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Optics Express

Magnetic-free polarization rotation in an atomic vapor cell

Jiangbin Zheng, De-Kang Chai, Zhu-Bo Wang, Guang-Jie Chen, Yadong Hu, Liang Chen, Hong-Jie Fan, Yan-Lei Zhang, Chun‐Hua Dong, Chang‐Ling Zou, Guang‐Can Guo, Ming-Yong Ye, Gong-Wei Lin, Xiu‐Min Lin

Published Dec 8, 2023• 1 citation
Publisher

Abstract

Magnetic-free nonreciprocal optical devices have attracted great attention in recent years. Here, we investigated the magnetic-free polarization rotation of light in an atom vapor cell. Two mechanisms of magnetic-free nonreciprocity have been realized in ensembles of hot atoms, including electromagnetically induced transparency and optically-induced magnetization. For a linearly polarized input probe light, a rotation angle up to 86.4° has been realized with external control and pump laser powers of 10 mW and is mainly attributed to the optically-induced magnetization effect. Our demonstration offers a new approach to realize nonreciprocal devices, which can be applied to solid-state atom ensembles and may be useful in photonic integrated circuits.

DOI
10.1364/oe.510933

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Acta Physica Sinica•Jan 1, 2022•3 citations
Magnetic-free nonreciprocal optical devices have attracted great attention in recent years. Here, we investigated the magnetic-free polarization rotation of light in an atom vapor cell. Two mechanisms of magnetic-free nonreciprocity have been realized in ensembles of hot atoms, including electromagnetically induced transparency and optically-induced magnetization. For a linearly polarized input probe light, a rotation angle up to 86.4° has been realized with external control and pump laser powers of 10 mW and is mainly attributed to the optically-induced magnetization effect. Our demonstration offers a new approach to realize nonreciprocal devices, which can be applied to solid-state atom ensembles and may be useful in photonic integrated circuits.
In this work, we employ 87 Rb atoms as rotation media to manipulate the polarization of optical fields in both magnetic and magnetic-free environments. Employing the nonlinear magneto-optical rotation mechanism, we achieve a state-of-the-art magneto-optical rotation coefficient of 1.74×10 8 rad⋅T −1 ⋅m −1 which is four orders of magnitude higher than commonly employed materials. Additionally, in a magnetic-free environment, we achieve all-optical cross-polarization modulation between the pump and probe light via Rb atoms. The nonlinear magneto-optical rotation configuration introduces inventive techniques for a new type of magneto-optical modulator while the all-optical configuration paves the way for exploring photonic integrated circuit (PIC) devices free from disruptions caused by electrical or magnetic crosstalk.
Optical nonreciprocity is an essential concept in optical signal processing and communication. The traditional way to achieve nonreciprocity is using magneto-optical nonreciprocal polarization rotation, which is incompatible with existing on-chip integration due to the applied magnetic field. Here, we theoretically and experimentally realize unidirectional polarization rotation with a magnetic-free mechanism using atomic ensembles. Free-space isolators and circulators are further formed based on the nonreciprocity of polarization rotation. As only one direction of the signal changes its polarization, the forward transmission and backward isolation can be adjusted separately. Compared with the existing magnetic-free circulators that rely on high-Q factor cavities or Mach–Zehnder interferometers, we experimentally realized circulators in free space. This dramatically simplifies the magnetic-free circulator structure and provides better stability.
Results of a fairly straightforward experiment on resonant magneto-optical rotation by rubidium-87 atoms revealed strong time-dependence of the polarization plane of light emerging from atomic vapors following a sudden irradiation with a laser beam. The rotation of the plane appears as a not direct consequence of the influence of the magnetic field on atoms. Reported measurements conducted using a vapor cell without any buffer gas or an anti-relaxation wall coating show that transmitted light has initially the same (linear) polarization as the incident one. Rotation of the polarization plane caused by an axial magnetic field develops in time scales similar to the pace of establishing the optical pumping/relaxation equilibrium in the atomic ensemble. The traditional passive Faraday rotation picture providing working description for the resonant magneto-optical effects in steady-state conditions does not explain the observed sequence of evolution of the polarization. The picture has to be augmented with analysis of time dependence in the spatial distribution of relevant quantum states within the atomic ensemble as well as longitudinal and transversal intensity profiles of the light beam. Isolation of external effects caused by the optical pumping and relaxation processes from consequences of internal atomic coherences should uncover more details of mechanisms of the latter in the presence of magnetic field. Plentitude of data available from time-dependent polarization measurements provides strong incentives for further development and tests of comprehensive models of coherent interactions of atomic ensembles with radiation and possibly a base for additional advance in understanding and applications of these phenomena.
Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.
Nonlinear resonances in alkali metal vapor, which are detected by the magneto-optical rotation of the linear polarization of light, are actively used in quantum magnetometry to fabricate atomic magnetometers. The magneto-optical rotation in most such sensors is due to magnetic birefringence, and rotation angles usually do not exceed tens of milliradians. In this work, an experiment where magneto-optical resonances of linear polarization rotation of a probe wave are due to strong dichroism induced in a medium by a counterpropagating pump wave has been proposed. Both waves are in resonance with the Fg = 2 → Fe = 1 optical transition in the 87Rb D1 line (λ ≈ 795 nm). Experiments have been carried out with a 2-cm-long cylindrical cell filled with a buffer gas, and the maximum rotation angle is ≈390 mrad (22°) at a width of resonance of about 300 nT. The results show that the configuration proposed for the observation of magneto-optical rotation is promising for the fabrication of compact high-sensitivity atomic magnetometers.
Owing to the potential applications in all-optical quantum information processing and quantum optical networks, magnet-free optical non-reciprocity transmission has attracted great interest and has been studied in many fields, such as parity-time-symmetry enhanced nonlinearity, optomechanical systems, photonic crystal, cold atomic Bragg lattices, chiral quantum optics, and hot atoms. In particular, the random thermal motion of hot atoms can be a useful resource to realize optical non-reciprocity. Here in this work, based on the susceptibility-momentum-locking of atomic thermal motion and the strong coupling characteristics of cavities, a magnetic-free optical reciprocity-nonreciprocity transmission conversion scheme is designed and realized through the atom-cavity compound system. Theoretical and experimental analysis show that the coupling field conditions determine the nonreciprocity of the system. Under the action of single traveling-wave field, the nonreciprocity in hot atoms depends on the propagation direction of the coupling field due to the Doppler effect. Therefore, by changing the opening and closing of the opposite coupling field, the two-way single channel optical nonreciprocal transmission based on intracavity electromagnetically induced transparency can be controlled. When the two coupling fields propagate simultaneously in the opposite directions, however, the cavity transmission changes from single-dark-state to double-dark-state peaks, in which the reciprocity outputs depend on the frequency difference between the two coupling fields. By tuning the frequency difference, the two-way multi-channel reciprocal-nonreciprocal transmission regulation based on double dark polar peaks can be realized. The study can be applied to all-optical quantum devices and quantum information processing, such as optical transistors, optical switching and routing, and quantum gate manipulation.