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Physical Review Letters

d -Mon: A Transmon with Strong Anharmonicity Based on Planar c -Axis Tunneling Junction between d -Wave and s -Wave Superconductors

Hrishikesh E. Patel, Vedangi Pathak, Oguzhan Can, Andrew C. Potter, Marcel Franz

Published Jan 5, 2024• 19 citations
Publisher

Abstract

We propose a novel qubit architecture based on a planar c-axis Josephson junction between a thin flake d-wave superconductor, such as a high-T_{c} cuprate Bi_{2}Sr_{2}CaCu_{2}O_{8+x}, and a conventional s-wave superconductor. When operated in the transmon regime the device-that we call "d mon"-becomes insensitive to offset charge fluctuations and, importantly, exhibits at the same time energy level spectrum with strong anharmonicity that is widely tunable through the device geometry and applied magnetic flux. Crucially, unlike previous qubit designs based on d-wave superconductors the proposed device operates in a regime where quasiparticles are fully gapped and can be therefore expected to achieve long coherence times.

DOI
10.1103/physrevlett.132.017002

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We propose a novel qubit architecture based on a planar c-axis Josephson junction between a thin flake d-wave superconductor, such as a high-T_{c} cuprate Bi_{2}Sr_{2}CaCu_{2}O_{8+x}, and a conventional s-wave superconductor. When operated in the transmon regime the device-that we call "d mon"-becomes insensitive to offset charge fluctuations and, importantly, exhibits at the same time energy level spectrum with strong anharmonicity that is widely tunable through the device geometry and applied magnetic flux. Crucially, unlike previous qubit designs based on d-wave superconductors the proposed device operates in a regime where quasiparticles are fully gapped and can be therefore expected to achieve long coherence times.
We propose a novel qubit architecture based on a planar ccc-axis Josephson junction between a thin flake ddd-wave superconductor (dddSC), such as a high-TcT_cTc​ cuprate Bi2_22​Sr2_22​CaCu2_22​O8+x_{8+x}8+x​, and a conventional sss-wave superconductor. When operated in the transmon regime the device -- that we call "ddd-mon" -- becomes insensitive to offset charge fluctuations and, importantly, exhibits at the same time energy level spectrum with strong anharmonicity that is widely tunable through the device geometry and applied magnetic flux. Crucially, unlike previous qubit designs based on ddd-wave superconductors the proposed device operates in a regime where quasiparticles are fully gapped and can be therefore expected to achieve long coherence times.
Superconducting transmon qubits with strong anharmonicity and insensitivity to offset charge are highly desirable for low-error implementation. In this work we propose a c-axis junction, comprising triplet superconductors, and set at a relative twist angle. Invoking spin-orbit coupling and spin polarization, which are known to occur in the material platform of choice, we examine the resulting transmon Hamiltonian. This junction allows for direct control of the single and double Cooper pair tunneling strength, and most remarkably, an anomalous magnetic flux -- i.e. a phase offset equivalent to magnetic flux, yet in zero magnetic field. Having control over these three parameters -- single and double pair tunneling and anomalous flux -- allows for optimal design of the transmon qubit. Interestingly, in this architecture, the anomalous flux is determined by the twist angle of the junction, thereby offering a novel zero-field functionality. Our key results rely on symmetry arguments, for concreteness we demonstrate the implementation of our concept using a model of moiré graphene-based c-axis junctions.
Van-der-Waals assembly enables the fabrication of novel Josephson junctions featuring an atomically sharp interface between two exfoliated and relatively twisted Bi_{2}Sr_{2}CaCu_{2}O_{8+x} (Bi2212) flakes. In a range of twist angles around 45°, the junction provides a regime where the interlayer two-Cooper pair tunneling dominates the current-phase relation. Here we propose employing this novel junction to realize a capacitively shunted qubit that we call flowermon. The d-wave nature of the order parameter endows the flowermon with inherent protection against charge-noise-induced relaxation and quasiparticle-induced dissipation. This inherently protected qubit paves the way to a new class of high-coherence hybrid superconducting quantum devices based on unconventional superconductors.
The anharmonicity of a transmon qubit, defined as the difference in energy level spacing, is a key design parameter. In transmons built from hybrid superconductor-semiconductor Josephson elements, the anharmonicity is tunable with gate voltages that control both the Josephson energy and the weak link transparency. In Sn-InAs nanowire transmons, we use two-tone microwave spectroscopy to extract anharmonicity ranging in absolute value from the transmon charging energy EcE_cEc​ to values smaller than Ec/10E_c/10Ec​/10. This behavior contrasts with the predictions of the multi-channel short-junction model, which sets a lower limit on anharmonicity at Ec/4E_c/4Ec​/4. Coherent operation of the qubit is still possible at the point of the lowest anharmonicity. These findings demonstrate the potential of quantum circuits that benefit from widely electrically tunable anharmonicity.
The quasicharge superconducting qubit realizes the dual of the transmon and shows strong robustness to flux and charge fluctuations thanks to a very large inductance closed on a Josephson junction. At the same time, a weak anharmonicity of the spectrum is inherited from the parent transmon, that introduces leakage errors and is prone to frequency crowding in multi-qubit setups. We propose a novel design that employs a quartic superinductor and confers a good degree of anharmonicity to the spectrum. The quartic regime is achieved through a properly designed chain of Josephson junction loops that shows minimal quantum fluctuations without introducing a severe dependence on the external fluxes.
Flux-tunable transmon incorporating a van der Waals superconductor via an Al/AlOx_xx​/4Hb-TaS2_22​ Josephson junction
Incorporating van der Waals (vdW) superconductors into Josephson elements extends circuit-QED beyond conventional Al/AlOx_xx​/Al tunnel junctions and enables microwave probes of unconventional condensates and subgap excitations. In this work, we realize a flux-tunable transmon whose nonlinear inductive element is an Al/AlOx_xx​/4Hb-TaS2_22​ Josephson junction. The tunnel barrier is formed by sequential deposition and full in-situ oxidation of ultrathin Al layers on an exfoliated 4Hb-TaS2_22​ flake, followed by deposition of a top Al electrode, yielding a robust, repeatable hybrid junction process compatible with standard transmon fabrication. Embedding the device in a three-dimensional copper cavity, we observe a SQUID-like flux-dependent spectrum that is quantitatively reproduced by a standard dressed transmon--cavity Hamiltonian, from which we extract parameters in the transmon regime. Across measured devices we obtain sub-microsecond energy relaxation (T1T_1T1​ from 0.080.080.08 to 0.69 μ0.69~μ0.69 μs), while Ramsey measurements indicate dephasing faster than our 161616 ns time resolution. We also find a pronounced discrepancy between the Josephson energy inferred from spectroscopy and that expected from the Ambegaokar--Baratoff relation using room-temperature junction resistances, pointing to nontrivial junction physics in the hybrid Al/AlOx_xx​/4Hb-TaS2_22​ system. Although we do not resolve material-specific subgap modes in the present geometry, this work establishes a practical route to integrating 4Hb-TaS2_22​ into coherent quantum circuits and provides a baseline for future edge-sensitive designs aimed at enhancing coupling to boundary and subgap degrees of freedom in vdW superconductors.