Ultracold plasmas (UCPs) are created by photo-ionization of a cloud of laser-cooled atoms, and have initial electron temperatures in the range 1-100 K and initial ion temperatures in the range 0.001-1 K. As a consequence UCPs can be in the strongly coupled regime, where the typical Coulomb interaction between the particles exceeds the thermal energy of the particles; a clear distinction with conventional plasmas. UCPs are not stable systems and the electron and ion temperature will rise during their evolution. The introduction of a disturbing rf-field to the plasma is expected to speed up the heating of the plasma.In this thesis the intrinsic electron heating mechanisms are studied as well as the heating mechanisms induced by an external rf field. Numerical simulations were performed with the General Particle Tracer code and compared to analytical theories.Two intrinsic heating mechanisms were studied: disorder-induced heating (DIH) and heating by three-body recombination (TBR). DIH arises due the random initial positions of the electrons. An excess of potential energy exists in the electron distribution which is rapidly converted into thermal energy. The time scale of DIH was found to be on the order of the inverse Mie-frequency, confirming analytical theories. TBR was identified in the simulations and the TBR heating rate was found to agree well with analytical models. Two rf-induced heating mechanisms were studied: collisionless energy absorption and collisional absorption. The first of these processes was found to depend strongly on the ratio between the rf field frequency and the oscillation frequency of the electrons in the plasma. Collisional absorption was studied in a regime that collisionless absorption is negligible. Absorption arises because the electrons, which are oscillating at the rf field frequency, are deflected by the Coulomb fields of the ions. The amount of collisional absorption was found to depend strongly on the amplitude of the rf field. It was found that the rf field effectively suppresses the electron-ion collision frequency as a function of increasing field amplitude, confirming analytical theories. For low to moderate amplitudes the amount of energy absorption increases, but less than one might intuitively expect due to the decrease in collision frequency. For very strong field amplitudes the energy absorption even decreases as a function of field amplitude.The understanding achieved, provides new roads to control these type of plasmas experimentally. Ultracold plasmas (UCPs) are created by photo-ionization of a cloud of laser-cooled atoms, and have initial electron temperatures in the range 1-100 K and initial ion temperatures in the range 0.001-1 K. As a consequence UCPs can be in the strongly coupled regime, where the typical Coulomb interaction between the particles exceeds the thermal energy of the particles; a clear distinction with conventional plasmas. UCPs are not stable systems and the electron and ion temperature will rise during their evolution. The introduction of a disturbing rf-field to the plasma is expected to speed up the heating of the plasma.In this thesis the intrinsic electron heating mechanisms are studied as well as the heating mechanisms induced by an external rf field. Numerical simulations were performed with the General Particle Tracer code and compared to analytical theories.Two intrinsic heating mechanisms were studied: disorder-induced heating (DIH) and heating by three-body recombination (TBR). DIH arises due the random initial positions of the electrons. An excess of potential energy exists in the electron distribution which is rapidly converted into thermal energy. The time scale of DIH was found to be on the order of the inverse Mie-frequency, confirming analytical theories. TBR was identified in the simulations and the TBR heating rate was found to agree well with analytical models. Two rf-induced heating mechanisms were studied: collisionless energy absorption and collisional absorption. The first of these processes was found to depend strongly on the ratio between the rf field frequency and the oscillation frequency of the electrons in the plasma. Collisional absorption was studied in a regime that collisionless absorption is negligible. Absorption arises because the electrons, which are oscillating at the rf field frequency, are deflected by the Coulomb fields of the ions. The amount of collisional absorption was found to depend strongly on the amplitude of the rf field. It was found that the rf field effectively suppresses the electron-ion collision frequency as a function of increasing field amplitude, confirming analytical theories. For low to moderate amplitudes the amount of energy absorption increases, but less than one might intuitively expect due to the decrease in collision frequency. For very strong field amplitudes the energy absorption even decreases as a function of field amplitude.The understanding achieved, provides new roads to control these type of plasmas experimentally.
