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ACS Photonics

Backscattering-Induced Chiral Absorption in Optical Microresonators

Linhao Ren, Shixing Yuan, Song Zhu, Lei Shi, Xinliang Zhang

Published Oct 6, 2023• 17 citations
Publisher

Abstract

Chirality in micro- and nanophotonic structures is crucial for both fundamental research and applied technology. Here, we experimentally demonstrate chiral absorption via backscattering in a single whispering-gallery microresonator under simultaneous excitation from both ports. Remarkably, this scheme does not rely on any nonlinear effects or the breaking of parity or time-reversal symmetry. These intriguing phenomena occur due to the interference between the clockwise- and counterclockwise-propagating light fields induced by the backscattering. Furthermore, we also achieve the chiral optical states in a coupled-microresonator system, which can be utilized to manipulate the electromagnetically induced transparency or absorption effect. Our work proposes a linear and all-optical scheme to realize chiral optical states, which can help control the light flow in photonic systems with a high operation rate.

DOI
10.1021/acsphotonics.3c01115

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Chirality in micro- and nanophotonic structures is crucial for both fundamental research and applied technology. Here, we experimentally demonstrate chiral absorption via backscattering in a single whispering-gallery microresonator under simultaneous excitation from both ports. Remarkably, this scheme does not rely on any nonlinear effects or the breaking of parity or time-reversal symmetry. These intriguing phenomena occur due to the interference between the clockwise- and counterclockwise-propagating light fields induced by the backscattering. Furthermore, we also achieve the chiral optical states in a coupled-microresonator system, which can be utilized to manipulate the electromagnetically induced transparency or absorption effect. Our work proposes a linear and all-optical scheme to realize chiral optical states, which can help control the light flow in photonic systems with a high operation rate.
The chiral light-matter interaction, which shows great potential in applications ranging from photonic devices to quantum information processing, can be achieved with the development of recent experimental advances of the fabrication technologies on nanoscales. Traditionally, the chiral optics based on spin-momentum locking in micro- and nanophotonics could be observed only for specific optical modes, such as the transverse magnetic mode. Here in this study, we investigate that the chirality of a whispering-gallery-mode (WGM) microresonator can be well controlled with assistance from coupled Rydberg-atom ensembles. The presented asymmetric backscattering also originates from interferences between scattered optical modes in the WGM microresonator, which is proposed by Wiersig [Phys. Rev. A 84, 063828 (2011)]. Therefore the flow of light can be well controlled, and the statistical properties of photons could be changed by regulating this asymmetric coupling. Most importantly, its universal chiral property is not limited by specific optical modes which may also be used as optical diodes and routers.
Summary form only given. Controlling the interaction of light and matter is the basis for diverse applications ranging from light technology to quantum information processing. Nowadays, many of these applications are based on nanophotonic structures. It turns out that the confinement of light in such nanostructures imposes an inherent link between its local polarization and its propagation direction, also referred to as spin-momentum locking of light [1]. Remarkably, this leads to chiral, i.e., propagation direction-dependent effects in the emission and absorption of light, and elementary processes of light-matter interaction are fundamentally altered. For example, when coupling plasmonic particles or atoms to evanescent fields, the intrinsic mirror symmetry of the particles' emission can be broken. In our group, we observed this effect in the interaction between single rubidium atoms and the evanescent part of a light field that is confined by continuous total internal reflection in a whispering-gallery-mode microresonator [2]. In the following, this allowed us to realize chiral nanophotonic interfaces in which the emission direction of light into the structure is controlled by the polarization of the excitation light [3] or by the internal quantum state of the emitter [4], respectively. Moreover, we employed this chiral interaction to demonstrate an integrated optical isolator [5] as well as an integrated optical circulator [6] which operate at the single-photon level and which exhibit low loss. The latter are the first two examples of a new class of nonreciprocal nanophotonic devices which exploit the chiral interaction between single quantum emitters and transversally confined photons.
Coherently manipulating single photons in nanophotonic structures with unidirectional propagation is one of the central goals for integrated quantum information processing. Photonic devices constructed by a single atom coupled to a whispering-gallery-mode microresonator (WGMM) with nonideal chiral photon-atom interactions inevitably induce undesired photon scattering. Here, an external scatterer is introduced to the WGMM to cancel the reflection of signal photons by an atom due to nonideal chiral interactions. By properly tuning the positions of the scatterer, destructive and constructive interferences between reflected photons of different pathways are utilized to control the reflection properties of single incident photons. The results show that the reflection probabilities can be suppressed by applying the interplay between chirality and backscattering. Constructing perfect destructive interferences directly leads to unidirectional propagation even when the photon-atom interactions are not ideal. Because the amplitudes of the reflected photons produced by the scatterer can be enhanced to meet requirements of perfect destructive interfering processes, unidirectional propagation is preserved against dissipations.
Optical behavior analogous to electromagnetically induced transparency and absorption is observed in experiments using coupled fused-silica microspheres. This behavior results from interference between coresonant whispering-gallery modes of the two spheres. Coupled-resonator-induced transparency and absorption are observed. Which effect is seen depends on the strength of coupling of incident light from a tapered fiber into the first sphere and on the strength of coupling between the two spheres. The observed effects can enhance microresonator performance in various applications.
Nanophotonic components allow the control of the flow of light in integrated optical environments. Thereby, the light’s strong confinement leads to an inherent link between its local polarization and propagation direction which fundamentally alters the physics of light-matter interaction and gives rise to phenomena such as directional emission and direction-dependent coupling strengths [1]. I will present the underlying principles of this chiral light-matter interaction and its consequences for integrated applications [1]. In particular, I will show how we employ this effect to control the direction of spontaneous emission [2] and to realize low-loss nonreciprocal transmission at the single-photon level through a silica nanofiber [3]. We use two different approaches where either an ensemble of spin-polarized atoms is weakly coupled to a nanofiber or a single atom is strongly coupled to the nanofiber via a whispering-gallery-mode resonator. The resulting optical isolators show a strong imbalance between the transmissions in forward and reverse direction and, at the same time, a forward transmissions exceeding 70%. We extended this system to a 4-port device, where a single atom routes photons nonreciprocally from one fiber port to the next. This realizes a quantum optical circulator [4] which can even be prepared in a superposition of its operational modes. The demonstrated systems exemplify a new class of (quantum) nanophotonic devices that are ideally suited for photonic quantum information processing and quantum simulation. [1] Nature 541, 473, (2017). [2] Science 346, 67 (2014). [3] Phys. Rev. X 5, 041036 (2015). [4] Science 354, 1577 (2016).
Abstract Transparency and perfect absorption are two contradictory terms; a perfect absorber never permits waves to transmit through. However, this statement only remains true in the linear regime, where the nonlinearity has been omitted and the physical system like the perfect absorber is not affected by the incoming waves. Here we experimentally demonstrate an intriguing self-induced transparency effect in a perfectly absorbing optical microcavity, which perfectly absorbs any incoming waves at the low power level, but allows a portion of waves to be transmitted at the higher power due to the nonlinear coupling between the fundamental and its second harmonic modes. Moreover, the asymmetric scattering nature of the microcavity enables a chiral and unidirectional reflection in one of the input ports, this leads to asymmetric and chiral coherent control of the perfect absorption states through phase varying. More importantly, such chiral behaviors also empower the chiral emission of second-harmonic generation with a high distinct ratio in the transparency state. These results pave the way for controllable transparency in a wide range of fields in optics, microwaves, acoustics, mechanics, and matter waves.