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arXiv:1304.7565 · Physical Review A

Dynamics of spin-1 bosons in an optical lattice: Spin mixing, quantum-phase-revival spectroscopy, and effective three-body interactions

Khan W. Mahmud, Eite Tiesinga

Published Aug 5, 2013• 41 citations
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Abstract

We study the dynamics of spin-1 atoms in a periodic optical-lattice potential and an external magnetic field in a quantum quench scenario where we start from a superfluid ground state in a shallow lattice potential and suddenly raise the lattice depth. The time evolution of the nonequilibrium state shows collective collapse-and-revival oscillations of matter-wave coherence as well as oscillations in the spin populations. We show that the complex pattern of these two types of oscillations reveals details about the superfluid and magnetic properties of the initial many-body ground state. Furthermore, we show that the strengths of the spin-dependent and spin-independent atom-atom interactions can be deduced from the observations. The Hamiltonian that describes the physics of the final deep lattice not only contains two-body interactions but also effective multibody interactions, which arise due to virtual excitations to higher bands. We derive these effective spin-dependent three-body interaction parameters for spin-1 atoms and describe how spin mixing is affected. Spinor atoms are unique in the sense that multibody interactions are directly evident in the in situ number densities in addition to the momentum distributions. We treat both antiferromagnetic (e.g., ${}^{23}$Na) and ferromagnetic (e.g., ${}^{87}$Rb and ${}^{41}$K) condensates.