Ultracold plasmas (UCPs) are created by photo-ionization of a cloud of laser-cooled atoms, and have initial electron temperatures in the range 1-100 K and initial ion temperatures in the range 0.001-1 K. As a consequence UCPs can be in the strongly coupled regime, where the typical Coulomb interaction between the particles exceeds the thermal energy of the particles; a clear distinction with conventional plasmas. UCPs are not stable systems and the electron and ion temperature will rise during their evolution. The introduction of a disturbing rf-field to the plasma is expected to speed up the heating of the plasma.In this thesis the intrinsic electron heating mechanisms are studied as well as the heating mechanisms induced by an external rf field. Numerical simulations were performed with the General Particle Tracer code and compared to analytical theories.Two intrinsic heating mechanisms were studied: disorder-induced heating (DIH) and heating by three-body recombination (TBR). DIH arises due the random initial positions of the electrons. An excess of potential energy exists in the electron distribution which is rapidly converted into thermal energy. The time scale of DIH was found to be on the order of the inverse Mie-frequency, confirming analytical theories. TBR was identified in the simulations and the TBR heating rate was found to agree well with analytical models. Two rf-induced heating mechanisms were studied: collisionless energy absorption and collisional absorption. The first of these processes was found to depend strongly on the ratio between the rf field frequency and the oscillation frequency of the electrons in the plasma. Collisional absorption was studied in a regime that collisionless absorption is negligible. Absorption arises because the electrons, which are oscillating at the rf field frequency, are deflected by the Coulomb fields of the ions. The amount of collisional absorption was found to depend strongly on the amplitude of the rf field. It was found that the rf field effectively suppresses the electron-ion collision frequency as a function of increasing field amplitude, confirming analytical theories. For low to moderate amplitudes the amount of energy absorption increases, but less than one might intuitively expect due to the decrease in collision frequency. For very strong field amplitudes the energy absorption even decreases as a function of field amplitude.The understanding achieved, provides new roads to control these type of plasmas experimentally. Ultracold plasmas (UCPs) are created by photo-ionization of a cloud of laser-cooled atoms, and have initial electron temperatures in the range 1-100 K and initial ion temperatures in the range 0.001-1 K. As a consequence UCPs can be in the strongly coupled regime, where the typical Coulomb interaction between the particles exceeds the thermal energy of the particles; a clear distinction with conventional plasmas. UCPs are not stable systems and the electron and ion temperature will rise during their evolution. The introduction of a disturbing rf-field to the plasma is expected to speed up the heating of the plasma.In this thesis the intrinsic electron heating mechanisms are studied as well as the heating mechanisms induced by an external rf field. Numerical simulations were performed with the General Particle Tracer code and compared to analytical theories.Two intrinsic heating mechanisms were studied: disorder-induced heating (DIH) and heating by three-body recombination (TBR). DIH arises due the random initial positions of the electrons. An excess of potential energy exists in the electron distribution which is rapidly converted into thermal energy. The time scale of DIH was found to be on the order of the inverse Mie-frequency, confirming analytical theories. TBR was identified in the simulations and the TBR heating rate was found to agree well with analytical models. Two rf-induced heating mechanisms were studied: collisionless energy absorption and collisional absorption. The first of these processes was found to depend strongly on the ratio between the rf field frequency and the oscillation frequency of the electrons in the plasma. Collisional absorption was studied in a regime that collisionless absorption is negligible. Absorption arises because the electrons, which are oscillating at the rf field frequency, are deflected by the Coulomb fields of the ions. The amount of collisional absorption was found to depend strongly on the amplitude of the rf field. It was found that the rf field effectively suppresses the electron-ion collision frequency as a function of increasing field amplitude, confirming analytical theories. For low to moderate amplitudes the amount of energy absorption increases, but less than one might intuitively expect due to the decrease in collision frequency. For very strong field amplitudes the energy absorption even decreases as a function of field amplitude.The understanding achieved, provides new roads to control these type of plasmas experimentally.
Several mechanisms by which an external electromagnetic field influences the temperature of a plasma are studied analytically and specialized to the system of an ultracold plasma (UCP) driven by a uniform radio-frequency (rf) field. Heating through collisional absorption is reviewed and applied to UCPs. Furthermore, it is shown that the rf field modifies the three-body recombination process by ionizing electrons from intermediate high-lying Rydberg states and upshifting the continuum threshold, resulting in a suppression of three-body recombination. Heating through collisionless absorption associated with the finite plasma size is calculated in detail, revealing a temperature threshold below which collisionless absorption is ineffective.
