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Optics Express

SERF-like magnetometry in room-temperature environment

Guzhi Bao, Jun Chen, Ruiqi Wang, L. Q. Chen, Weiping Zhang

Published Sep 19, 2023• 6 citations
Publisher

Abstract

We demonstrate an atomic magnetometry using amplitude-modulated pumping and hyperfine repumping techniques in a paraffin-coated cell. By exploiting the constructive interference between spins polarized by the pump beam and an additional repump beam, we observe a three-fold increase in the amplitude of magnetic resonance, along with a reduction in linewidth by approximately two times. The implementation of the repump beam effectively narrows the linewidth, demonstrating successful suppression of spin-exchange relaxation. This reduction in relaxation rate, combined with the enhanced signal, significantly improves the sensitivity of the magnetometer. Consequently, our technique offers a promising approach for achieving SERF-like magnetometry with sub-fT-level sensitivity in Earth-field range and room-temperature environment.

DOI
10.1364/oe.500875

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We demonstrate an atomic magnetometry using amplitude-modulated pumping and hyperfine repumping techniques in a paraffin-coated cell. By exploiting the constructive interference between spins polarized by the pump beam and an additional repump beam, we observe a three-fold increase in the amplitude of magnetic resonance, along with a reduction in linewidth by approximately two times. The implementation of the repump beam effectively narrows the linewidth, demonstrating successful suppression of spin-exchange relaxation. This reduction in relaxation rate, combined with the enhanced signal, significantly improves the sensitivity of the magnetometer. Consequently, our technique offers a promising approach for achieving SERF-like magnetometry with sub-fT-level sensitivity in Earth-field range and room-temperature environment.
We investigated the operation of an all-optical rubidium-87 atomic magnetometer with amplitude-modulated light. To study the suppression of spin-exchange relaxation, three schemes of pumping were implemented with room-temperature and heated paraffin coated vacuum cells. Efficient pumping and accumulation of atoms in the F=2 ground state were obtained. However, the sought-for narrowing of the resonance lines has not been achieved. A theoretical analysis of the polarization degree is presented to illustrate the absence of light narrowing due to radiation trapping at high temperature.
For the experimental implementation of an optically pumped atomic magnetometer, the magnetic resonance signal with a narrow linewidth and a high signal-to-noise ratio (SNR) is required for achieving a high sensitivity. Using 795-nm laser as both the pumping and the probe laser, we compare the magnetic resonance signals from different rubidium atomic vapor cells and investigate the variations of magnetic resonance signals with temperature. Optimized magnetic resonance signal is achieved with a paraffin-coated rubidium atomic vapor cell. Then the 780-nm laser at rubidium D2 line is introduced as a repumping laser, and we explore the changes of linewidth and SNR of the magnetic resonance signal under different power of the pumping laser and the repumping laser. Owing to the 780-nm repumping laser beam, the signal amplitude of rubidium-85 magnetic resonance signal is improved remarkably because more rubidium-85 atoms are spin- polarized by the 795-nm pumping laser beam. At the same time, the linewidth of rubidium-85 magnetic resonance signal is roughly not broadened anymore. We realize a closed-loop optically pumped rubidium-85 atomic magnetometer with a bandwidth of ~1.2 kHz, and the sensitivity is calibrated to be ~245.5 pT/Hz1/2 only with the 795-nm pumping laser beam. Owing to the employment of the 780-nm repumping laser beam, the sensitivity is improved to be ~26.4 pT/Hz1/2 which is improved roughly by one order of magnitude. We also calibrate the measurement accuracy and deviation of a commercial fluxgate magnetometer by using the enhanced rubidium magnetic resonance signal.
