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Photonics

Towards a Lithium Niobate Photonic Integrated Circuit for Quantum Sensing Applications

Jessica César-Cuello, Isabel Carnoto Amat, Luis Enrique García-Muñoz, Guillermo Carpintero

Published Mar 6, 2024• 4 citations
Publisher

Abstract

Quantum transducers are key components for hybrid quantum networks, enabling the transfer of quantum states between microwave and optical photons. In the quantum community, many efforts have focused on creating and verifying the entanglement between microwave and optical fields in systems that typically operate at temperatures in the millikelvin range. Our goal is to develop an integrated microwave optical entanglement device based on a lithium niobate whispering gallery mode resonator (WGMR). To investigate the feasibility of developing such an integrated device, first, a passive photonic integrated circuit (PIC) was designed, fabricated, and characterized. The PIC was developed on a thin-film lithium niobate (TFLN) on an insulator platform, and it includes eight ring resonators and four asymmetric Mach–Zehnder interferometers. This paper presents the design and operational principles of the integrated device for microwave–optical entanglement, as well as the results of the characterization of the passive PIC.

DOI
10.3390/photonics11030239

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Quantum transducers are key components for hybrid quantum networks, enabling the transfer of quantum states between microwave and optical photons. In the quantum community, many efforts have focused on creating and verifying the entanglement between microwave and optical fields in systems that typically operate at temperatures in the millikelvin range. Our goal is to develop an integrated microwave optical entanglement device based on a lithium niobate whispering gallery mode resonator (WGMR). To investigate the feasibility of developing such an integrated device, first, a passive photonic integrated circuit (PIC) was designed, fabricated, and characterized. The PIC was developed on a thin-film lithium niobate (TFLN) on an insulator platform, and it includes eight ring resonators and four asymmetric Mach–Zehnder interferometers. This paper presents the design and operational principles of the integrated device for microwave–optical entanglement, as well as the results of the characterization of the passive PIC.
Quantum photonics has advanced rapidly and become a leading approach for developing a broad range of quantum technologies, including quantum communications, quantum information processing, quantum computing, and quantum sensing. Besides, the emerging photonic integrated circuits (PIC) technology has been widely used to implement versatile optical elements advantageous for different quantum applications. For example, PIC-based devices have functioned as building blocks, such as photonic qubit sources, linear optical circuits, modulators, and even single-photon detectors, for realizing highly integrated, large-scale quantum computing schemes. In such a powerful quantum photonic integrated circuits (QPIC) scheme, the creation, manipulation, and testing of quantum entanglement states from the generated qubits via a reconfigurable photonic circuitry are essential. Though the state-of-the-art PIC technology is established based on Si photonics due to its widely mature nanophotonic circuit (waveguide) fabrication technology supported by the existing immense semiconductor industry, Si-based PIC has limitations in implementing efficient and fast active elements that usually demand a quadratic nonlinearity. Lithium niobate (LN), renowned as “the silicon of photonics”, has long been a popular material widely used in integrated-optical and nonlinear-optical applications. A great variety of passive and active photonic elements have been realized in the LN platform. Recently, a novel material based on high-quality single-crystalline films of LN, known as thin-film LN on insulator (LNOI), has been developed and has soon drawn enormous attention for its greatly promising ability to realize nanoscale PIC/QPIC in this iconic optical material platform. In this presentation, we report our recent studies on several key LN PIC building blocks for developing novel quantum photonic sources and circuits, including highly integrated photonic-circuit periodically poled lithium niobate (PPLN) chips for photon-pair generation and manipulation, for high-dimensional frequency-entangled qudit production, for time-frequency grid-state generation, for continuous-variable squeezed vacuum state generation, and their potential applications to quantum computing/communication/sensing technology. Besides, a PP-LNOI electro-optic (EO) polarization mode converter (PMC) useful for demonstrating fast control of quantum polarization states and other LNOI circuit elements as QPIC building blocks will also be presented.
Photonic integrated circuits operating at cryogenic temperatures are necessary for many quantum technologies such as quantum transduction, integrated single-photon emitters and detectors, as well as deep-space communication and sensing devices. Thin-film lithium niobate (TFLN) is an emerging platform that is a strong candidate for fully integrated quantum photonics, offering low loss, fast electro-optic reconfigurability, nonlinear quantum light sources, and the ability to host quantum emitters and single-photon detectors. To interface TFLN with technologies that require cryogenic operation, like superconducting single-photon detectors, microwave-to-optical transducers, and solid-state quantum emitters, it is important to study its optical and electrical properties from room temperature down to cryogenic temperatures. Here, we investigate linear and nonlinear photonic devices, including racetrack resonators, Mach-Zehnder modulators and periodically poled waveguides in TFLN using a cryogenic fiber probe station with full temperature control down to 5 K. We quantify a shift in resonances, a 22% increase in electro-optic modulator half-wave voltage, a blue shift of 18 nm for Type-0 phase-matching as well as a red shift of 64 nm for Type-II phase-matching as the sample temperature decreases. Our study of nonlinear processes in a cryogenic environment will contribute towards developing novel devices for inter-platform quantum information processing, secure communication, and enhanced sensing.