By photoionizing samples of laser-cooled atoms with laser light tuned just above the ionization limit, plasmas can be created with electron and ion temperatures below 10 K. These ultracold neutral plasmas have extended the temperature bounds of plasma physics by two orders of magnitude. Table-top experiments, using many of the tools from atomic physics, allow for the study of plasma phenomena in this new regime with independent control over the density and temperature of the plasma through the excitation process. Characteristic of these systems is an inhomogeneous density profile, inherited from the density distribution of the laser-cooled neutral atom sample. Most work has dealt with unconfined plasmas in vacuum, which expand outward at velocities of order 100 m/s, governed by electron pressure, and with lifetimes of order 100 μs, limited by stray electric fields. Using detection of charged particles and optical detection techniques, a wide variety of properties and phenomena have been observed, including expansion dynamics, collective excitations in both the electrons and ions, and collisional properties. Through three-body recombination collisions, the plasmas rapidly form Rydberg atoms, and clouds of cold Rydberg atoms have been observed to spontaneously avalanche ionize to form plasmas. Of particular interest is the possibility of the formation of strongly coupled plasmas, where Coulomb forces dominate thermal motion and correlations become important. The strongest impediment to strong coupling is disorder-induced heating, a process in which Coulomb energy from an initially disordered sample is converted into thermal energy. This restricts electrons to a weakly coupled regime and leaves the ions barely within the strongly coupled regime. This review will give an overview of the field of ultracold neutral plasmas, from its inception in 1999 to current work, including efforts to increase strong coupling and effects on plasma properties due to strong coupling.
Ultracold neutral plasmas are created by photoionizing laser-cooled atoms in a magneto-optical trap (MOT). Due to their large electrical potential energies and comparatively small kinetic energies, ultracold plasmas fall into a regime of plasma systems which are called “strongly coupled.” A priority in the field of ultracold plasmas is to generate plasmas with higher values of the strong coupling parameter Γ, which is given as the ratio of the nearest-neighbor Coulomb potential energy to the average kinetic energy. The equilibrium strong coupling in ultracold plasmas is limited by the ultrafast relaxation of the ions due to spatial disorder in the initial system. This heating mechanism is called “disorder-induced heating” (DIH) and it limits the ion strong coupling in ultracold plasmas to order unity. This thesis describes experiments that explore ways to generate higher values of the strong coupling parameter in an ultracold neutral calcium plasma.One way to increase Γ is to mitigate the effects of DIH using electron screening. This thesis describes an experiment in which the initial electron temperature was systematically changed to determine the effect that electron screening has on the ion thermalization. At lower initial electron temperatures, corresponding to a higher degree of electron shielding, it was found that the screening slows the ion thermalization and reduces the equilibrium ion temperature by as much as a factor of two. However, electron screening also reduces the ion interaction strength by the same amount, which has the net effect of leaving the effective Γ unchanged.Another method for increasing the strong coupling of an ultracold plasma is to excite the plasma ions to a higher ionization state. Simulations predict that doubly ionizing the plasma ions can increase the strong coupling in an ultracold plasma by as much as a factor of 4, with the maximum value of Γ depending on the timing of the second ionization relative to the DIH process. This thesis describes an experiment designed to test these predictions in a Ca2+ plasma. Measurements of the change in the Ca+ ion temperature as a function of the timing of the second ionization pulses were made using laser-induced fluorescence. Results of these measurements show that the heating of the Ca+ ions due to the second ionization depends on the timing of the second ionization pulses, as predicted by MD simulations.