We describe a Cs atomic magnetometer operating in the spin-exchange-relaxation-free (SERF) regime. With a vapor cell temperature of $103\text{ }\ifmmode^\circ\else\textdegree\fi{}\text{C}$ we achieve intrinsic magnetic resonance widths $\ensuremath{\Delta}B=17\text{ }\ensuremath{\mu}\text{G}$ corresponding to an electron spin-relaxation rate of $300\text{ }{\text{s}}^{\ensuremath{-}1}$ when the spin-exchange rate is ${\ensuremath{\Gamma}}_{\text{SE}}=14\text{ }000\text{ }{\text{s}}^{\ensuremath{-}1}$. We also observe an interesting narrowing effect due to diffusion. Signal-to-noise measurements yield a sensitivity of about 400 pG/Hz400\text{ }\text{pG}/\sqrt{\text{Hz}}400 pG/Hz​. Based on photon shot noise, we project a sensitivity of 40 pG/Hz40\text{ }\text{pG}/\sqrt{\text{Hz}}40 pG/Hz​. A theoretical optimization of the magnetometer indicates sensitivities on the order of 2 pG/Hz2\text{ }\text{pG}/\sqrt{\text{Hz}}2 pG/Hz​ should be achievable in a 1 cm31\text{ }{\text{cm}}^{3}1 cm3 volume. Because Cs has a higher saturated vapor pressure than other alkali metals, SERF magnetometers using Cs atoms are particularly attractive in applications requiring lower temperatures.
Abstract The chip-scale hybrid optical pumping spin-exchange relaxation-free (SERF) atomic magnetometer with a single-beam arrangement has prominent applications in biomagnetic measurements because of its outstanding features, including ultrahigh sensitivity, an enhanced signal-to-noise ratio, homogeneous spin polarization and a much simpler optical configuration than other devices. In this work, a miniaturized single-beam hybrid optical pumping SERF atomic magnetometer based on a microfabricated atomic vapor cell is demonstrated. Although the optically thin Cs atoms are spin-polarized, the dense Rb atoms determine the experimental results. The enhanced signal strength and narrowed resonance linewidth are experimentally proven, which shows the superiority of the proposed magnetometer scheme. By using a differential detection scheme, we effectively suppress optical noise with an approximate five-fold improvement. Moreover, the cell temperature markedly affects the performance of the magnetometer. We systematically investigate the effects of temperature on the magnetometer parameters. The theoretical basis for these effects is explained in detail. The developed miniaturized magnetometer has an optimal magnetic sensitivity of 20 fT/Hz 1/2 . The presented work provides a foundation for the chip-scale integration of ultrahighly sensitive quantum magnetometers that can be used for forward-looking magnetocardiography (MCG) and magnetoencephalography (MEG) applications.
We demonstrate the bandwidth enhancement of an all-optical spin-exchange relaxation-free (SERF) magnetometer based on amplitude-modulated (AM) light. Alkali metal atoms are modulated directly by the pump beam instead of the modulation field or radio frequency field. The first harmonic demodulation of an AM SERF magnetometer with a modulation intensity of 15 kHz results in a high bandwidth of over 11 kHz with a sensitivity of 20 fT/Hz1/2 at 30 Hz and 60 fT/Hz1/2 at 10 kHz. Meanwhile, the AM SERF magnetometer with DC demodulation presents the same sensitivity as a traditional DC SERF magnetometer (6 fT/Hz1/2 at 30 Hz). The presented technique for modulating the amplitude of the pump beam allows AM SERF magnetometers to enter the domain of high-bandwidth magnetometers and opens the door to many areas that are inaccessible to conventional magnetometers.
We describe our approach to atomic magnetometry based on the push-pull optical pumping technique. Cesium vapor is pumped and probed by a resonant laser beam whose circular polarization is modulated synchronously with the spin evolution dynamics induced by a static magnetic field. The magnetometer is operated in a phase-locked loop, and it has an intrinsic sensitivity below 20fT/Hz, using a room temperature paraffin-coated cell. We use the magnetometer to monitor magnetic field fluctuations with a sensitivity of 300fT/Hz.