Abstract Single electron spins bound to multi-phosphorus nuclear spin registers in silicon have demonstrated fast (0.8 ns) two-qubit SWAP SWAP gates and long spin relaxation times (~30 s). In these spin registers, when the donors are ionized, the nuclear spins remain weakly coupled to their environment, allowing exceptionally long coherence times. When the electron is present, the hyperfine interaction allows coupling of the spin and charge degrees of freedom for fast qubit operation and control. Here we demonstrate the use of the hyperfine interaction to enact electric dipole spin resonance to realize high-fidelity ( F=100−6+0 F = 10 0 − 6 + 0 %) initialization of all the nuclear spins within a four-qubit nuclear spin register. By controllably initializing the nuclear spins to ∣⇓⇓⇓⟩ ⇓ ⇓ ⇓ , we achieve single-electron qubit gate fidelities of F = 99.78 ± 0.07% (Clifford gate fidelities of 99.58 ± 0.14%), above the fault-tolerant threshold for the surface code with a coherence time of $${T}_{2}^{\,* }=12\,\upmu {{{\rm{s}}}}$$ T 2 * = 12 μ s .
Abstract Phosphorus atoms in silicon are an outstanding platform for quantum computing as their nuclear spins exhibit coherence time over seconds [1, 2]. By placing multiple phosphorus atoms within a radius of a few nanometers, they couple via the hyperfine interaction to a single, shared electron. Such a nuclear spin register enables multi-qubit control above the fault-tolerant threshold [3] and the execution of small-scale quantum algorithms [4]. To achieve quantum error correction, fast and efficient interconnects have to be implemented between spin registers while maintaining high fidelity across all qubit metrics. Here, we demonstrate such integration with a fully controlled 11-qubit atom processor composed of two multi-nuclear spin registers which are linked via electron exchange interaction. Through the development of scalable calibration and control protocols, we achieve coherent coupling between nuclear spins using a combination of single- and multi-qubit gates with all fidelities ranging from 99.5% to 99.99%. We verify the efficient all-to-all connectivity by preparing both local and non-local Bell states with a record state fidelity beyond 99% and extend entanglement through the generation of Greenberger-Horne-Zeilinger (GHZ) states over all data qubits. By establishing high-fidelity operation across interconnected nuclear-spin registers, we ealise a key milestone towards fault-tolerant quantum computation with atom processors.
Spin qubits in silicon are strong contenders for the realization of a practical quantum computer, having demonstrated single- and two-qubit gates with fidelities above the fault-tolerant threshold, and entanglement of three qubits. However, maintaining high-fidelity operations while increasing the qubit count remains challenging and therefore only two-qubit algorithms have been executed. Here we utilize a four-qubit silicon processor with all control fidelities above the fault-tolerant threshold and demonstrate a three-qubit Grover's search algorithm with a ~95% probability of finding the marked state. Our processor is made of three phosphorus atoms precision-patterned into isotopically pure silicon, which localise one electron. The long coherence times of the qubits enable single-qubit fidelities above 99.9% for all qubits. Moreover, the efficient single-pulse multi-qubit operations enabled by the electron-nuclear hyperfine interaction facilitate controlled-Z gates between all pairs of nuclear spins with fidelities above 99% when using the electron as an ancilla. These control fidelities, combined with high-fidelity non-demolition readout of all nuclear spins, allow the creation of a three-qubit Greenberger-Horne-Zeilinger state with 96.2% fidelity. Looking ahead, coupling neighbouring nuclear spin registers, as the one shown here, via electron-electron exchange may enable larger, fault-tolerant quantum processors.