DOI
10.1103/physreva.88.023602

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We study the dynamics of spin-1 atoms in a periodic optical-lattice potential and an external magnetic field in a quantum quench scenario where we start from a superfluid ground state in a shallow lattice potential and suddenly raise the lattice depth. The time evolution of the nonequilibrium state shows collective collapse-and-revival oscillations of matter-wave coherence as well as oscillations in the spin populations. We show that the complex pattern of these two types of oscillations reveals details about the superfluid and magnetic properties of the initial many-body ground state. Furthermore, we show that the strengths of the spin-dependent and spin-independent atom-atom interactions can be deduced from the observations. The Hamiltonian that describes the physics of the final deep lattice not only contains two-body interactions but also effective multibody interactions, which arise due to virtual excitations to higher bands. We derive these effective spin-dependent three-body interaction parameters for spin-1 atoms and describe how spin mixing is affected. Spinor atoms are unique in the sense that multibody interactions are directly evident in the in situ number densities in addition to the momentum distributions. We treat both antiferromagnetic (e.g., 23{}^{23}23Na) and ferromagnetic (e.g., 87{}^{87}87Rb and 41{}^{41}41K) condensates.
We study the dynamics of interacting superfluid bosons in a one-dimensional vertical optical lattice after a sudden increase of the lattice potential depth. We show that this system can be exploited to investigate the effects of strong interactions on Bloch oscillations. We perform theoretical modeling of this system, identify experimental challenges, and explore a regime of Bloch oscillations characterized by interaction-induced matter-wave collapse and revivals which modify the Bloch oscillations dynamics. In addition, we study three dephasing mechanisms: finite value of tunneling, effective three-body interactions, and a background harmonic potential. We also find that the center-of-mass motion in the presence of finite tunneling goes through collapse and revivals, giving an example of quantum transport where interaction-induced revivals are important. We quantify the effects of residual harmonic trapping on the momentum distribution dynamics and show the occurrence of an interaction-modified temporal Talbot effect. Finally, we analyze the prospects and challenges of exploiting Bloch oscillations of cold atoms in the strongly interacting regime for precision measurement of the gravitational acceleration ggg.
We present an experimental study on nonequilibrium dynamics of a spinor condensate after it is quenched across a superfluid to Mott insulator (MI) phase transition in cubic lattices. Intricate dynamics consisting of spin-mixing oscillations at multiple frequencies are observed in time evolutions of the spinor condensate localized in deep lattices after the quantum quench. Similar spin dynamics also appear after spinor gases in the MI phase are suddenly moved away from their ground states via quenching magnetic fields. We confirm these observed spectra of spin-mixing dynamics can be utilized to reveal atom number distributions of an inhomogeneous system, and to study transitions from two-body to many-body dynamics. Our data also imply the nonequilibrium dynamics depend weakly on the quench speed but strongly on the lattice potential. This enables precise measurements of the spin-dependent interaction, a key parameter determining the spinor physics.
Recent experiments have shown a remarkable number of collapse and revival oscillations of the matter-wave coherence of ultracold atoms in optical lattices [Will et al., Nature (London) 465, 197 (2010)]. Using a mean-field approximation to the Bose-Hubbard model, we show that the visibility of collapse and revival interference patterns reveals number squeezing of the initial superfluid state. To describe the dynamics, we use an effective Hamiltonian that incorporates the intrinsic two-body and induced three-body interactions, and we analyze in detail the resulting complex pattern of collapse and revival frequencies generated by virtual transitions to higher bands, as a function of lattice parameters and mean-atom number. Our work shows that a combined analysis of both the multiband, nonstationary dynamics in the final deep lattice and the number squeezing of the initial superfluid state explains important characteristics of optical lattice collapse and revival physics. Finally, by treating the two- and three-body interaction strengths and the coefficients describing the initial superposition of number states as free parameters in a fit to the experimental data, it should be possible to go beyond some of the limitations of our model and obtain insight into the breakdown of the mean-field theory for the initial state or the role of nonperturbative effects in the final-state dynamics.
Bose-Einstein condensation (BEC) is a phenomenon in which identical bosons occupy the same quantum state below a certain critical temperature. A hallmark of BEC is the coherence between particles every particle shares the same quantum wavefunction and phase. This coherence has been demonstrated for the external (motional) degrees of freedom of the atomic condensates by interfering two condensates. In this thesis, the coherence is shown to extend to the internal spin degrees of freedom of a spin-1 Bose gas evidenced by the observed coherent and reversible spin-changing collisions. The observed coherent dynamics are analogous to Josephson oscillations in weakly connected superconductors and represent a type of matter-wave four-wave mixing. Control of the coherent evolution of the system using magnetic fields is also demonstrated. The studies on spinor condensates begin by creating spinor condensates directly using all-optical approaches that were first developed in our laboratory. All-optical formation of Bose-Einstein condensates (BEC) in 1D optical lattice and single focus trap geometries are developed and presented. These techniques offer considerable flexibility and speed compared to magnetic trap approaches, and the trapping potential can be essentially spin-independent and are ideally suited for studying spinor condensates. Using condensates with well-defined initial non-equilibrium spin configuration, spin mixing of F = 1 and F = 2 spinor condensates of rubidium-87 atoms confined in an optical trap is observed. The equilibrium spin configuration in the F = 1 manifold confirms that 87Rb is ferromagnetic. The coherent spinor dynamics are demonstrated by initiating spin mixing deterministically with a non-stationary spin population configuration. Finally, the interplay between the coherent spin mixing and spatial dynamics in spin-1 condensates with ferromagnetic interactions is investigated.
Since the experimental realization of Bose-Einstein condensation in 1995, the field of ultracold atoms has expanded rapidly, and has become an important arena for exploring diverse quantum many-body physics, as highlighted by the experimental observation of quantum phase transitions in the system of bosons in a periodic potential, which is described by the Bose-Hubbard model.Recently, ultracold atoms with spin degrees of freedom are actively studied because the coupling between the internal spin degrees of freedom and the spatial degrees of freedom can give rise to novel and interesting physics.A minimal model for studying such physics is the spin-1 Bose-Hubbard model, which describes spin-1 bosons in a periodic potential.The model has a spin-dependent interaction, which can be ferromagnetic or antiferromagnetic, and it is known that although the ferromagnetic model resembles the spinless counterpart, the antiferromagnetic model exhibits totally different features, which make the model much more intensively studied compared with the ferromagnetic one.However, the presence of an external magnetic field can change the situation, because the positive quadratic Zeeman energy competes with the ferromagnetic interaction, which can give rise to rich phases.In this thesis, we explore the ground-state and nonzero-temperature phase diagrams of the spin-1 Bose-Hubbard model under an external magnetic field.To analyze the model, we use an approximation method called the decoupling approximation, or equivalently, the Gutzwiller variational ansatz.It is shown that, in addition to the Mott insulator phase, the model possesses two superfluid phases.Moreover, for large values of a spin-dependent interaction, the phase transitions between the two superfluid phases can be discontinuous.Such discontinuous phase transitions are shown to survive at nonzero but sufficiently low temperature.The discontinuous phase transitions are in clear contrast to the mean-field theory of weakly interacting spin-1 bosons without a lattice, which predicts that the corresponding phase transition is continuous, signifying the importance of the effect of strong interactions on the interplay between the spatial and spinor degrees of freedom. 4.1.2The grand Hamiltonian . . . . . . . . .
Quantum-phase collapse and revival are studied in a binary mixture of bosonic atomic species loaded in a one-dimensional optical lattice. Oscillations in the quasimomentum distribution are usually observed after a sudden quench of the lattice parameters from the superfluid regime to the Mott-insulator regime. The influence of one species dynamics on the collapse and revival oscillations in the quasimomentum distribution of the second species is examined. The nontrivial dependencies on the interspecies and intraspecies interactions are illustrated distinguishing between the zero-tunneling and nonzero-tunneling cases.