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Journal of Plasma Physics

Calibrated heating rate measurements using electric-field-induced electron extraction in ultracold neutral plasmas

John Guthrie, Puchang Jiang, Jacob Roberts

Published Feb 1, 2024• 2 citations
Publisher

Abstract

The heating rate of plasma electrons induced by external fields or other processes can be used as an experimental tool to measure fundamental plasma properties such as electrical conductivity or electron–ion collision rates. We have developed a technique that can measure electron heating rates in ultracold neutral plasmas (UNPs) with $\sim 10\,\%$ precision while simultaneously referencing the measurement to a calibrated amount of heating. This technique uses a sequence of applied electric fields in four sections: to control the ratio of electrons to ions in the UNP; to provide a time for the application of fields that cause electron heating and subsequent thermalization of the electrons after the application of those fields; to extract electrons from the UNP using a method sensitive to electron temperature that allows the measurement of electron heating; and to extract the remaining electrons to measure the total electron (and therefore ion) number. The primary signal used to measure the heating rate is the measurement of the number of electrons that escape in the third section of the experiment as a larger number of escaping electrons indicates a larger amount of heating. We illustrate the use of this technique by measuring electron heating caused by high-frequency radiofrequency (RF) fields. In addition to the main technique, several subtechniques to calibrate the electron temperature, electron density, amount of heating and applied RF field amplitude were developed as well.

