our work demonstrates that atomic FWM can be used to probe the coherence and the atomic interactions, which should benefit various areas related to multicomponent atomic interactions and spin dynamics in the future.

DOI
10.1103/physreva.109.063316

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Atomic four-wave mixing (FWM) is an important nonlinear process in ultracold physics. Despite numerous works on atomic FWM, the phase coherence effect has not been extensively studied. Here, by preparing multiple spin-momentum modes with ultracold 87Rb^{87}\mathrm{Rb}87Rb atoms in a crossed dipole trap and applying an external magnetic field to regulate the atomic motions and interactions, we extensively investigate how the coherence fluctuation affects the atomic FWM process. We observe that the atomic motion and spin-exchange collision involve a periodic collapse and revival of the yield fraction of the atomic FWM. The oscillation period is mainly determined by the spin-exchange rate and thus the atomic scattering cross section. Our work demonstrates that atomic FWM can be used to probe the coherence and the atomic interactions, which should benefit various areas related to multicomponent atomic interactions and spin dynamics in the future.
We present an exact quantum-mechanical analysis of collinear four-wave mixing in a multicomponent Bose-Einstein condensate consisting of sodium atoms in the F=1F=1F=1 ground state. Technically, this is achieved by taking advantage of the conservation laws of the system to cast its Hamiltonian in terms of angular momentum operators. We discuss explicitly the build-up of matter-wave side modes from quantum fluctuations, as well as the correlations between these modes. We show the appearance of a strong quantum entanglement between hyperfine states. We also demonstrate that for finite atomic numbers, the system exhibits periodic collapses and revivals in the exchange of atoms between different spin states.
Abstract We describe possibilities of spontaneous, degenerate four-wave mixing (FWM) processes in spin–orbit coupled Bose–Einstein condensates. Phase matching conditions (i.e., energy and momentum conservation laws) in such systems allow one to identify four different configurations characterized by involvement of distinct spinor states in which such a process can take place. We derived these conditions from first principles and then illustrated dynamics with direct numerical simulations. We found, among others, the unique configuration, where both probe waves have smaller group velocity than pump wave and proved numerically that it can be observed experimentally under proper choice of the parameters. We also reported the case when two different FWM processes can occur simultaneously. The described resonant interactions of matter waves is expected to play an important role in the experiments of BEC with artificial gauge fields. Beams created by FWM processes are an important source of correlated particles and can be used in the experiments testing quantum properties of atomic ensembles.
We study the dynamics of spin-1 atoms in a periodic optical-lattice potential and an external magnetic field in a quantum quench scenario where we start from a superfluid ground state in a shallow lattice potential and suddenly raise the lattice depth. The time evolution of the nonequilibrium state shows collective collapse-and-revival oscillations of matter-wave coherence as well as oscillations in the spin populations. We show that the complex pattern of these two types of oscillations reveals details about the superfluid and magnetic properties of the initial many-body ground state. Furthermore, we show that the strengths of the spin-dependent and spin-independent atom-atom interactions can be deduced from the observations. The Hamiltonian that describes the physics of the final deep lattice not only contains two-body interactions but also effective multibody interactions, which arise due to virtual excitations to higher bands. We derive these effective spin-dependent three-body interaction parameters for spin-1 atoms and describe how spin mixing is affected. Spinor atoms are unique in the sense that multibody interactions are directly evident in the in situ number densities in addition to the momentum distributions. We treat both antiferromagnetic (e.g., 23{}^{23}23Na) and ferromagnetic (e.g., 87{}^{87}87Rb and 41{}^{41}41K) condensates.
We calculate the four-wave mixing (FWM) in a Bose-Einstein condensate system having multiple spin wave packets that are initially overlapping in physical space, but have nonvanishing relative momentum that causes them to recede from one another. Three receding condensate atom wave packets can result in production of a fourth wave packet by the process of FWM due to atom-atom interactions. We consider cases where the four final wave packets are composed of one, two, three, and four different internal spin components. FWM with one or two-spin state wave packets is much stronger than three- or four-spin state FWM, wherein two of the coherent moving Bose-Einstein condensate wave packets form a spin-polarization grating that rotates the spin projection of the third wave into that of the fourth diffracted wave (as opposed to the one- or two-spin state case where a regular density grating is responsible for the diffraction). Calculations of FWM for 87Rb^{87}\mathrm{Rb}87Rb and 23Na^{23}\mathrm{Na}23Na condensate systems are presented.
The advent of the laser as an intense, coherent light source gave birth to nonlinear optics, which now plays an important role in many areas of science and technology. One of the first applications of nonlinear optics was the production of coherent light of a new frequency by multi-wave mixing of several optical fields in a nonlinear medium. Until the experimental realization of Bose-Einstein Condensation (BEC) there had been no intense coherent source of matter-waves analogous to the optical laser. FEC has already been exploited to produce a matter-wave `laser' leading to the threshold of a new field of physics: nonlinear atom optics. Recently the first experiment in nonlinear atom optics was reported: the observation of coherent four wave mixing in which three sodium matter waves mix to produce a fourth. The experiment utilized light pulses to create two high-momentum wavepackets via Bragg diffraction from a stationary Bose- Einstein condensate. The high-momentum components and the remaining zero momentum condensate component interact to form a new momentum component due to the nonlinear self- interaction of the bosonic atoms. We develop a quantum mechanical description, based on the slowly-varying-envelope approximation to the time-dependent nonlinear Schrodinger equation (also called the Gross-Pitaevskii equation), to describe four-wave mixing in Bose-Einstein condensates and apply this description to understand the experimental observations and to make new predictions. We examine the role of phase-modulation, momentum and energy conservation (i.e., phase-matching), and particle number conservation in four-wave mixing of matter waves.
Bose-Einstein condensation (BEC) is a phenomenon in which identical bosons occupy the same quantum state below a certain critical temperature. A hallmark of BEC is the coherence between particles every particle shares the same quantum wavefunction and phase. This coherence has been demonstrated for the external (motional) degrees of freedom of the atomic condensates by interfering two condensates. In this thesis, the coherence is shown to extend to the internal spin degrees of freedom of a spin-1 Bose gas evidenced by the observed coherent and reversible spin-changing collisions. The observed coherent dynamics are analogous to Josephson oscillations in weakly connected superconductors and represent a type of matter-wave four-wave mixing. Control of the coherent evolution of the system using magnetic fields is also demonstrated. The studies on spinor condensates begin by creating spinor condensates directly using all-optical approaches that were first developed in our laboratory. All-optical formation of Bose-Einstein condensates (BEC) in 1D optical lattice and single focus trap geometries are developed and presented. These techniques offer considerable flexibility and speed compared to magnetic trap approaches, and the trapping potential can be essentially spin-independent and are ideally suited for studying spinor condensates. Using condensates with well-defined initial non-equilibrium spin configuration, spin mixing of F = 1 and F = 2 spinor condensates of rubidium-87 atoms confined in an optical trap is observed. The equilibrium spin configuration in the F = 1 manifold confirms that 87Rb is ferromagnetic. The coherent spinor dynamics are demonstrated by initiating spin mixing deterministically with a non-stationary spin population configuration. Finally, the interplay between the coherent spin mixing and spatial dynamics in spin-1 condensates with ferromagnetic interactions is investigated.