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Low Temperature Physics

The energy spectrum and magnetization profile of the decorated spin ladder systems

Vladyslav O. Cheranovskii, E. V. Ezerskaya, S. Ye. Kononenko

Published Feb 1, 2024• 1 citation
Publisher

Abstract

The peculiarities of the energy spectrum of the decorated mixed spin two-leg ladder system having three spin unit cells have been studied by the perturbation theory in the limit of dominant spin coupling in ladder rungs. It is shown, that despite the singlet ground state, this spin ladder may have an intermediate plateau in a low-temperature magnetization profile. The existence of a similar plateau was shown also in the case of some intermediate values of coupling parameters by means of exact diagonalization study of small ladder clusters and by the density-matrix renormalization group calculations. We also found that the Ising type of interactions in ladder rungs may lead to the disappearance of the above intermediate magnetization plateau for the corresponding isotropic spin ladder.

DOI
10.1063/10.0024327

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The peculiarities of the energy spectrum of the decorated mixed spin two-leg ladder system having three spin unit cells have been studied by the perturbation theory in the limit of dominant spin coupling in ladder rungs. It is shown, that despite the singlet ground state, this spin ladder may have an intermediate plateau in a low-temperature magnetization profile. The existence of a similar plateau was shown also in the case of some intermediate values of coupling parameters by means of exact diagonalization study of small ladder clusters and by the density-matrix renormalization group calculations. We also found that the Ising type of interactions in ladder rungs may lead to the disappearance of the above intermediate magnetization plateau for the corresponding isotropic spin ladder.
The energy spectra and low-temperature magnetic properties of two one-dimensional Heisenberg mixed spin (s = 1, 1/2) systems, namely decorated two-leg mixed spin ladders with the lattice topology of polyacene, are studied. The gapless character of the exact excitation energy spectra for both ladder models has been determined. We found numerically that the model with macroscopic ground state spin S0 has gapped excitations with the spin S > S0. This leads to the appearance of an intermediate plateau in field dependence of magnetization at low temperatures. We have shown that the ladder with equal coupling in legs has the maximal size of this plateau at the same coupling in rungs. For a mixed spin ladder model with Ising interactions in legs, the appearance of two intermediate magnetization plateaus at low temperatures and some values of coupling parameters was shown.
Using the density-matrix renormalization-group technique we investigate the low-energy properties and the magnetization-plateau behavior in a two-leg mixed spin ladder consisting of a spin-1/2 chain coupled with a spin-1 chain. The calculated results show that the system is in the same universality class as the spin-3/2 chain when the interchain coupling is strongly ferromagnetic, but the similarity between the two systems is less clear under other coupling conditions. We have identified two types of magnetization-plateau phases. The calculation of the magnetization distribution on the spin-1/2 and the spin-1 chains on the ladder shows that one plateau phase is related to the partially magnetized valence-bond-solid state, and the other plateau state contains strongly coupled S=1S=1S=1 and s=1/2s=1/2s=1/2 spins on the rung.
The experimental realization of various spin ladder systems has prompted their detailed theoretical investigations. Here we study the evolution of ground-state magnetization with an external magnetic field for two different antiferromagnetic systems: a three-legged spin-1/21/21/2 ladder, and a two-legged spin-1/21/21/2 ladder with an additional diagonal interaction. The finite system density-matrix renormalization-group method is employed for numerical studies of the three-chain system, and an effective low-energy Hamiltonian is used in the limit of strong interchain coupling to study the two- and three-chain systems. The three-chain system has a magnetization plateau at one-third of the saturation magnetization. The two-chain system has a plateau at zero magnetization due to a gap above the singlet ground state. It also has a plateau at half of the saturation magnetization for a certain range of values of the couplings. We study the regions of transitions between plateaus numerically and analytically, and find that they are described, at first order in a strong-coupling expansion, by an XXZ\mathrm{XXZ}XXZ spin-1/21/21/2 chain in a magnetic field; the second-order terms give corrections to the XXZ\mathrm{XXZ}XXZ model. We also study numerically some low-temperature properties of the three-chain system, such as the magnetization, magnetic susceptibility and specific heat.
We investigate, at T =0, the magnetization process of the S =1 frustrated two-leg spin ladder having the leg interaction ( J ), the rung interaction ( J 0 ) and the diagonal interaction ( J d ), especially focusing on the appearance and the disappearance of the magnetization plateaux. We use the degenerate perturbation theory, the level spectroscopy analysis of the numerical diagonalization data and the DMRG. When J d =0, the M s /2 plateau ( M s is the saturation magnetization) appears for J 0 / J > 1.463. Then there is no M s /2 plateau for the so-called isotropic case J = J 0 . In case of J d > 0, J d helps the M s /2 plateau. And also, the M s /4 and (3/4) M s plateaux appear when J d is sufficiently large. These two plateaux are associated with the spontaneous breaking of the translation symmetry along the leg direction. We show the plateau phase diagram on the J d versus J plane, and also the magnetic phase diagram on the H versus J d plane for fixed J .
We show that the low-energy physics of the three-leg-ladder model in the presence of a critical magnetic field can be described by a broken SU(3) spin chain for a periodic rung model and a broken SU(2) spin chain for an open rung model. Using the Lieb-Schultz-Mattis theorem we characterize the possible magnetization plateaus and study the critical behaviour in the region of transition between the plateaus S z = 1/2 and S z = 3/2 by means of renormalization group calculations performed on the bosonized effective continuum field theory. We show that in certain regions of the parameter space of the effective theory the system remains gapless, and we compute the spin-spin correlation functions for these regions. We also discuss the possibility of a plateau at S z = 1, and show that although there exists in the continuum theory a term that might cause the appearance of a plateau there, such a term is unlikely to be relevant. This conjecture is proved by density-matrix renormalization group (DMRG) techniques. The modifications of the three-leg-ladder Hamiltonian that show plateaus at S z = 1, 5/6, 7/6 are discussed. We show the S z = 1 plateau in the XXZ -type modification by means of the DMRG technique. We find non-magnetic gapless excitation on this plateau in the periodic rung case.
We have studied the ground state phase diagram of a spin ladder with alternating rung exchange J⊥n=J⊥[1+(−1)nδ]J^{n}_{\perp} = J_{\perp}[1 + (-1)^{n} δ]J⊥n​=J⊥​[1+(−1)nδ] in a magnetic filed, in the limit where the rung coupling is dominant. In this limit the model is mapped onto an XXZXXZXXZ Heisenberg chain in a uniform and staggered longitudinal magnetic fields, where the amplitude of the staggered field is ∼δ\sim δ∼δ. We have shown that the magnetization curve of the system exhibits a plateau at magnetization equal to the half of the saturation value. The width of a plateau scales as δνδ^νδν, where ν=4/5ν=4/5ν=4/5 in the case of ladder with isotropic antiferromagnetic legs and ν=2ν=2ν=2 in the case of ladder with isotropic ferromagnetic legs. We have calculated four critical fields (Hc1±H^{\pm}_{c1}Hc1±​ and Hc2±H^{\pm}_{c2}Hc2±​) corresponding to transitions between different magnetic phases of the system. We have shown that these transitions belong to the universality class of the commensurate-incommensurate transition.