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Opto-Electronic Science

High-intensity spatial-mode steerable frequency up-converter toward on-chip integration

Haizhou Huang, Huaixi Chen, Huagang Liu, Zhi Zhang, Xinkai Feng, Jiaying Chen, Hongchun Wu, Jing Deng, Wanguo Liang, Wenxiong Lin

Published Jan 1, 2024• 12 citations
Publisher

Abstract

Integrated photonic devices are essential for on-chip optical communication, optical-electronic systems, and quantum information sciences. To develop a high-fidelity interface between photonics in various frequency domains without disturbing their quantum properties, nonlinear frequency conversion, typically steered with the quadratic (χ2) process, should be considered. Furthermore, another degree of freedom in steering the spatial modes during the χ2 process, with unprecedent mode intensity is proposed here by modulating the lithium niobate (LN) waveguide-based inter-mode quasi-phase-matching conditions with both temperature and wavelength parameters. Under high incident light intensities (25 and 27.8 dBm for the pump and the signal lights, respectively), mode conversion at the sum-frequency wavelength with sufficient high output power (−7 – 8 dBm) among the TM01, TM10, and TM00 modes is realized automatically with characterized broad temperature (ΔT ≥ 8 °C) and wavelength windows (Δλ ≥ 1 nm), avoiding the previous efforts in carefully preparing the signal or pump modes. The results prove that high-intensity spatial modes can be prepared at arbitrary transparent wavelength of the χ2 media toward on-chip integration, which facilitates the development of chip-based communication and quantum information systems because spatial correlations can be applied to generate hyperentangled states and provide additional robustness in quantum error correction with the extended Hilbert space.

