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arXiv:1905.08738 · Physical Review Letters

Quantum Quench and Nonequilibrium Dynamics in Lattice-Confined Spinor Condensates

Z. Chen, Tao Tang, Jared Austin, Zachary Shaw, Lichao Zhao, Yingmei Liu

Published Sep 10, 2019• 35 citations
arXivHTMLPDF

Abstract

We present an experimental study on nonequilibrium dynamics of a spinor condensate after it is quenched across a superfluid to Mott insulator (MI) phase transition in cubic lattices. Intricate dynamics consisting of spin-mixing oscillations at multiple frequencies are observed in time evolutions of the spinor condensate localized in deep lattices after the quantum quench. Similar spin dynamics also appear after spinor gases in the MI phase are suddenly moved away from their ground states via quenching magnetic fields. We confirm these observed spectra of spin-mixing dynamics can be utilized to reveal atom number distributions of an inhomogeneous system, and to study transitions from two-body to many-body dynamics. Our data also imply the nonequilibrium dynamics depend weakly on the quench speed but strongly on the lattice potential. This enables precise measurements of the spin-dependent interaction, a key parameter determining the spinor physics.

DOI
10.1103/physrevlett.123.113002

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We present an experimental study on nonequilibrium dynamics of a spinor condensate after it is quenched across a superfluid to Mott insulator (MI) phase transition in cubic lattices. Intricate dynamics consisting of spin-mixing oscillations at multiple frequencies are observed in time evolutions of the spinor condensate localized in deep lattices after the quantum quench. Similar spin dynamics also appear after spinor gases in the MI phase are suddenly moved away from their ground states via quenching magnetic fields. We confirm these observed spectra of spin-mixing dynamics can be utilized to reveal atom number distributions of an inhomogeneous system, and to study transitions from two-body to many-body dynamics. Our data also imply the nonequilibrium dynamics depend weakly on the quench speed but strongly on the lattice potential. This enables precise measurements of the spin-dependent interaction, a key parameter determining the spinor physics.
We study the dynamics of spin-1 atoms in a periodic optical-lattice potential and an external magnetic field in a quantum quench scenario where we start from a superfluid ground state in a shallow lattice potential and suddenly raise the lattice depth. The time evolution of the nonequilibrium state shows collective collapse-and-revival oscillations of matter-wave coherence as well as oscillations in the spin populations. We show that the complex pattern of these two types of oscillations reveals details about the superfluid and magnetic properties of the initial many-body ground state. Furthermore, we show that the strengths of the spin-dependent and spin-independent atom-atom interactions can be deduced from the observations. The Hamiltonian that describes the physics of the final deep lattice not only contains two-body interactions but also effective multibody interactions, which arise due to virtual excitations to higher bands. We derive these effective spin-dependent three-body interaction parameters for spin-1 atoms and describe how spin mixing is affected. Spinor atoms are unique in the sense that multibody interactions are directly evident in the in situ number densities in addition to the momentum distributions. We treat both antiferromagnetic (e.g., 23{}^{23}23Na) and ferromagnetic (e.g., 87{}^{87}87Rb and 41{}^{41}41K) condensates.
Quantum simulators are easily controllable quantum systems that allow us to physically model the behavior of more complex systems, that are intractable with even the most advanced supercomputers, to gain insight into their behavior. Using lattice confined spinor Bose-Einstein condensates (BEC) as quantum simulators, we explore the quantum critical dynamics of the superfluid to Mott insulator phase transition in a three-dimensional cubic optical lattice. Our observations reveal that, in a quantum version of the Kibble-Zurek mechanism, the dynamics can be frozen by a sufficiently quick ramp across the transition. Additionally, we utilize discrete energy signatures in nonequilibrium spin mixing dynamics generated by atoms that are tightly confined to single lattice sites after a quench across this transition to understand the spatial dynamics of a BEC during this transition. This "indirect microscopy" method is required to determine the spatial distribution because achieving single lattice site resolved imaging of three dimensional lattice confined quantum gases remains experimentally challenging even with advanced quantum gas microscopy methods. The observed number distributions additionally demonstrate that it may be possible to design lattice ramp sequences to manipulate the distribution of atoms to enhance desired effects.
This thesis discusses non-equilibrium phenomena in antiferromagnetic spinor quantum gases. We investigate, both experimentally and theoretically, the quench dynamics of antiferromagnetic spinor Bose-Einstein condensates in the vicinity of a zero temperature quantum phase transition. A microwave dressing field was used as a novel tool to access the polar to antiferrmagnetic quantum phase transition at the quadratic Zeeman shift, q=0. By performing instantaneous quenches across the phase transition,a dynamical instability was induced in the atomic cloud. This lead to pair formation and rapid amplification of spin +/-1 atoms through spin-mixing collisions. The spatial ordering kinetics in the vicinity of the phase transition was quantified by performing the local spin measurement. The coarsening dynamics was observed for the instability for q < 0, as it nucleated small domains that grew to the axial size of the cloud. Rich nonequilibrium behavior was observed in the form of growth and decay of both nematic and magnetic spin waves, following the quench. The spatiotemporal evolution was characterized through two particle correlations between atoms in each pair of spin states, which revealed dramatic differences between the dynamics of the spin correlations and those of the spin populations. \nFinally, we demonstrate the remarkable influence of linear Zeeman term on non-equilibrium dynamics of spinor Bose-Einstein condensates. We show that contrary to prior understanding magnetic field gradient actually suppresses the tendency of spin 0 state to separate into spin +/-1 state. This reconciles the Bogoliubov discrepancies and leads to a dramatic sharpening of the transition point, resulting in a resolution at the 1 Hz level. Our results point to the use of dynamics, rather than equilibrium quantities for high precision measurements of phase transitions in quantum gases.
We present an experimental study demonstrating the manipulation of atom-number distributions of spinor gases after nonequilibrium quantum quenches across superfluid to Mott-insulator phase transitions in cubic optical lattices. Our data indicate that atom distributions in individual Mott lobes can be tuned by properly designing quantum quench sequences, which suggests methods of maximizing the fraction of atoms in Mott lobes of even occupation numbers and has applications in attaining different quantum magnetic phases including massively entangled states. Spatial distributions of gases in three-dimensional lattices are derived from the observed number distributions, which reveal complex spatial dynamics during the quantum quenches. Qualitative agreements are also found between our experimental data and numerical simulations based on time-dependent Gutzwiller approximations in two-dimensional systems.
We observe evidence of first-order superfluid-to-Mott-insulator quantum phase transitions in a lattice-confined antiferromagnetic spinor Bose-Einstein condensate. The observed signatures include the hysteresis effect, significant heatings across the phase transitions, and changes in spin populations due to the formation of spin singlets in the Mott-insulator phase. The nature of the phase transitions is found to strongly depend on the ratio of the quadratic Zeeman energy to the spin-dependent interaction. Our observations are qualitatively understood by the mean field theory and suggest tuning the quadratic Zeeman energy is a new approach to realize superfluid-to-Mott-insulator phase transitions.
We present the experimental detection of coherent three-body interactions, often masked by stronger two-body effects, through nonequilibrium spin dynamics induced by controllably quenching lattice-confined spinor gases. Three-body interactions are characterized through both real-time and frequency domain analyses of the observed dynamics. Our results, well-described by an extended Bose-Hubbard model, further demonstrate the importance of three-body interactions for correctly determining atom distributions in lattice systems, which has applications in quantum sensing via spin singlets. The techniques demonstrated in this work can be directly applied to other atomic species, offering a promising avenue for future studies of higher-body interactions with broad relevance to strongly-interacting quantum systems.