The performance of superconducting quantum circuits for quantum computing has advanced tremendously in recent decades; however, a comprehensive understanding of relaxation mechanisms does not yet exist. In this work, we utilize a multimode approach to characterizing energy losses in superconducting quantum circuits, with the goals of predicting device performance and improving coherence through materials, process, and circuit design optimization. Using this approach, we measure significant reductions in surface and bulk dielectric losses by employing a tantalum-based materials platform and annealed sapphire substrates. With this knowledge we predict the relaxation times of aluminum- and tantalum-based transmon qubits, and find that they are consistent with experimental results. We additionally optimize device geometry to maximize coherence within a coaxial tunnel architecture, and realize on-chip quantum memories with single-photon Ramsey times of 2.0 - 2.7 ms, limited by their energy relaxation times of 1.0 - 1.4 ms. These results demonstrate an advancement towards a more modular and compact coaxial circuit architecture for bosonic qubits with reproducibly high coherence.
The performance of superconducting quantum circuits for quantum computing has advanced tremendously in recent decades; however, a comprehensive understanding of relaxation mechanisms does not yet exist. In this work, we utilize a multimode approach to characterizing energy losses in superconducting quantum circuits, with the goals of predicting device performance and improving coherence through materials, process, and circuit design optimization. Using this approach, we measure significant reductions in surface and bulk dielectric losses by employing a tantalum-based materials platform and annealed sapphire substrates. With this knowledge we predict and experimentally verify the relaxation times of aluminum- and tantalum-based transmon qubits. We additionally optimize device geometry to maximize coherence within a coaxial tunnel architecture, and realize on-chip quantum memories with single-photon Ramsey times of 2.0$-
2.7ms,limitedbytheirenergyrelaxationtimesof1.0-$1.4 ms. To our knowledge this is the highest coherence achieved in an on-chip quantum memory, and demonstrates an advancement towards a more modular and compact coaxial circuit architecture for bosonic qubits with reproducibly high coherence.
The superconducting transmon qubit is a leading platform for quantum computing and quantum science. Building large, useful quantum systems based on transmon qubits will require significant improvements in qubit relaxation and coherence times, which are orders of magnitude shorter than limits imposed by bulk properties of the constituent materials. This indicates that relaxation likely originates from uncontrolled surfaces, interfaces, and contaminants. Previous efforts to improve qubit lifetimes have focused primarily on designs that minimize contributions from surfaces. However, significant improvements in the lifetime of two-dimensional transmon qubits have remained elusive for several years. Here, we fabricate two-dimensional transmon qubits that have both lifetimes and coherence times with dynamical decoupling exceeding 0.3 milliseconds by replacing niobium with tantalum in the device. We have observed increased lifetimes for seventeen devices, indicating that these material improvements are robust, paving the way for higher gate fidelities in multi-qubit processors.
Superconducting qubits are a leading system for realizing large-scale quantum processors, but overall gate fidelities suffer from coherence times limited by microwave dielectric loss.Recently discovered tantalum-based qubits exhibit record lifetimes exceeding 0.3 ms.Here, we perform systematic, detailed measurements of superconducting tantalum resonators in order to disentangle sources of loss that limit state-of-the-art tantalum devices.By studying the dependence of loss on temperature, microwave photon number, and device geometry, we quantify materials-related losses and observe that the losses are dominated by several types of saturable two-level systems (TLSs), with evidence that both surface and bulk related TLSs contribute to loss.Moreover, we show that surface TLSs can be altered with chemical processing.With four different surface conditions, we quantitatively extract the linear absorption associated with different surface TLS sources.Finally, we quantify the impact of the chemical processing at singlephoton powers, the relevant conditions for qubit device performance.In this regime, we measure resonators with internal quality factors ranging from 5 to 15 × 10 6 , comparable to the best qubits reported.In these devices, the surface and bulk TLS contributions to loss are comparable, showing that systematic improvements in materials on both fronts are necessary to improve qubit coherence further.
We assess independently the impact of high-temperature substrate annealing and metal deposition conditions on the coherence of transmon qubits in the standard 2D circuit-QED architecture. We restrict our study to devices made with aluminum interdigital capacitors on sapphire substrates. We record more than an order-of-magnitude improvement in the relaxation time of devices made with an annealed substrate, independent of whether a conventional evaporator or molecular beam epitaxy chamber was used to deposit the aluminum. We also infer similar levels of flux noise and photon shot noise through dephasing measurements on these devices. Our results indicate that substrate annealing plays a primary role in fabricating low-loss qubits, consistent with the hypothesis that substrate-air and substrate-metal interfaces are essential factors limiting the qubit lifetimes in superconducting circuits.
Abstract Superconducting quantum circuits are a leading platform for quantum-information processing, but their development requires expertise spanning device design, microfabrication, cryogenic operation, microwave control, and quantum characterization. In this work, we report the realization of a flux-tunable superconducting transmon platform and present an integrated workflow encompassing design, fabrication, measurement, and numerical modeling. The device consists of an
Al/AlOx/Al transmon coupled to a three-dimensional microwave cavity operating in the circuit quantum electrodynamics (cQED) dispersive regime. Two-tone spectroscopy reveals a fundamental transition frequency of
ω01=5.0122 GHz and an anharmonicity of
α/2π=−202.4 MHz , corresponding to
EJ/EC≈82.9 . Flux spectroscopy yields a cavity-qubit coupling strength of
g/2π=260 MHz , while the cavity linewidth gives a loaded quality factor of
QL=6127 and a Purcell limit of
T1Purcell≈82 μs . Time-domain measurements yield coherence times of
T1=17.4 μs and
T2∗=5.8 μs . To investigate coherence and dissipation in the device, the experimental observations are analyzed within a Lindblad master-equation framework describing cavity photon loss and thermal excitation, qubit energy relaxation, and pure dephasing processes. Using a set of experimentally extracted parameters, the model reproduces the measured spectroscopic and time-domain observables, providing a quantitative description of the open-system dynamics of the transmon-cavity platform. The analysis shows that the measured coherence is primarily limited by pure dephasing and energy-relaxation processes, whereas thermal excitation plays a minor role under the experimental conditions. Inspired by the broader framework of quantum dissipation in macroscopic quantum systems pioneered by Caldeira and collaborators, this approach enables a quantitative analysis of relaxation and dephasing processes in superconducting quantum circuits. Beyond the characterization of a single device, the present work demonstrates the establishment of the expertise, infrastructure, and experimental workflow required for the design, fabrication, measurement, and modeling of superconducting quantum circuits, contributing to the development of quantum technologies in Brazil and related applications.
A promising way to store quantum information is by encoding it in the bosonic excitations of microwave resonators. This provides for long coherence times, low dephasing rates, as well as a hardware-efficient approach to quantum error correction. There are two main methods used to make superconducting microwave resonators: by traditionally machining them out of bulk material and by lithographically fabricating them on a chip in thin film. 3D resonators have few loss channels and larger mode volumes, and therefore smaller participations in the lossy parts, but it can be challenging to achieve high material quality. On-chip resonators can use low-loss thin films, but they confine the field more tightly, resulting in higher participations and additional loss channels from the dielectric substrate. In this work, we present a design in which a dielectric scaffold supports a thin-film conductor within a 3D package, thus combining the low surface participations of bulk-machined cavities with high quality and control over materials of thin-film circuits. By incorporating a separate chip containing a transmon qubit, we realize a quantum memory and measure single-photon lifetimes in excess of a millisecond. This hybrid 3D architecture has several advantages for scaling as it relaxes the importance of the package and permits modular construction with separately replaceable qubit and resonator devices.