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Physical Review A

Multidimensional matter-wave beam splitters by multiphoton hyperfine Raman transitions

Xu-Dong Liu, Zongyou Chen, Weichun Huang, Yang-Kao Lee, Yong‐Fan Chen, Pei-Chen Kuan

Published Jan 31, 2024• 3 citations
Publisher

Abstract

Multidimensional beamsplitters play crucial roles in the development of multidimensional atom interferometers and have the potential for applications in quantum information in higher dimensions. We present different configurations of multidimensional beamsplitters using both conventional two-photon Raman transitions and recently discovered four-photon Raman transitions. The differences between these configurations arise from the selection of external magnetic fields to serve as quantization axes. We explored and estimated statistical and systematic errors that may occur when multiple Raman transitions are used to construct multidimensional atom interferometers with deviated quantization axes. Our results demonstrated a tradeoff between the simplicity of axis alignment relative to the beams and the required optical power. These considerations are pertinent to the future design and optimization of multidimensional atom interferometry systems.

DOI
10.1103/physreva.109.013327

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Multidimensional beamsplitters play crucial roles in the development of multidimensional atom interferometers and have the potential for applications in quantum information in higher dimensions. We present different configurations of multidimensional beamsplitters using both conventional two-photon Raman transitions and recently discovered four-photon Raman transitions. The differences between these configurations arise from the selection of external magnetic fields to serve as quantization axes. We explored and estimated statistical and systematic errors that may occur when multiple Raman transitions are used to construct multidimensional atom interferometers with deviated quantization axes. Our results demonstrated a tradeoff between the simplicity of axis alignment relative to the beams and the required optical power. These considerations are pertinent to the future design and optimization of multidimensional atom interferometry systems.
The quantization axis defines the local interaction between the electromagnetic fields and the atoms. We studied both theoretically and experimentally the hyperfine Raman transition with different quantization axis and found a four-photon Raman transition which happened when the quantization axis is shifting from being parallel to perpendicular to the Raman beams' direction. It keeps the magnetic-field-insensitive feature like the two-photon Raman transition but can be used straightforwardly in multidimensional applications, like inertial sensors or even higher-dimensional quantum walk systems. In addition to inertial sensors, we also discuss the potential quantum sensing applications in magnetometers when the quantization axis is away from perpendicular due to magnetic-field perturbations.
The coherent control of atomic wave packets in multiple momentum dimensions is a central challenge in Raman atom optics and a key requirement for multidimensional atom interferometry. In this paper, a momentum-basis theoretical framework is developed for two-dimensional Raman interactions. We formulate the atom-laser interaction for two-dimensional Raman beams and obtain the effective two-level ground-state Hamiltonian after adiabatic elimination of the excited states. The resulted Hamiltonian is constructed on the reachable momentum-state lattice and includes AC Stark shifts, intra-dimensional Raman couplings, and cross-dimensional Raman coupling terms, thereby describing multidimensional Raman dynamics beyond a simple superposition of independent single-dimensional models. The framework is used to analyze the principles and operating conditions of two-dimensional atom interferometry. Cross-dimensional Raman coupling and sequential reverse Raman transitions are identified as the main mechanisms that redistribute atoms into non-target momentum states and reduce the contrast of atomic interferometer fringe. Experimentally, Ramsey fringes are observed in a cold-atom fountain interferometer, with a contrast of 14.8%14.8\%14.8% at an interrogation time of T=10 msT=10~{\rm ms}T=10 ms, in good agreement with the theoretical calculation. The conditions required for velocity-sensitive multidimensional atom interferometry are further clarified, including detuning control, velocity-class selection, and suppression of undesired inter-dimensional transitions. This work provides a theoretical and experimental basis for multidimensional Raman atom interferometry.
A special kind of atomic beam splitter using a four-level atomic system in combination with polarized light fields is demonstrated. These specific atom optical elements are used to operate an atom interferometer where the beam-splitting mechanism acts selectively on specific paths only and therefore allows for several different interferometer geometries. Based on a Ramsey-Bord\'e configuration, the experimental data show considerably better accuracy and a contrast enhanced by 65% compared to the two-level interferometer. Our concept appears to be especially interesting in the context of metrological aspects in matter-wave interferometry.
We propose and demonstrate a new scheme for atom interferometry, using light pulses inside an optical cavity as matter wave beam splitters. The cavity provides power enhancement, spatial filtering, and a precise beam geometry, enabling new techniques such as low power beam splitters (<100 μW), large momentum transfer beam splitters with modest power, or new self-aligned interferometer geometries utilizing the transverse modes of the optical cavity. As a first demonstration, we obtain Ramsey-Raman fringes with >75% contrast and measure the acceleration due to gravity, g, to 60 μg/sqrt[Hz] resolution in a Mach-Zehnder geometry. We use >10(7) cesium atoms in the compact mode volume (600 μm 1/e(2) waist) of the cavity and show trapping of atoms in higher transverse modes. This work paves the way toward compact, high sensitivity, multiaxis interferometry.