DOI
10.1017/s0022377824000114

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The heating rate of plasma electrons induced by external fields or other processes can be used as an experimental tool to measure fundamental plasma properties such as electrical conductivity or electron–ion collision rates. We have developed a technique that can measure electron heating rates in ultracold neutral plasmas (UNPs) with ∼10 %\sim 10\,\%∼10% precision while simultaneously referencing the measurement to a calibrated amount of heating. This technique uses a sequence of applied electric fields in four sections: to control the ratio of electrons to ions in the UNP; to provide a time for the application of fields that cause electron heating and subsequent thermalization of the electrons after the application of those fields; to extract electrons from the UNP using a method sensitive to electron temperature that allows the measurement of electron heating; and to extract the remaining electrons to measure the total electron (and therefore ion) number. The primary signal used to measure the heating rate is the measurement of the number of electrons that escape in the third section of the experiment as a larger number of escaping electrons indicates a larger amount of heating. We illustrate the use of this technique by measuring electron heating caused by high-frequency radiofrequency (RF) fields. In addition to the main technique, several subtechniques to calibrate the electron temperature, electron density, amount of heating and applied RF field amplitude were developed as well.
Ultracold plasmas (UCPs) are created by photo-ionization of a cloud of laser-cooled atoms, and have initial electron temperatures in the range 1-100 K and initial ion temperatures in the range 0.001-1 K. As a consequence UCPs can be in the strongly coupled regime, where the typical Coulomb interaction between the particles exceeds the thermal energy of the particles; a clear distinction with conventional plasmas. UCPs are not stable systems and the electron and ion temperature will rise during their evolution. The introduction of a disturbing rf-field to the plasma is expected to speed up the heating of the plasma.In this thesis the intrinsic electron heating mechanisms are studied as well as the heating mechanisms induced by an external rf field. Numerical simulations were performed with the General Particle Tracer code and compared to analytical theories.Two intrinsic heating mechanisms were studied: disorder-induced heating (DIH) and heating by three-body recombination (TBR). 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The amount of collisional absorption was found to depend strongly on the amplitude of the rf field. It was found that the rf field effectively suppresses the electron-ion collision frequency as a function of increasing field amplitude, confirming analytical theories. For low to moderate amplitudes the amount of energy absorption increases, but less than one might intuitively expect due to the decrease in collision frequency. For very strong field amplitudes the energy absorption even decreases as a function of field amplitude.The understanding achieved, provides new roads to control these type of plasmas experimentally. Ultracold plasmas (UCPs) are created by photo-ionization of a cloud of laser-cooled atoms, and have initial electron temperatures in the range 1-100 K and initial ion temperatures in the range 0.001-1 K. As a consequence UCPs can be in the strongly coupled regime, where the typical Coulomb interaction between the particles exceeds the thermal energy of the particles; a clear distinction with conventional plasmas. UCPs are not stable systems and the electron and ion temperature will rise during their evolution. The introduction of a disturbing rf-field to the plasma is expected to speed up the heating of the plasma.In this thesis the intrinsic electron heating mechanisms are studied as well as the heating mechanisms induced by an external rf field. Numerical simulations were performed with the General Particle Tracer code and compared to analytical theories.Two intrinsic heating mechanisms were studied: disorder-induced heating (DIH) and heating by three-body recombination (TBR). DIH arises due the random initial positions of the electrons. An excess of potential energy exists in the electron distribution which is rapidly converted into thermal energy. The time scale of DIH was found to be on the order of the inverse Mie-frequency, confirming analytical theories. TBR was identified in the simulations and the TBR heating rate was found to agree well with analytical models. Two rf-induced heating mechanisms were studied: collisionless energy absorption and collisional absorption. The first of these processes was found to depend strongly on the ratio between the rf field frequency and the oscillation frequency of the electrons in the plasma. Collisional absorption was studied in a regime that collisionless absorption is negligible. Absorption arises because the electrons, which are oscillating at the rf field frequency, are deflected by the Coulomb fields of the ions. The amount of collisional absorption was found to depend strongly on the amplitude of the rf field. It was found that the rf field effectively suppresses the electron-ion collision frequency as a function of increasing field amplitude, confirming analytical theories. For low to moderate amplitudes the amount of energy absorption increases, but less than one might intuitively expect due to the decrease in collision frequency. For very strong field amplitudes the energy absorption even decreases as a function of field amplitude.The understanding achieved, provides new roads to control these type of plasmas experimentally.
Using high-resolution laser-induced fluorescence spectroscopy, ion dynamics in\nan expanding ultracold neutral plasma (UNP) have been studied in unprecedented\ndetail. The evolution of the ion temperature is of great interest because the ions in\nan ultracold neutral plasma are strongly coupled, meaning their Coulomb interaction\nenergy exceeds the thermal energy. This leads to novel plasma properties that are\nhard to describe theoretically. Understanding all the factors that contribute to ion\ntemperature evolution is critical for designing schemes to cool the ions and achieve\neven stronger Coulomb coupling.\nThis work has also observed several phenomena that have not previously been\nstudied in ultracold plasmas. Ion adiabatic cooling has been observed in a UNP for\nthe first time, resulting in ion temperatures as low as 100mK and up to a tripling of\nthe Coulomb coupling parameter. The importance of electron-ion energy transfer is\ndemonstrated with the first observations of electron-ion collisional heating. Inclusion\nof this effect into existing numerical models provides better agreement with experimental\nresults. Results of molecular dynamics simulations of equilibrating plasmas\nhave been compared to early time experimental data, which provides a new method\nof density determination that is much less sensitive to experimental systematics and\nis accurate to within 10%. This improved certainty in the density allows accurate\ncomparison between data and a theoretical model of the plasma dynamics. The\nagreement is excellent, but on a hydrodynamic time scale a small amount of extra\nheat (on order of 100mK), not ascribable to electron-ion collisions or other sources in\nthe model, is detected in the ion component. Potential sources are discussed within\nas well as proposals for further studies and improvements.
We have experimentally demonstrated both heating and cooling of electrons in an ultracold neutral plasma (UNP) by embedding Rydberg atoms into the plasma soon after its creation. We have determined the relationship between the initial electron temperature, Te,i{T}_{e,i}Te,i​, and the binding energy of the added Rydberg atoms, Eb{E}_{b}Eb​, at the crossover between heating and cooling behaviors (that is, the binding energy of the atoms, which, when they are added to the plasma, neither accelerate nor slow down the plasma expansion). Specifically, this condition is $|{E}_{b}|\ensuremath{\approx}2.7\ifmmode\times\else\texttimes\fi{}{k}_{B}{T}_{e,i}$ when the diagnostic used is the effect of the Rydberg atoms on the plasma asymptotic expansion velocity. Additionally, we have obtained experimental estimates for the amount of heating or cooling which occurs when the Rydberg binding energy does not satisfy the crossover condition. The experimental results for the crossover condition, and the degree of heating or cooling away from the crossover, are in agreement with predictions obtained from numerical modeling of the interactions between Rydberg atoms and the plasma. We have also developed a simple intuitive picture of how the Rydberg atoms affect the plasma, which supports the concept of a ``bottleneck'' in the Rydberg state distribution of atoms in equilibrium with a coexisting plasma.
tion of the electrons. This oscillation will damp after the application of the electric eld pulse. We have found that under certain achievable experimental conditions, this damping can be dominated by the electron-ion collision rate. We have measured this damping rate experimentally under these conditions and thus can compare it to theoretical predictions. We will present our measurement technique and results. In addition, we will discuss extensions of this technique to measurements of electron temperature, to investigating strong-coupling physics in the electron component of an ultracold plasma, and to measuring the electron-ion collision rate when the electrons are highly magnetized.
The expansion of ultracold neutral plasmas (UCP) is driven primarily by the thermal pressure of the electron component and is therefore sensitive to the electron temperature. For typical UCP spatial extents, evaporative cooling has a significant influence on the UCP expansion rate at lower densities (less than 108/cm3). We studied the effect of electron evaporation in this density range. Owing to the low density, the effects of three-body recombination were negligible. We modeled the expansion by taking into account the change in electron temperature owing to evaporation as well as adiabatic expansion and found good agreement with our data. We also developed a simple model for initial evaporation over a range of ultracold plasma densities, sizes, and electron temperatures to determine over what parameter range electron evaporation is expected to have a significant effect. We also report on a signal calibration technique, which relates the signal at our detector to the total number of ions and electrons in the ultracold plasma.