In this dissertation I describe a number of different computational investigations which I have undertaken during my time at Colorado State University. Perhaps the most significant of my accomplishments was the development of a general molecular dynamic model that simulates a wide variety of physical phenomena in ultracold plasmas (UCPs). This model formed the basis of most of the numerical investigations discussed in this thesis. The model utilized the massively parallel architecture of GPUs to achieve significant computing speed increases (up to 2 orders of magnitude) above traditional single core computing. This increased computing power allowed for each particle in an actual UCP experimental system to be explicitly modeled in simulations. By using this model, I was able to undertake a number of theoretical investigations into ultracold plasma systems. Chief among these was our lab's investigation of electron center-of-mass damping, in which the molecular dynamics model was an essential tool in interpreting the results of the experiment. Originally, it was assumed that this damping would solely be a function of electron-ion collisions. However, the model was able to identify an additional collisionless damping mechanism that was determined to be significant in the first iteration of our experiment. To mitigate this collisionless damping, the model was used to find a new parameter range where this mechanism was negligible. In this new parameter range, the model was an integral part in verifying the achievement of a record low measured UCP electron temperature of 1.57 ± 0.28K and a record high electron strong coupling parameter, Γ, of 0.35 ± 0.08. Additionally, the model, along with experimental measurements, was used to verify the breakdown of the standard weak coupling approximation for Coulomb collisions. The general molecular dynamics model was also used in other contexts. These included the modeling of both the formation process of ultracold plasmas and the thermalization of the electron component of an ultracold plasma. Our modeling of UCP formation is still in its infancy, and there is still much outstanding work. However, we have already discovered a previously unreported electron heating mechanism that arises from an external electric field being applied during UCP formation. Thermalization modeling showed that the ion density distribution plays a role in the thermalization of electrons in ultracold plasma, a consideration not typically included in plasma modeling. A Gaussian ion density distribution was shown to lead to a slightly faster electron thermalization rate than an equivalent uniform ion density distribution as a result of collisionless effects. Three distinct phases of UCP electron thermalization during formation were identified. Finally, the dissertation will describe additional computational investigations that preceded the general molecular dynamics model. These include simulations of ultracold plasma ion expansion driven by non-neutrality, as well as an investigation into electron evaporation. To test the effects of non-neutrality on ion expansion, a numerical model was developed that used the King model of the electron to describe the electron distribution for an arbitrary charge imbalance. The model found that increased non-neutrality of the plasma led to the rapid expansion of ions on the plasma exterior, which in turn led to a sharp ion cliff-like spatial structure. Additionally, this rapid expansion led to additional cooling of the electron component of the plasma. The evaporation modeling was used to test the underlying assumptions of previously developed analytical expression for charged particle evaporation. The model used Monte Carlo techniques to simulate the collisions and the evaporation process. The model found that neither of the underlying assumption of the charged particle evaporation expressions held true for typical ultracold plasma parameters and provides a route for computations in spite of the breakdown of these two typical assumptions.
Disorder-induced heating (DIH) is one of the main reasons reducing the coupling strength in ultracold plasma. We propose applying an optical lattice as periodic confinement before the ultracold atomic cloud is ionized to eliminate its effect. We demonstrate a numerical simulation for the dynamics of the ultracold plasmas using classical molecular dynamics method with open boundary. DIH is reproduced in the simulation with the random Gaussian initial distribution and is absent in the results with the ordered lattice initial distribution. We further find that the collisional heating from electrons is important for ultracold plasmas with chosen spatial correlations in the optical lattice. Carefully preparing the initial condition (e.g., the ion density, initial electron temperature, and so on), collisional heating for the ions would be significantly reduced and eventually negligible. This allows a much stronger coupling in ultracold plasma to be realized.
Ultracold neutral plasmas provide a useful system for studying extreme parameter regime plasma physics in an accessible laboratory setting. The parameter space of plasma physics can be characterized in part by coupling strength and degree of magnetization. The range of achievable strong coupling is determined in part by the lowest possible temperatures that can be achieved. This work examines the early-lifetime electron heating of moderately coupled, strongly magnetized plasmas. This heating is dominated by disorder-induced heating (DIH) and heating due to Rydberg atom formation. By using experimentally informed simulations, it is found that DIH has a large influence in electron temperature well into the plasma lifetime. Additionally, the dependence of the minimum achievable electron temperature on magnetization and initial electron energy is examined. In this work, we find electron temperatures as low as 0.53 ± 0.05 K (for an electron density, ne, of 6.1×1012 m−3), which determines the maximum coupling strength for the measured experimental conditions.