This cumulative thesis consists of four publications [1-4], presented as three contributions (I) - (III), where the second one (II) consists of the joint publications [2,3]. All publications were written during the author's research activities at the Institute of Quantum Physics under the supervision of Prof. Dr. W. P. Schleich. All of the presented publications consider light-matter interactions and their potential application in atom interferometry, a comparatively young and rapidly evolving technique. Atom interferometers find application in high-precision measurements, the determination of physical constants, the testing of fundamental physics, and the provision of gravimeters and gyroscopes. The advancement of technology and science has led to significant improvements in performance and the development of ambitious mobile and space-based devices. The recent success of several experiments has led to the proposal of further experiments with the aim of opening up new frontiers. However, the construction of future devices necessitates a decision regarding the employed diffraction mechanism and geometry, depending on the specific technical and scientific requirements. Furthermore, it is necessary to enhance the sensitivity of future devices. The contributions in this dissertation address these issues. The first contribution (I) focuses on the diffraction of atoms by laser pulses which can be employed to generate atom-optical diffraction elements like beam splitters and mirrors. These diffraction elements can be combined to construct atom interferometers, which have been successfully employed for precision measurements regarding fundamental physics as well as practical applications. The article presents a numerical comparison of two distinct diffraction mechanisms (Bragg and Raman) and diffraction geometries (single and double diffraction) in microgravity. It discusses the fundamental differences between the mechanisms and geometries with respect to the diffraction efficiency, taking into account the width of the initial wave function and the duration of the light pulse. Additionally, it explores the transition between the two diffraction geometries when starting from an atom initially at rest and increasing its momentum. The results may serve as a reference for experimentalists in selecting the most suitable configuration, based on their aims and requirements in the realization of more advanced atom interferometers. The second contribution (II) is a follow-up to the previous one, but focuses exclusively on a single diffraction type in microgravity, namely the so-called double Raman diffraction. In contrast to the previous article, where we only discussed single two-photon processes, we consider in this article a six-photon process, also known as third-order diffraction, as well as three subsequent two-photon processes, which both lead to the same amount of transferred momentum and can both be used to realize large-momentum transfer (LMT). We demonstrate that third-order double Raman diffraction is a viable and advantageous method for the diffraction of small momentum distributions like Bose-Einstein condensates (BECs) compared to a sequence of three two-photon processes. Furthermore, we show that third-order Raman pulses can be successfully applied to create higher-order Raman atom interferometers. Third-order diffraction can be perfectly combined with other LMT techniques and, moreover, allows for a reduction in the overall duration of the diffraction process and the complexity of the experimental set-up, as only two distinct laser frequencies are required. Moreover, we present a third-order Mach-Zehnder interferometer with spurious paths being disregarded. As demonstrated later on in [3], this interferometer generates optimal contrast and a substantial amplitude. The third contribution (III) extends the semi-classical λ-scheme of single Raman diffraction, as discussed in detail in contribution (I), into a fully quantized multi-atom multi-λ configuration with center-of-mass motion inside a cavity. Therefore, the incorporation of an internal structure allows for a more realistic modeling of the atoms, which is relevant for multi-photon interaction or cooling processes. We use for our analysis the framework of second quantization, i.e., we take into account the field-theoretical nature of the multi-particle atomic field as well as of the diffracting light field. We reduce this model with a Hamiltonian averaging theory applied to the atomic field operators and obtain an effective Hamiltonian, which determines the time evolution of the system. We demonstrate the efficiency of our model by the application of a typical initial state. Moreover, for a specific input state, we obtain the Hong-Ou-Mandel effect simultaneously in the atomic and the optical system. Our many-body formalism is perfectly suited to theoretically describe contemporary high-precision atom interferometric experiments based on entanglement between the atoms, that aim to surpass the shot-noise limit.
An atom interferometer based on Doppler-insensitive Raman transition is proposed, which has sharply peaked interference fringes for multi-wave interference. We show that two sets of counter-propagating Doppler-insensitive Raman beam pairs can be used to construct a new type of multi-wave beam splitter, which can be used to construct an atom interferometer. Although the spacing between adjacent diffraction orders of the interferometer is small, they can be distinguished by the internal state of the atom. Our analysis shows that the width of the fringes of this atom interferometer is inversely proportional to the width (duration) of the beam splitter and the Rabi frequency of the Raman beams, that is, the interferometer can achieve high resolution at high light intensity and long pulse width.