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Physical Review A

Experimental verification of many-body entanglement using thermodynamic quantities

Jitendra A. Joshi, Mir Alimuddin, T. S. Mahesh, Manik Banik

Published Feb 29, 2024• 9 citations
Publisher

Abstract

In this study, the authors introduce entanglement certification criteria which can be conveniently confirmed by measuring specific thermodynamic quantities. To illustrate the effectiveness of this approach, the authors conduct a proof-of-concept experiment utilizing nuclear spin registers containing up to 10 qubits, employing the nuclear magnetic resonance architecture.

DOI
10.1103/physreva.109.l020403

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In this study, the authors introduce entanglement certification criteria which can be conveniently confirmed by measuring specific thermodynamic quantities. To illustrate the effectiveness of this approach, the authors conduct a proof-of-concept experiment utilizing nuclear spin registers containing up to 10 qubits, employing the nuclear magnetic resonance architecture.
The phenomenon of quantum entanglement underlies several important protocols that enable emerging quantum technologies. Entangled states, however, are extremely delicate and often get perturbed by tiny fluctuations in their external environment. Certification of entanglement is therefore immensely crucial for the successful implementation of protocols involving this resource. In this work, we propose a set of entanglement criteria for multi-qubit systems that can be easily verified by measuring certain thermodynamic quantities. In particular, the criteria depend on the difference in optimal global and local works extractable from an isolated quantum system under global and local interactions, respectively. As a proof of principle, we demonstrate the proposed scheme on nuclear spin registers of up to 10 qubits using the Nuclear Magnetic Resonance architecture. We prepare noisy Bell-diagonal state and noisy Greenberger-Horne-Zeilinger class of states in star-topology systems and certify their entanglement through our thermodynamic criteria. Along the same line, we also propose an entanglement certification scheme in many-body systems when only partial or even no knowledge about the state is available.
We employ a nuclear magnetic resonance (NMR) quantum information processor to simulate the ground state of an XXZ spin chain and measure its NMR analog of entanglement, or pseudoentanglement. The observed pseudoentanglement for a small-size system already displays a singularity, a signature which is qualitatively similar to that in the thermodynamical limit across quantum phase transitions, including an infinite-order critical point. The experimental results illustrate a successful approach to investigate quantum correlations in many-body systems using quantum simulators.
In this work, we have been working on the concept of quantum entanglement. At first, we studied the theory of entanglement in its characterization and measurement, introducing a new scheme for detection of entanglement. The new approach links molecular-spin entities involving nuclear spins to quantum computing as more appropriate physical systems of interest. Then, we continued with the realization of entanglement in experiments. NMR has been the first choice due to its well approved advantages for quantum computing. NMR, however, has not been an appropriate system for demonstrating entangled states. Through a mathematical proof, NMR with low spin polarization has been invalidated for true implementations of non-local quantum algorithms, particularly supserdense coding. The point is that high spin polarization is inevitably required to acquire entanglement while in the current NMR it has been a formidable task to get highly polarized nuclear spins. In order to acquire high spin polarization, introducing electron spins can be much effective because of its three-order-of-magnitude larger gyromagnetic ratio compared to nuclear spins. Electron Nuclear DOuble Resonance (ENDOR) is spin manipulation technology that enables us to deal with both electron and nuclear spins. Thus, in this context, it can be more appropriate device for quantum computing. We emphasize that (pseudo)entanglement and interconversion between the entangled states have been realized with ENDOR on extremely stable organic molecular-spin entities. The required experimental conditions to obtain true quantum entanglement are also discussed. The appropriate entanglement witness for the corresponding ensemble quantum computing is introduced and examined.
We report the implementation of an entanglement transfer on a four-qubit liquid-state nuclear-magnetic resonance quantum information processor. This consists of creating an (pseudopure) entangled state among two directly coupled spins, and then transferring this two-spin state to another pair of spins whose direct interactions are negligible. Such transfers are expected to be an essential operation in scalable quantum computer architectures, and provide a useful benchmark for the coherent control available in specific implementations.
The highly parallel nature of the fundamental principles of quantum mechanics means that certain key resource-intensive tasks --- including searching, code decryption and medical, chemical and material simulations --- can be computed polynomially or even exponentially faster with a quantum computer. In spite of its remarkably fast development, the field of quantum computing is still young, and a large-scale prototype using any one of the candidate quantum bits (or 'qubits') under investigation has yet to be developed. Spin-based qubits in condensed matter systems are excellent candidates. Spins controlled using magnetic resonance have provided the first, most advanced, and highest fidelity experimental demonstrations of quantum algorithms to date. Despite having highly promising control characteristics, most physical ensembles investigated using magnetic resonance are unable to produce entanglement, a critical missing ingredient for a pure-state quantum computer. Quantum objects are said to be entangled if they cannot be described individually: they remain fundamentally linked regardless of their physical separation. Such highly non-classical states can be exploited for a host of quantum technologies including teleportation, metrology, and quantum computation. Here I describe how to experimentally create, control and characterise entangled quantum ensembles using magnetic resonance. I first explore the relationship between entanglement and quantum metrology and demonstrate a sensitivity enhancement over classical resources using molecular sensors controlled with liquid-state nuclear magnetic resonance. I then examine the computational potential of irreversible relaxation processes in combination with traditional reversible magnetic resonance control techniques. I show how irreversible processes can polarise both nuclear and electronic spins, which improves the quality of qubit initialisation. I discuss the process of quantum state tomography, where an arbitrary quantum state can be accurately measured and characterised, including components which go undetected using traditional magnetic resonance techniques. Lastly, I combine the above findings to initialise, create and characterise entanglement between an ensemble of electron and nuclear spin defects in silicon. I further this by generating pseudo-entanglement between an ensemble of nuclear spins mediated by a transient electron spin in a molecular system. These findings help pave the way towards a particular architecture for a scalable, spin-based quantum computer.
We show how entanglement may be quantified in spin and cold atom many-body systems using standard experimental techniques only. The scheme requires no assumptions on the state in the laboratory, and a lower bound to the entanglement can be read off directly from the scattering cross section of neutrons deflected from solid state samples or the time-of-flight distribution of cold atoms in optical lattices, respectively. This removes a major obstacle which so far has prevented the direct and quantitative experimental study of genuine quantum correlations in many-body systems: The need for a full characterization of the state to quantify the entanglement contained in it. Instead, the scheme presented here relies solely on global measurements that are routinely performed and is versatile enough to accommodate systems and measurements different from the ones we exemplify in this work.