DOI
10.29026/oes.2024.230036

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Integrated photonic devices are essential for on-chip optical communication, optical-electronic systems, and quantum information sciences. To develop a high-fidelity interface between photonics in various frequency domains without disturbing their quantum properties, nonlinear frequency conversion, typically steered with the quadratic (χ2) process, should be considered. Furthermore, another degree of freedom in steering the spatial modes during the χ2 process, with unprecedent mode intensity is proposed here by modulating the lithium niobate (LN) waveguide-based inter-mode quasi-phase-matching conditions with both temperature and wavelength parameters. Under high incident light intensities (25 and 27.8 dBm for the pump and the signal lights, respectively), mode conversion at the sum-frequency wavelength with sufficient high output power (−7 – 8 dBm) among the TM01, TM10, and TM00 modes is realized automatically with characterized broad temperature (ΔT ≥ 8 °C) and wavelength windows (Δλ ≥ 1 nm), avoiding the previous efforts in carefully preparing the signal or pump modes. The results prove that high-intensity spatial modes can be prepared at arbitrary transparent wavelength of the χ2 media toward on-chip integration, which facilitates the development of chip-based communication and quantum information systems because spatial correlations can be applied to generate hyperentangled states and provide additional robustness in quantum error correction with the extended Hilbert space.
Spatial-mode-selective frequency conversion is potentially useful for both classical and quantum communication applications. By a judicious choice of the quasi-phase-matching period in a Kai(2) multimode waveguide, such conversion can be achieved with high efficiency (close to 100%) and with low crosstalk (< -20 dB). For space-division multiplexing application with classical signals, where each spatial mode represents a separate signal channel, the selective conversion of a spatial mode without disrupting other signal modes can be used for reconfigurable spatial-mode de-multiplexing. This classical de-multiplexing capability can be also extended to the quantum regime, where the quantum state of the signal is preserved during frequency conversion, owing to the unitary nature of the sum-frequency generation (SFG) process. Building upon our previous experimental demonstration of the classical spatial-mode-selective frequency up-conversion in a two-mode PPLN waveguide, here we report the extension of this work into the single-photon-level regime. The signal (1540 nm) in either a single mode (TM00 or TM01) or a superimposition mode (TM00+TM01, TM00+iTM01) of the waveguide is selectively up-converted into TM01 SFG mode, by interacting with an appropriate pump mode (1560 nm). An accurate measurement of the single-photon-level SFG signals requires thorough filtering of the unwanted photons contributed by the second harmonic of the pump, residual pump noise extending to the signal band, and the Raman noise generated in the waveguide. We have investigated these unwanted photon sources and suppressed them by a combination of thin-film-interference and volume-Bragg-grating filters. Resulting single-photon-counting measurements show >70% internal conversion efficiency, better than -12dB crosstalk, and >100 ratio of the signal to background photon counts for all selected modes and mode superpositions.
Nonlinear wavelength conversion is essential for many classical and quantum pho-tonic applications. The underlying second-order nonlinear optical processes, however, generally exhibit limited spectral bandwidths that impact their application potential. Here we use a high-Q X-cut lithium niobate microdisk resonator to demonstrate both second-harmonic generation and spontaneous parametric down-conversion on chip. In particular, our lithium niobate microresonator, with its wide-range cyclic phase matching and rich optical mode structures, is able to achieve ultra-broadband spontaneous parametric down-conversion, with a bandwidth over 400 nm, inferred from recorded spectra of the down-converted photons. The produced biphoton pairs exhibit strong temporal correlation, with a coincidence-to-accidental ratio measured to be 43.1. Our device is promising for integrated quantum photonics where optical frequency could be used as a degree of freedom for signal processing.
On-chip quantum information network requires qubit transfer between different wavelengths while preserving quantum coherence and entanglement, which requires the availability of broadband upconversion. Herein, we demonstrate a mode-hybridization-based broadband nonlinear frequency conversion on X-cut thin film lithium niobate. With the spontaneous quasi-phase matching and quasi-group-velocity matching being simultaneously satisfied, broadband second-harmonic generation with a 3-dB bandwidth up to 13 nm has been achieved in a micro-racetrack resonator. The same mechanism can work on the frequency conversion of the ultrashort pulse in the bent waveguide structure. This work will be beneficial to on-chip tunable frequency conversion and quantum light source generation on integrated photonic platforms and further enable on-chip large-capacity multiplexing, multichannel optical information processing, and large quantum information networks.
On-chip quantum information network requires qubit transfer between different wavelengths while preserving quantum coherence and entanglement, which needs broadband up-conversion available. Herein, we demonstrate a mode-hybridization based broadband nonlinear frequency conversion on X-cut thin film lithium niobate. With the spontaneous quasi-phase matching and quasi groupvelocity matching being simultaneously satisfied, broadband second harmonic generation with a 3-dB bandwidth up to 13 nm has been achieved in a micro-racetrack resonator. The same mechanism can work on the frequency conversion of the ultra-short pulse in the bent waveguide structure. This work will be beneficial to on-chip tunable frequency conversion and quantum light source generation on integrated photonic platforms, and further enable on-chip large-capacity multiplexing, multichannel optical information processing, and large quantum information networks.
Chip-integrated nonlinear photonics holds the key for advanced optical information processing with superior performance and novel functionalities. Here, we present an optimally mode-matched, periodically poled lithium niobate nanowaveguide for efficient parametric frequency conversions on chip. Using a 4-mm nanowaveguide with subwavelength mode confinement, we demonstrate second harmonic generation with efficiency over 2200% W −1 c m −2, and broadband difference frequency generation over a 4.3-THz spectral span. These allow us to generate correlated photon pairs over multiple frequency channels via spontaneous parametric down conversion, all in their fundamental spatial modes, with a coincidence to accidental ratio as high as 600. The high efficiency and dense integrability of the present chip devices may pave a viable route to scalable nonlinear applications in both classical and quantum domains.
Within the last decade, thin-film lithium niobate (TFLN) has emerged as a leading integrated photonics platform with immediate applications in classical communications. Concurrently, TFLN components tailored to the requirements of photonic quantum information processing have also garnered considerable interest. Chief among these is the quasi-phase matched (QPM) nonlinear frequency mixer—implemented via periodic domain inversion in ferroelectric lithium niobate—which can be used to generate photon pairs, squeezed states of light, and to perform single photon frequency conversion. Here, we demonstrate progress towards realizing a spectrally separable photon pair source in lithium niobate via waveguide dispersion engineering—a technique uniquely enabled by sub-wavelength optical mode confinement in the thin-film platform. Subsequently, we design optimize a scalable fabrication process to produce QPM TFLN devices for applications that require strict adherence to a specified operating wavelength, such as quantum frequency conversion in a quantum communications network. Finally, we explore how high-performance electro-optic devices can be combined with these nonlinear optical devices to realize a multi-functional platform in which quantum states of light can be generated and manipulated within a single, compact photonic integrated circuit.