Integrated thin-film lithium niobate (TFLN) photonics has emerged as a powerful platform for quantum information science, offering its outstanding nonlinear, electro-optic (EO), and integration capabilities. In this review, we present the latest advances in TFLN-based integrated photonics tailored to quantum technologies. We first explore state-of-the-art quantum light sources realized in both straight waveguide and resonator configuration, including high-brightness photon pair generations, squeezed light, and versatile entanglement schemes. Next, we detail progress in integrated photonic processors, with a focus on programmable interferometric networks, ultrafast EO modulators, and essential passive components for photonic qubit processing. We then address critical challenges in optical interfacing and detection technologies, discussing recent innovations in low-loss fiber-to-chip and grating coupler designs, as well as the integration of on-chip single photon detectors. This review provides a forward-looking perspective on scalable quantum photonic systems that could underpin future advances in quantum communication, computing, and sensing.
Abstract Entanglement is central to quantum technologies such as cryptography, sensing, and computing. Photon pairs generated via nonlinear optical processes are excellent for preparing entangled states due to their long coherence times and compatibility with fiber optic networks. Steady progress in nanofabrication has positioned lithium niobate-on-insulator (LNOI) as a leading platform for monolithic integration of photon pair sources into optical circuits, leveraging its strong second-order nonlinearity. Here, we present a reconfigurable photonic integrated circuit on LNOI, which combines two on-chip photon pair sources with programmable interferometers, enabling the generation of entangled states. The photon pair sources achieve a source brightness of 26 MHz nm −1 mW −1 while maintaining a coincidence-to-accidental ratio above 100. We successfully interfere the two sources with 99.0 ± 0.7% visibility, demonstrating the indistinguishability required for producing entanglement on-chip. We show the preparation of any of the maximally entangled Bell states with fidelity above 90% verified by quantum state tomography. These results establish LNOI as a compelling, scalable platform to explore integrated quantum photonic technologies enabled by high-brightness sources of entangled quantum states.
Quantum networks of superconducting qubits linked by optical channels could leverage both the quantum information processing capabilities of superconducting circuits and the long communication distances provided by optical photons. Such networks would require high efficiency, low noise, and wide bandwidth transducers between microwave and optical frequencies. Transducers based on the Pockels electro-optic (EO) effect are particularly promising in this application for their direct conversion mechanism and potential for strong performance. EO transducers could also be used for sensitive optical modulators and low-noise detection of microwave and millimeter-wave signals. This dissertation presents recent work to create cavity EO transducers in thin-film lithium niobate, an integrated photonics platform that provides low optical loss and strong EO coupling. I first describe the theory of cavity electro-optics and how it can be used to generate high-efficiency transduction between microwave and optical fields. An initial device is presented and characterized, demonstrating per-photon on-chip transduction efficiencies of up to (2.7 ± 0.3) × 10^−5. A key benefit of the device described here, which is based on photonic molecule modes, is the ability to use a static electro-optic bias to trim the transducer into resonance. However, we find the migration of free carriers in thin-film lithium niobate reduces the EO response of the device to static fields, making such trimming ineffective. This carrier migration is a key challenge for enabling the promise of low-power electro-optics provided by thin-film lithium niobate devices. I characterize the low-frequency electro-optic response, which suggests that conduction occurs on the etched surface of lithium niobate. I show how this conduction can be reduced – and low-frequency EO performance improved – by changing the electrode design and annealing the devices. Following this, I describe the design and initial characterization of an improved transducer device. Finally, I describe a scheme by which even relatively low-efficiency transducers could be used to generate remote entanglement using an optically heralding scheme. Demonstration of such a system appears possible with current devices, suggesting that small opticallymediated quantum networks of superconducting qubits may be feasible soon.
Efficient and stable microwave-optical transduction is a key enabling technology for distributed superconducting quantum computing and heterogeneous quantum networks. Electro-optic transducers based on thin-film lithium niobate (TFLN) have shown strong promise, but demonstrations to date have been limited by various factors such as low frequency bias drift, low efficiency, fabrication complexity, and scalability. Here we demonstrate the first integrated electro-optic microwave-optical transducers realized in thin-film lithium tantalate (TFLT), a material platform offering Pockels nonlinearity comparable to TFLN together with improved bias stability and high-power handling. We fabricate superconducting microwave resonators coupled to tunable photonic-molecule optical resonators using wafer-scale deep ultraviolet lithography, offering high-throughput production of hundreds of devices per wafer. Across six devices we observe coherent bidirectional conversion between C-band optical photons and 4.9-5.5 GHz microwave photons, with measured on-chip efficiencies and inferred single-photon coupling rates g_0/2π ~ 1 kHz consistent with theory. Continuous operation over multiple days is achieved using a static bias field with minimal feedback, demonstrating a major operational advantage. We further characterize optical loss statistics, microwave resonator performance, and optically induced added noise under pulsed pumping, finding less than one added photon for 100 microsecond pulses at the highest measured efficiencies. These results establish TFLT as a scalable and robust electro-optic platform for future quantum interconnects and modular quantum processors.